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SARLEP SIGNED

Simulation and Understanding of the Atmospheric Radical Budget for Regions with Large Emissions from Plants

Total Cost €

EC-Contrib. €

Partnership

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Outcomes and
results

SARLEP project word cloud

Explore the words cloud of the SARLEP project. It provides you a very rough idea of what is the project "SARLEP" about.

rural species advantages quantified single removal simulation saphir budget ozone laboratory greatest life calculations radical gap secondary chamber organic biosphere hydroxyl influence plants suggest linked complexity chemical greenhouse causes emissions found aerosol oxidized photochemically remote cleansing accurate entire sources experiments planet considerable efficiency emitted destruction oxidation lifetime gases atmosphere quantify natural accurately experimental reactions overlooked atmospherically quantum instrumentation anthropogenic significantly pollutants quality recycling predicting innovative compounds precise host couplings chemistry plant lack climate radicals comprehensively self biogenic harmful acids close rates atmospheric regions

Project "SARLEP" data sheet

The following table provides information about the project.

Coordinator	FORSCHUNGSZENTRUM JULICH GMBH Organization address address: WILHELM JOHNEN STRASSE city: JULICH postcode: 52428 website: www.fz-juelich.de contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.
Coordinator Country	Germany [DE]
Total cost	1˙850˙000 €
EC max contribution	1˙850˙000 € (100%)
Programme	1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
Code Call	ERC-2015-CoG
Funding Scheme	ERC-COG
Starting year	2016
Duration (year-month-day)	from 2016-03-01 to 2021-02-28

Partnership

Take a look of project's partnership.

#	participants	country	role	EC contrib. [€]
1	FORSCHUNGSZENTRUM JULICH GMBH FORSCHUNGSZENTRUM JULICH GMBH Organization address address: WILHELM JOHNEN STRASSE city: JULICH postcode: 52428 website: www.fz-juelich.de contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	DE (JULICH)	coordinator	1˙850˙000.00

Map

Project objective

Atmospheric pollutants emitted by natural and anthropogenic sources influence significantly the quality of life on our planet. Their removal in the atmosphere is controlled by their reactions with photochemically produced hydroxyl radicals. Recent findings from experimental studies and quantum-chemical calculations suggest that an important part of atmospheric radical chemistry, which is directly linked to the self-cleansing ability of our atmosphere, has been overlooked. This causes considerable uncertainty in our understanding of the couplings between the biosphere, atmospheric chemistry and climate. The greatest impact of this lack of understanding has been found for regions with large emissions of organic compounds from plants in remote or rural areas. Within this project, the oxidation of organic compounds will be comprehensively investigated for the most important, biogenic organic compounds. The innovative experimental approach will quantify the radical destruction and production rates in experiments in the unique atmosphere simulation chamber SAPHIR at the host institution. These experiments aim to close the gap between laboratory and field studies. The advantages are: (1) Experiments will be conducted under atmospherically relevant conditions. (2) Radical recycling efficiency will be quantified for the entire chemical system, not just for single reactions. (3) The complexity of the chemical system studied will be increased from single compounds to natural plant emissions. New innovative instrumentation will be developed for accurate and precise measurements of radical species and oxidized organic compounds. These are also of great interest beyond this project. The results of this project will improve our understanding of atmospheric radical chemistry required for accurately predicting the atmospheric radical budget, the formation of harmful secondary pollutants such as ozone, acids and aerosol and the lifetime of greenhouse gases affecting climate change.

Publications

List of publications.
year	authors and title	journal	last update
2017	Hendrik Fuchs, Anna Novelli, Michael Rolletter, Andreas Hofzumahaus, Eva Y. Pfannerstill, Stephan Kessel, Achim Edtbauer, Jonathan Williams, Vincent Michoud, Sebastien Dusanter, Nadine Locoge, Nora Zannoni, Valerie Gros, Francois Truong, Roland Sarda-Esteve, Danny R. Cryer, Charlotte A. Brumby, Lisa K. Whalley, Daniel Stone, Paul W. Seakins, Dwayne E. Heard, Coralie Schoemaecker, Marion Blocquet, Sebastien Coudert, Sebastien Batut, Christa Fittschen, Alexander B. Thames, William H. Brune, Cheryl Ernest, Hartwig Harder, Jennifer B. A. Muller, Thomas Elste, Dagmar Kubistin, Stefanie Andres, Birger Bohn, Thorsten Hohaus, Frank Holland, Xin Li, Franz Rohrer, Astrid Kiendler-Scharr, Ralf Tillmann, Robert Wegener, Zhujun Yu, Qi Zou, Andreas Wahner Comparison of OH reactivity measurements in the atmospheric simulation chamber SAPHIR published pages: 4023-4053, ISSN: 1867-8548, DOI: 10.5194/amt-10-4023-2017	Atmospheric Measurement Techniques 10/10	2019-06-18
2017	Martin Kaminski, Hendrik Fuchs, Ismail-Hakki Acir, Birger Bohn, Theo Brauers, Hans-Peter Dorn, Rolf HÃ¤seler, Andreas Hofzumahaus, Xin Li, Anna Lutz, Sascha Nehr, Franz Rohrer, Ralf Tillmann, Luc Vereecken, Robert Wegener, Andreas Wahner Investigation of the <i>Î²</i>-pinene photooxidation by OH in the atmosphere simulation chamber SAPHIR published pages: 6631-6650, ISSN: 1680-7324, DOI: 10.5194/acp-17-6631-2017	Atmospheric Chemistry and Physics 17/11	2019-06-18
2018	Hendrik Fuchs, Sascha Albrecht, Ismailâ€“Hakki Acir, Birger Bohn, Martin Breitenlechner, Hans-Peter Dorn, Georgios I. Gkatzelis, Andreas Hofzumahaus, Frank Holland, Martin Kaminski, Frank N. Keutsch, Anna Novelli, David Reimer, Franz Rohrer, Ralf Tillmann, Luc Vereecken, Robert Wegener, Alexander Zaytsev, Astrid Kiendler-Scharr, Andreas Wahner Investigation of the oxidation of methyl vinyl ketone (MVK) by OH radicals in the atmospheric simulation chamber SAPHIR published pages: 8001-8016, ISSN: 1680-7324, DOI: 10.5194/acp-18-8001-2018	Atmospheric Chemistry and Physics 18/11	2019-06-18
2018	Anna Novelli, Martin Kaminski, Michael Rolletter, Ismail-Hakki Acir, Birger Bohn, Hans-Peter Dorn, Xin Li, Anna Lutz, Sascha Nehr, Franz Rohrer, Ralf Tillmann, Robert Wegener, Frank Holland, Andreas Hofzumahaus, Astrid Kiendler-Scharr, Andreas Wahner, Hendrik Fuchs Evaluation of OH and HO<sub>2</sub> concentrations and their budgets during photooxidation of 2-methyl-3-butene-2-ol (MBO) in the atmospheric simulation chamber SAPHIR published pages: 11409-11422, ISSN: 1680-7324, DOI: 10.5194/acp-18-11409-2018	Atmospheric Chemistry and Physics 18/15	2019-06-18
2019	Sascha R. Albrecht, Anna Novelli, Andreas Hofzumahaus, Sungah Kang, Yare Baker, Thomas Mentel, Andreas Wahner, Hendrik Fuchs Measurements of hydroperoxy radicals (HO<sub>2</sub>) at atmospheric concentrations using bromide chemical ionisation mass spectrometry published pages: 891-902, ISSN: 1867-8548, DOI: 10.5194/amt-12-891-2019	Atmospheric Measurement Techniques 12/2	2019-05-09

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