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ZeBiolApp SIGNED

Developing Structure-Reactivity Relationships of the Zeolite Catalysed Bio-alcohol Mediated Aromatic Alkylation Processes via a Multi-Spectroscopic Investigative Approach

Total Cost €

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EC-Contrib. €

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Partnership

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 ZeBiolApp project word cloud

Explore the words cloud of the ZeBiolApp project. It provides you a very rough idea of what is the project "ZeBiolApp" about.

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Project "ZeBiolApp" data sheet

The following table provides information about the project.

Coordinator
UNIVERSITEIT UTRECHT 

Organization address
address: HEIDELBERGLAAN 8
city: UTRECHT
postcode: 3584 CS
website: www.uu.nl

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Netherlands [NL]
 Project website https://www.uu.nl/en/research/inorganic-chemistry-catalysis
 Total cost 177˙598 €
 EC max contribution 177˙598 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2015
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2016
 Duration (year-month-day) from 2016-06-01   to  2018-05-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    UNIVERSITEIT UTRECHT NL (UTRECHT) coordinator 177˙598.00

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 Project objective

A top priority of the European Union under the Horizon 2020 protocol is that chemical industries must reduce their dependence on fossil fuels. In the petro-chemical industry, aromatic alkylation processes using olefins as alkylating agents and zeolites or inorganic Lewis acids as catalysts are still exclusively depending on fossil fuels. Other limitations of these processes include corrosion, toxicity, contamination and undesired side reactions. Hence, I will develop new zeolite-based catalytic technologies for the alkylation of aromatics using bio-alcohols (derived from biomass) as alkylating agents. Here I hypothesize that MWW type medium pore zeolites and MTW/MOR type large pore zeolites are ideal catalysts for aromatic alkylation using short and long chain alcohols, respectively. In this regard, the specific project aims are: (1) evaluation of these specific medium and large pore zeolites for the production of alkylated aromatics with high selectivity and purity in bio-alcohol mediated aromatic alkylation processes, (2) proper process optimization by tuning all reaction parameters in order to achieve excellent selectivity at reasonably higher reactivity and (3) elucidation of the catalytic cycle and deactivation mechanism and establishment of the structure-property-function relationships through the application of advanced in situ/operando (micro-)spectroscopic techniques. Altogether, the acquired knowledge from this research project will help the chemical community to design future catalyst materials for bio-alcohol mediated aromatic alkylation processes. This project will be carried out within Inorganic Chemistry and Catalysis (ICC) group at Utrecht University under the supervision of Prof. Bert M. Weckhuysen. This will allow me to develop my knowledge and skills in the fields of heterogeneous catalysis and in situ spectroscopy in order to steer my future as an independent researcher in the direction of heterogeneous catalysis for organic syntheses.

 Publications

year authors and title journal last update
List of publications.
2018 Abhishek Dutta Chowdhury, Alessandra Lucini Paioni, Klaartje Houben, Gareth T. Whiting, Marc Baldus, Bert M. Weckhuysen
Bridging the Gap between the Direct and Hydrocarbon Pool Mechanisms of the Methanol-to-Hydrocarbons Process
published pages: 8095-8099, ISSN: 1433-7851, DOI: 10.1002/anie.201803279
Angewandte Chemie International Edition 57/27 2019-06-13
2018 Abhishek Dutta Chowdhury, Klaartje Houben, Gareth T. Whiting, Sang-Ho Chung, Marc Baldus, Bert M. Weckhuysen
Electrophilic aromatic substitution over zeolites generates Wheland-type reaction intermediates
published pages: 23-31, ISSN: 2520-1158, DOI: 10.1038/s41929-017-0002-4
Nature Catalysis 1/1 2019-06-13

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The information about "ZEBIOLAPP" are provided by the European Opendata Portal: CORDIS opendata.

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