Explore the words cloud of the ELICOS project. It provides you a very rough idea of what is the project "ELICOS" about.
The following table provides information about the project.
TECHNISCHE UNIVERSITAET MUENCHEN
|Coordinator Country||Germany [DE]|
|Total cost||2˙357˙901 €|
|EC max contribution||2˙357˙901 € (100%)|
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
|Duration (year-month-day)||from 2016-01-01 to 2020-12-31|
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|1||TECHNISCHE UNIVERSITAET MUENCHEN||DE (MUENCHEN)||coordinator||2˙357˙901.00|
Photochemical reactions are induced by ultraviolet or visible light and they enable the construction of molecular skeletons that are difficult or even impossible to access by any other means. In order to secure a widespread application of these reactions in organic synthesis and in order to make the respective products available for high-tech applications, it is required that photochemical reactions can be performed enantioselectively, i.e. that the three-dimensional architecture of the product molecules is unambiguously defined. Despite some progress in recent years, this challenge has as yet remained unsolved. It is the objective of this proposal to develop catalytic methods that allow the enantioselective synthesis of a broad variety of compound classes by light-induced reactions. The mode of action of potential catalysts is based on energy transfer or on wavelength-selective excitation. In the former scenario, the substrate-catalyst complex will be held together by non-covalent interactions, which position the substrate for an efficient energy transfer and for an enantioselective approach of the reagent. In the latter approach, acid-base interactions in the substrate-catalyst complex will lead to a significant bathochromic absorption shift of the substrate, enabling a selective excitation within the complex and a subsequent enantioselective reaction pathway within a spatially defined chiral environment. Both approaches include the option to employ sunlight as the exclusive energy source to drive enantioselective processes without the need to apply external heat or pressure.
|year||authors and title||journal||last update|
Florian Mayr, Richard Brimioulle, Thorsten Bach
A Chiral Thiourea as a Template for Enantioselective Intramolecular [2 + 2] Photocycloaddition Reactions
published pages: 6965-6971, ISSN: 0022-3263, DOI: 10.1021/acs.joc.6b01039
|The Journal of Organic Chemistry 81/16||2019-07-02|
Thorsten Bach, Florian Mayr, Lisa-Marie Mohr, Elsa Rodriguez
Synthesis of Chiral Thiourea-Thioxanthone Hybrids
published pages: 5238-5250, ISSN: 0039-7881, DOI: 10.1055/s-0036-1590931
Thorsten Bach, Lisa-Marie Mohr
Intermolecular [2+2] Photocycloaddition of Î²-Nitrostyrenes to Olefins upon Irradiation with Visible Light
published pages: 2946-2950, ISSN: 0936-5214, DOI: 10.1055/s-0036-1588524
Christoph Brenninger, Thorsten Bach
Î±-Thio Carbocations (Thionium Ions) as Intermediates in BrÃ¸nsted Acid-Catalyzed Reactions of Enone-Derived 1,3-Dithianes and 1,3-Dithiolanes
published pages: 623-629, ISSN: 1022-5528, DOI: 10.1007/s11244-018-0905-6
|Topics in Catalysis 61/7-8||2019-07-02|
Fabian M. HÃ¶rmann, Tim S. Chung, Elsa Rodriguez, Matthias Jakob, Thorsten Bach
Evidence for Triplet Sensitization in the Visible-Light-Induced [2+2]â€…Photocycloaddition of Eniminium Ions
published pages: 827-831, ISSN: 1433-7851, DOI: 10.1002/anie.201710441
|Angewandte Chemie International Edition 57/3||2019-07-02|
Saner Poplata, Thorsten Bach
Enantioselective Intermolecular [2+2] Photocycloaddition Reaction of Cyclic Enones and Its Application in a Synthesis of (âˆ’)-Grandisol
published pages: 3228-3231, ISSN: 0002-7863, DOI: 10.1021/jacs.8b01011
|Journal of the American Chemical Society 140/9||2019-07-02|
Saner Poplata, Andreas TrÃ¶ster, You-Quan Zou, Thorsten Bach
Recent Advances in the Synthesis of Cyclobutanes by Olefin [2â€¯+â€¯2] Photocycloaddition Reactions
published pages: 9748-9815, ISSN: 0009-2665, DOI: 10.1021/acs.chemrev.5b00723
|Chemical Reviews 116/17||2019-07-02|
Christoph Brenninger, John D. Jolliffe, Thorsten Bach
Chromophore Activation of Î±,Î²-Unsaturated Carbonyl Compounds and Its Application to Enantioselective Photochemical Reactions
published pages: 14338-14349, ISSN: 1433-7851, DOI: 10.1002/anie.201804006
|Angewandte Chemie International Edition 57/44||2019-07-02|
Christoph Brenninger, Alexander PÃ¶thig, Thorsten Bach
BrÃ¸nsted Acid Catalysis in Visible-Light-Induced [2+2]â€…Photocycloaddition Reactions of Enone Dithianes
published pages: 4337-4341, ISSN: 1433-7851, DOI: 10.1002/anie.201700837
|Angewandte Chemie International Edition 56/15||2019-07-02|
Sachin G. Modha, Alexander PÃ¶thig, Andreas Dreuw, Thorsten Bach
[6Ï€] Photocyclization to cis -Hexahydrocarbazol-4-ones: Substrate Modification, Mechanism, and Scope
published pages: 1139-1153, ISSN: 0022-3263, DOI: 10.1021/acs.joc.8b03144
|The Journal of Organic Chemistry 84/3||2019-03-25|
Simone Stegbauer, Christian Jandl, Thorsten Bach
Enantioselective Lewis Acid Catalyzed ortho Photocycloaddition of Olefins to Phenanthrene-9-carboxaldehydes
published pages: 14593-14596, ISSN: 1433-7851, DOI: 10.1002/anie.201808919
|Angewandte Chemie International Edition 57/44||2019-03-25|
Verena EdtmÃ¼ller, Alexander PÃ¶thig, Thorsten Bach
Enantioselective photocyclisation reactions of 2-aryloxycyclohex-2-enones mediated by a chiral copper-bisoxazoline complex
published pages: 5037-5048, ISSN: 0040-4020, DOI: 10.1016/j.tet.2017.05.005
You-Quan Zou, Fabian M. HÃ¶rmann, Thorsten Bach
Iminium and enamine catalysis in enantioselective photochemical reactions
published pages: 278-290, ISSN: 0306-0012, DOI: 10.1039/c7cs00509a
|Chemical Society Reviews 47/2||2019-07-02|
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