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Opendata, web and dolomites

CATLIGCAR SIGNED

Designing Novel Efficient Catalytic Strategies for the Transformation of Lignocellulose into Lignin-derived Chemicals and Valorisable Carbohydrates

Total Cost €

EC-Contrib. €

Partnership

Views

Outcomes and
results

CATLIGCAR project word cloud

Explore the words cloud of the CATLIGCAR project. It provides you a very rough idea of what is the project "CATLIGCAR" about.

mechanistic tested solvent donor reactive h2 fraction kinetic varying fossil minimizing economic tuned family structure synergistic redox ethanol acidic strength ni stability context strategy ing superior enriched exposure planes ruthenium sites hemicellulose catalyst ru tremendous class pot alternative pd social cellulose integration reductive polyhedra abundant zinc techniques selective catalytic biomass size nickel hemi particles oxide catalysts acid lewis received chemicals efficiency aid spheres enhanced rods interactions palladium nanoscale renewable simultaneously metals efficient conversion zno multifunctional fractionation retaining reusability understand nanoparticles lignocellulose relationships effect heterogeneous lignin dispersed crystal shape crlf analytical noble proper fuels paper solid

Project "CATLIGCAR" data sheet

The following table provides information about the project.

Coordinator	KATHOLIEKE UNIVERSITEIT LEUVEN Organization address address: OUDE MARKT 13 city: LEUVEN postcode: 3000 website: www.kuleuven.be contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.
Coordinator Country	Belgium [BE]
Total cost	172˙800 €
EC max contribution	172˙800 € (100%)
Programme	1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
Code Call	H2020-MSCA-IF-2016
Funding Scheme	MSCA-IF-EF-ST
Starting year	2017
Duration (year-month-day)	from 2017-10-01 to 2019-09-30

Partnership

Take a look of project's partnership.

#	participants	country	role	EC contrib. [€]
1	KATHOLIEKE UNIVERSITEIT LEUVEN KATHOLIEKE UNIVERSITEIT LEUVEN Organization address address: OUDE MARKT 13 city: LEUVEN postcode: 3000 website: www.kuleuven.be contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	BE (LEUVEN)	coordinator	172˙800.00

Map

Project objective

The utilization of renewable lignocellulose biomass (composed of cellulose, hemicellulose and lignin) alternative to fossil fuels is crucial for long-term economic and social stability. In this context, the catalytic reductive lignocellulose fractionation (CRLF) process has received tremendous research interest as this strategy enables one-pot conversion of lignocellulose into useful lignin-derived chemicals, while retaining a solid (hemi)cellulose fraction that can be used for the production of fuels, chemicals or paper. The development of promising heterogeneous catalysts having abundant redox and acid properties, along with the application of a proper solvent is a great challenge for efficient CRLF process.

Nanoscale palladium-nickel (Pd-Ni) and ruthenium-nickel (Ru-Ni) particles dispersed on shape-controlled zinc oxide (ZnO) are considered to be a unique class of heterogeneous catalysts due to the size- and shape-tuned catalytic properties. The integration of Ni with Pd and Ru can provide new, enriched, selective redox sites and simultaneously minimizing the use of noble metals. As well, controlling the shape of ZnO particles allows a selective exposure of reactive crystal planes, resulting in enhanced Lewis acidic strength. Thus, the synergistic interactions of Pd-Ni and Ru-Ni nanoparticles with the shape-controlled ZnO will provide superior redox and acid properties that can show a promising effect in CRLF process. Therefore, this project aims to develop a family of novel multifunctional M-Ni/ZnO (M = Pd, Ru) catalysts by varying the ZnO shape (spheres, rods and polyhedra). A range of analytical techniques will be used to understand the catalysts’ properties and aid catalyst design. The efficiency of developed catalysts will be tested for one-pot CRLF process using ethanol as both the solvent and the H2-donor. In-depth catalysts’ reusability and kinetic/mechanistic studies will be conducted to determine structure-activity relationships in the CRLF process.

Publications

List of publications.
year	authors and title	journal	last update
2019	Putla Sudarsanam, Elise Peeters, Ekaterina V. Makshina, Vasile I. Parvulescu, Bert F. Sels Advances in porous and nanoscale catalysts for viable biomass conversion published pages: 2366-2421, ISSN: 0306-0012, DOI: 10.1039/c8cs00452h	Chemical Society Reviews 48/8	2019-12-17
2018	Putla Sudarsanam, Ruyi Zhong, Sander Van den Bosch, Simona M. Coman, Vasile I. Parvulescu, Bert F. Sels Functionalised heterogeneous catalysts for sustainable biomass valorisation published pages: , ISSN: 0306-0012, DOI: 10.1039/C8CS00410B	Chemical Society Reviews	2019-04-18

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The information about "CATLIGCAR" are provided by the European Opendata Portal: CORDIS opendata.