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CATLIGCAR SIGNED

Designing Novel Efficient Catalytic Strategies for the Transformation of Lignocellulose into Lignin-derived Chemicals and Valorisable Carbohydrates

Total Cost €

EC-Contrib. €

Partnership

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Outcomes and
results

CATLIGCAR project word cloud

Explore the words cloud of the CATLIGCAR project. It provides you a very rough idea of what is the project "CATLIGCAR" about.

noble reactive mechanistic strength fuels crlf reusability chemicals nanoparticles alternative structure hemicellulose ni received fossil stability biomass class ethanol pd social simultaneously sites catalytic tremendous kinetic pot lignin economic efficient enriched acidic minimizing planes aid reductive techniques context varying proper interactions zinc crystal ing cellulose understand heterogeneous effect particles solid multifunctional polyhedra paper conversion relationships lignocellulose donor efficiency redox h2 nickel tuned retaining synergistic metals ru analytical rods dispersed superior ruthenium lewis catalysts shape abundant solvent family spheres tested renewable fraction oxide palladium selective catalyst acid fractionation hemi zno exposure nanoscale strategy integration size enhanced

Project "CATLIGCAR" data sheet

The following table provides information about the project.

Coordinator	KATHOLIEKE UNIVERSITEIT LEUVEN Organization address address: OUDE MARKT 13 city: LEUVEN postcode: 3000 website: www.kuleuven.be contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.
Coordinator Country	Belgium [BE]
Total cost	172˙800 €
EC max contribution	172˙800 € (100%)
Programme	1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
Code Call	H2020-MSCA-IF-2016
Funding Scheme	MSCA-IF-EF-ST
Starting year	2017
Duration (year-month-day)	from 2017-10-01 to 2019-09-30

Partnership

Take a look of project's partnership.

#	participants	country	role	EC contrib. [€]
1	KATHOLIEKE UNIVERSITEIT LEUVEN KATHOLIEKE UNIVERSITEIT LEUVEN Organization address address: OUDE MARKT 13 city: LEUVEN postcode: 3000 website: www.kuleuven.be contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	BE (LEUVEN)	coordinator	172˙800.00

Map

Project objective

The utilization of renewable lignocellulose biomass (composed of cellulose, hemicellulose and lignin) alternative to fossil fuels is crucial for long-term economic and social stability. In this context, the catalytic reductive lignocellulose fractionation (CRLF) process has received tremendous research interest as this strategy enables one-pot conversion of lignocellulose into useful lignin-derived chemicals, while retaining a solid (hemi)cellulose fraction that can be used for the production of fuels, chemicals or paper. The development of promising heterogeneous catalysts having abundant redox and acid properties, along with the application of a proper solvent is a great challenge for efficient CRLF process.

Nanoscale palladium-nickel (Pd-Ni) and ruthenium-nickel (Ru-Ni) particles dispersed on shape-controlled zinc oxide (ZnO) are considered to be a unique class of heterogeneous catalysts due to the size- and shape-tuned catalytic properties. The integration of Ni with Pd and Ru can provide new, enriched, selective redox sites and simultaneously minimizing the use of noble metals. As well, controlling the shape of ZnO particles allows a selective exposure of reactive crystal planes, resulting in enhanced Lewis acidic strength. Thus, the synergistic interactions of Pd-Ni and Ru-Ni nanoparticles with the shape-controlled ZnO will provide superior redox and acid properties that can show a promising effect in CRLF process. Therefore, this project aims to develop a family of novel multifunctional M-Ni/ZnO (M = Pd, Ru) catalysts by varying the ZnO shape (spheres, rods and polyhedra). A range of analytical techniques will be used to understand the catalysts’ properties and aid catalyst design. The efficiency of developed catalysts will be tested for one-pot CRLF process using ethanol as both the solvent and the H2-donor. In-depth catalysts’ reusability and kinetic/mechanistic studies will be conducted to determine structure-activity relationships in the CRLF process.

Publications

List of publications.
year	authors and title	journal	last update
2019	Putla Sudarsanam, Elise Peeters, Ekaterina V. Makshina, Vasile I. Parvulescu, Bert F. Sels Advances in porous and nanoscale catalysts for viable biomass conversion published pages: 2366-2421, ISSN: 0306-0012, DOI: 10.1039/c8cs00452h	Chemical Society Reviews 48/8	2019-12-17
2018	Putla Sudarsanam, Ruyi Zhong, Sander Van den Bosch, Simona M. Coman, Vasile I. Parvulescu, Bert F. Sels Functionalised heterogeneous catalysts for sustainable biomass valorisation published pages: , ISSN: 0306-0012, DOI: 10.1039/C8CS00410B	Chemical Society Reviews	2019-04-18

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