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CATLIGCAR SIGNED

Designing Novel Efficient Catalytic Strategies for the Transformation of Lignocellulose into Lignin-derived Chemicals and Valorisable Carbohydrates

Total Cost €

0

EC-Contrib. €

0

Partnership

0

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 CATLIGCAR project word cloud

Explore the words cloud of the CATLIGCAR project. It provides you a very rough idea of what is the project "CATLIGCAR" about.

enhanced    heterogeneous    ru    economic    reductive    fossil    effect    acidic    donor    analytical    varying    nanoscale    ing    shape    chemicals    rods    exposure    context    h2    mechanistic    size    stability    fuels    kinetic    reactive    proper    structure    pot    ruthenium    lignin    family    social    abundant    simultaneously    alternative    interactions    efficiency    redox    received    catalysts    multifunctional    zno    acid    paper    zinc    synergistic    ethanol    fractionation    nickel    catalytic    conversion    superior    sites    efficient    spheres    aid    planes    lignocellulose    oxide    tested    crlf    solvent    hemi    biomass    crystal    solid    pd    fraction    ni    enriched    particles    lewis    tuned    dispersed    nanoparticles    catalyst    renewable    relationships    integration    understand    class    hemicellulose    tremendous    palladium    strength    retaining    noble    strategy    reusability    techniques    polyhedra    metals    selective    cellulose    minimizing   

Project "CATLIGCAR" data sheet

The following table provides information about the project.

Coordinator
KATHOLIEKE UNIVERSITEIT LEUVEN 

Organization address
address: OUDE MARKT 13
city: LEUVEN
postcode: 3000
website: www.kuleuven.be

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Belgium [BE]
 Total cost 172˙800 €
 EC max contribution 172˙800 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2016
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2017
 Duration (year-month-day) from 2017-10-01   to  2019-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    KATHOLIEKE UNIVERSITEIT LEUVEN BE (LEUVEN) coordinator 172˙800.00

Map

 Project objective

The utilization of renewable lignocellulose biomass (composed of cellulose, hemicellulose and lignin) alternative to fossil fuels is crucial for long-term economic and social stability. In this context, the catalytic reductive lignocellulose fractionation (CRLF) process has received tremendous research interest as this strategy enables one-pot conversion of lignocellulose into useful lignin-derived chemicals, while retaining a solid (hemi)cellulose fraction that can be used for the production of fuels, chemicals or paper. The development of promising heterogeneous catalysts having abundant redox and acid properties, along with the application of a proper solvent is a great challenge for efficient CRLF process.

Nanoscale palladium-nickel (Pd-Ni) and ruthenium-nickel (Ru-Ni) particles dispersed on shape-controlled zinc oxide (ZnO) are considered to be a unique class of heterogeneous catalysts due to the size- and shape-tuned catalytic properties. The integration of Ni with Pd and Ru can provide new, enriched, selective redox sites and simultaneously minimizing the use of noble metals. As well, controlling the shape of ZnO particles allows a selective exposure of reactive crystal planes, resulting in enhanced Lewis acidic strength. Thus, the synergistic interactions of Pd-Ni and Ru-Ni nanoparticles with the shape-controlled ZnO will provide superior redox and acid properties that can show a promising effect in CRLF process. Therefore, this project aims to develop a family of novel multifunctional M-Ni/ZnO (M = Pd, Ru) catalysts by varying the ZnO shape (spheres, rods and polyhedra). A range of analytical techniques will be used to understand the catalysts’ properties and aid catalyst design. The efficiency of developed catalysts will be tested for one-pot CRLF process using ethanol as both the solvent and the H2-donor. In-depth catalysts’ reusability and kinetic/mechanistic studies will be conducted to determine structure-activity relationships in the CRLF process.

 Publications

year authors and title journal last update
List of publications.
2019 Putla Sudarsanam, Elise Peeters, Ekaterina V. Makshina, Vasile I. Parvulescu, Bert F. Sels
Advances in porous and nanoscale catalysts for viable biomass conversion
published pages: 2366-2421, ISSN: 0306-0012, DOI: 10.1039/c8cs00452h
Chemical Society Reviews 48/8 2019-12-17
2018 Putla Sudarsanam, Ruyi Zhong, Sander Van den Bosch, Simona M. Coman, Vasile I. Parvulescu, Bert F. Sels
Functionalised heterogeneous catalysts for sustainable biomass valorisation
published pages: , ISSN: 0306-0012, DOI: 10.1039/C8CS00410B
Chemical Society Reviews 2019-04-18

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