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PINNACLE SIGNED

Perovskite Nanocrystal-Nanoreactors for Enhanced Light Emission

Total Cost €

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EC-Contrib. €

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Partnership

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 PINNACLE project word cloud

Explore the words cloud of the PINNACLE project. It provides you a very rough idea of what is the project "PINNACLE" about.

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Project "PINNACLE" data sheet

The following table provides information about the project.

Coordinator
LUDWIG-MAXIMILIANS-UNIVERSITAET MUENCHEN 

Organization address
address: GESCHWISTER SCHOLL PLATZ 1
city: MUENCHEN
postcode: 80539
website: www.uni-muenchen.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Total cost 1˙498˙187 €
 EC max contribution 1˙498˙187 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2017-STG
 Funding Scheme ERC-STG
 Starting year 2018
 Duration (year-month-day) from 2018-03-01   to  2023-02-28

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    LUDWIG-MAXIMILIANS-UNIVERSITAET MUENCHEN DE (MUENCHEN) coordinator 1˙498˙187.00

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 Project objective

The unprecedented advancement of halide perovskite photovoltaics and light-emission applications has far outpaced the basic scientific research necessary to understand this fascinating yet perplexing material and to optimize material quality and device integration. Additionally, the intricate nature of the perovskite is susceptible to degradation from environmental stress, such as moisture and heat, currently deterring commercialization.

This research project will realize a novel synthesis for perovskite nanocrystals (NCs) by means of block copolymer nanoreactors. These will enable an unprecedented control over size and dimensionality of the NCs into the quantum-confinement regime. Using these NCs, we will determine the fundamental optical, electrical, and phononic properties of perovskite, mainly by means of temperature-controlled transient optical spectroscopy.

Elucidation of the degradation mechanisms through controlled subjecting to external stress, will lead to strategies for designing the nanoreactor to shield the NCs, mitigating these effects. Additionally, we will investigate the high mobility of (halide) ions in perovskites, and likewise design the polymeric nanoreactor to deter ion migration and enable NC implementation into existing optoelectronic applications and currently unattainable architectures, such as hetero-structures and exciton funnels.

We will create stable, high-quality NC-films, enabling the formation of multilayers for exciton funnelling by means of Förster resonance energy transfer (FRET). We will highlight the NC potential by integrating them into LEDs of various architectures, by demonstrating low-threshold ASE and realizing unprecedented perovskite-laser geometries, e.g. vertical cavity surface emitting lasers (VCSELs) and plasmonic nanopatch lasers. PINNACLE will greatly further the understanding of halide perovskites, benefitting the research community, and lead to novel optoelectronic devices and exciting new applications.

 Publications

year authors and title journal last update
List of publications.
2019 Robert L. Z. Hoye, May-Ling Lai, Miguel Anaya, Yu Tong, Krzysztof Gałkowski, Tiarnan Doherty, Weiwei Li, Tahmida N. Huq, Sebastian Mackowski, Lakshminarayana Polavarapu, Jochen Feldmann, Judith L. MacManus-Driscoll, Richard H. Friend, Alexander S. Urban, Samuel D. Stranks
Identifying and Reducing Interfacial Losses to Enhance Color-Pure Electroluminescence in Blue-Emitting Perovskite Nanoplatelet Light-Emitting Diodes
published pages: 1181-1188, ISSN: 2380-8195, DOI: 10.1021/acsenergylett.9b00571
ACS Energy Letters 4/5 2019-11-08
2019 Jasmina A. Sichert, Annick Hemmerling, Carlos Cardenas-Daw, Alexander S. Urban, Jochen Feldmann
Tuning the optical bandgap in layered hybrid perovskites through variation of alkyl chain length
published pages: 41116, ISSN: 2166-532X, DOI: 10.1063/1.5087296
APL Materials 7/4 2019-11-08
2018 Verena A. Hintermayr, Lakshminarayana Polavarapu, Alexander S. Urban, Jochen Feldmann
Accelerated Carrier Relaxation through Reduced Coulomb Screening in Two-Dimensional Halide Perovskite Nanoplatelets
published pages: 10151-10158, ISSN: 1936-0851, DOI: 10.1021/acsnano.8b05029
ACS Nano 12/10 2019-11-08
2019 Verena A. Hintermayr, Carola Lampe, Maximilian Löw, Janina Roemer, Willem Vanderlinden, Moritz Gramlich, Anton X. Böhm, Cornelia Sattler, Bert Nickel, Theobald Lohmüller, Alexander S. Urban
Polymer Nanoreactors Shield Perovskite Nanocrystals from Degradation
published pages: 4928-4933, ISSN: 1530-6984, DOI: 10.1021/acs.nanolett.9b00982
Nano Letters 19/8 2019-11-08
2018 Bernhard J. Bohn, Yu Tong, Moritz Gramlich, May Ling Lai, Markus Döblinger, Kun Wang, Robert L. Z. Hoye, Peter Müller-Buschbaum, Samuel D. Stranks, Alexander S. Urban, Lakshminarayana Polavarapu, Jochen Feldmann
Boosting Tunable Blue Luminescence of Halide Perovskite Nanoplatelets through Postsynthetic Surface Trap Repair
published pages: 5231-5238, ISSN: 1530-6984, DOI: 10.1021/acs.nanolett.8b02190
Nano Letters 18/8 2019-11-08

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