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EDAX SIGNED

Beating Complexity through Selectivity: Excited state Dynamics from Anti-Stokes and non-linear resonant inelastic X-ray scattering

Total Cost €

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EC-Contrib. €

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Partnership

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Project "EDAX" data sheet

The following table provides information about the project.

Coordinator
UNIVERSITAET POTSDAM 

Organization address
address: AM NEUEN PALAIS 10
city: POTSDAM
postcode: 14469
website: www.uni-potsdam.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Total cost 2˙496˙250 €
 EC max contribution 2˙496˙250 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2014-ADG
 Funding Scheme ERC-ADG
 Starting year 2016
 Duration (year-month-day) from 2016-01-01   to  2020-12-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    UNIVERSITAET POTSDAM DE (POTSDAM) coordinator 1˙804˙565.00
2    HELMHOLTZ-ZENTRUM BERLIN FUR MATERIALIEN UND ENERGIE GMBH DE (BERLIN) participant 434˙750.00
3    EUROPEAN X-RAY FREE-ELECTRON LASERFACILITY GMBH DE (SCHENEFELD) participant 256˙935.00

Map

 Project objective

The key to move from a mere description of static materials properties to the determination and control of functionality and chemistry lies in understanding dynamic pathways through multidimensional energy landscapes.

Through my efforts over the last decade my group accomplished breakthroughs towards the required excited states selectivity and to follow dynamic pathways with resonant inelastic soft x-ray scattering (RIXS) in three aspects: Non-linear RIXS for materials science to boost scattering efficiency. Time resolved and Anti-Stokes RIXS for back-ground free detection of excited states. Sub-natural line width RIXS to map out potential energy surfaces at selected atoms.

In the ERC research I link these unfolding fields and combine them with ab-initio treatment of excited states to create unprecedented back-ground free X-ray probes of excited states of matter and their dynamics. This will be femtosecond time resolved Anti-Stokes RIXS for excited state selectivity with transform limited pulses and doubly resonant soft X-ray 4 wave mixing to determine multi-center dynamics on atomic scales.

The ERC grant will answer long standing questions on the governing principles of functionality, regarding chemical pathways and energy landscapes in molecules as well as phase transitions, driven phases and emergence in functional materials.

These novel approaches become only now feasible through the unprecedented brilliance of Free-Electron Lasers and the efforts of my group over the last decade. The ERC grant will establish proof-of-principle at brilliant soft X-ray Free-Electron Lasers that will be followed by world leading, ideal conditions implemented at the European XFEL.

 Publications

year authors and title journal last update
List of publications.
2016 Kristjan Kunnus, Ida Josefsson, Ivan Rajkovic, Simon Schreck, Wilson Quevedo, Martin Beye, Sebastian Grübel, Mirko Scholz, Dennis Nordlund, Wenkai Zhang, Robert W Hartsock, Kelly J Gaffney, William F Schlotter, Joshua J Turner, Brian Kennedy, Franz Hennies, Simone Techert, Philippe Wernet, Michael Odelius, Alexander Föhlisch
Anti-Stokes resonant x-ray Raman scattering for atom specific and excited state selective dynamics
published pages: 103011, ISSN: 1367-2630, DOI: 10.1088/1367-2630/18/10/103011
New Journal of Physics 18/10 2019-09-02
2017 Danilo Kühn, Florian Sorgenfrei, Erika Giangrisostomi, Raphael Jay, Abdurrahman Musazay, Ruslan Ovsyannikov, Christian Stråhlman, Svante Svensson, Nils Mårtensson, Alexander Föhlisch
Capabilities of Angle Resolved Time of Flight electron spectroscopy with the 60° wide angle acceptance lens
published pages: , ISSN: 0368-2048, DOI: 10.1016/j.elspec.2017.06.008
Journal of Electron Spectroscopy and Related Phenomena 2019-09-02
2017 Sebastian Eckert, Jesper Norell, Piter S. Miedema, Martin Beye, Mattis Fondell, Wilson Quevedo, Brian Kennedy, Markus Hantschmann, Annette Pietzsch, Benjamin E. Van Kuiken, Matthew Ross, Michael P. Minitti, Stefan P. Moeller, William F. Schlotter, Munira Khalil, Michael Odelius, Alexander Föhlisch
Ultrafast Independent N−H and N−C Bond Deformation Investigated with Resonant Inelastic X-Ray Scattering
published pages: 6088-6092, ISSN: 1433-7851, DOI: 10.1002/anie.201700239
Angewandte Chemie International Edition 56/22 2019-09-02
2016 S. Eckert, P.S. Miedema, W. Quevedo, B. O’Cinneide, M. Fondell, M. Beye, A. Pietzsch, M. Ross, M. Khalil, A. Föhlisch
Molecular structures and protonation state of 2-Mercaptopyridine in aqueous solution
published pages: 103-106, ISSN: 0009-2614, DOI: 10.1016/j.cplett.2016.01.050
Chemical Physics Letters 647 2019-09-02
2017 Vinícius Vaz da Cruz, Emelie Ertan, Rafael C. Couto, Sebastian Eckert, Mattis Fondell, Marcus Dantz, Brian Kennedy, Thorsten Schmitt, Annette Pietzsch, Freddy F. Guimarães, Hans Ågren, Faris Gel\'mukhanov, Michael Odelius, Alexander Föhlisch, Victor Kimberg
A study of the water molecule using frequency control over nuclear dynamics in resonant X-ray scattering
published pages: 19573-19589, ISSN: 1463-9076, DOI: 10.1039/C7CP01215B
Phys. Chem. Chem. Phys. 19/30 2019-09-02
2016 Daniel Schick, Sebastian Eckert, Niko Pontius, Rolf Mitzner, Alexander Föhlisch, Karsten Holldack, Florian Sorgenfrei
Versatile soft X-ray-optical cross-correlator for ultrafast applications
published pages: 54304, ISSN: 2329-7778, DOI: 10.1063/1.4964296
Structural Dynamics 3/5 2019-09-02
2017 Sebastian Eckert, Jesper Norell, Piter S. Miedema, Martin Beye, Mattis Fondell, Wilson Quevedo, Brian Kennedy, Markus Hantschmann, Annette Pietzsch, Benjamin E. Van Kuiken, Matthew Ross, Michael P. Minitti, Stefan P. Moeller, William F. Schlotter, Munira Khalil, Michael Odelius, Alexander Föhlisch
Untersuchung unabhängiger N-H- und N-C-Bindungsverformungen auf ultrakurzen Zeitskalen mit resonanter inelastischer Röntgenstreuung
published pages: 6184-6188, ISSN: 0044-8249, DOI: 10.1002/ange.201700239
Angewandte Chemie 129/22 2019-09-02
2018 Jesper Norell, Raphael M. Jay, Markus Hantschmann, Sebastian Eckert, Meiyuan Guo, Kelly J. Gaffney, Philippe Wernet, Marcus Lundberg, Alexander Föhlisch, Michael Odelius
Fingerprints of electronic, spin and structural dynamics from resonant inelastic soft X-ray scattering in transient photo-chemical species
published pages: 7243-7253, ISSN: 1463-9076, DOI: 10.1039/c7cp08326b
Physical Chemistry Chemical Physics 20/10 2019-09-02
2017 Mattis Fondell, Sebastian Eckert, Raphael M. Jay, Christian Weniger, Wilson Quevedo, Johannes Niskanen, Brian Kennedy, Florian Sorgenfrei, Daniel Schick, Erika Giangrisostomi, Ruslan Ovsyannikov, Katrin Adamczyk, Nils Huse, Philippe Wernet, Rolf Mitzner, Alexander Föhlisch
Time-resolved soft X-ray absorption spectroscopy in transmission mode on liquids at MHz repetition rates
published pages: 54902, ISSN: 2329-7778, DOI: 10.1063/1.4993755
Structural Dynamics 4/5 2019-09-02
2017 Rafael C. Couto, Vinícius V. Cruz, Emelie Ertan, Sebastian Eckert, Mattis Fondell, Marcus Dantz, Brian Kennedy, Thorsten Schmitt, Annette Pietzsch, Freddy F. Guimarães, Hans Ågren, Faris Gel’mukhanov, Michael Odelius, Victor Kimberg, Alexander Föhlisch
Selective gating to vibrational modes through resonant X-ray scattering
published pages: 14165, ISSN: 2041-1723, DOI: 10.1038/ncomms14165
Nature Communications 8 2019-09-02
2017 Annette Pietzsch, Alexander Föhlisch
Local Maps of Potential Energy Surfaces and Chemical Pathways
published pages: 8-13, ISSN: 0894-0886, DOI: 10.1080/08940886.2017.1289799
Synchrotron Radiation News 30/2 2019-09-02

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