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2D-CHEM SIGNED

Two-Dimensional Chemistry towards New Graphene Derivatives

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EC-Contrib. €

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Partnership

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Project "2D-CHEM" data sheet

The following table provides information about the project.

Coordinator
UNIVERZITA PALACKEHO V OLOMOUCI 

Organization address
address: KRIZKOVSKEHO 8
city: OLOMOUC
postcode: 771 47
website: www.upol.cz

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Czech Republic [CZ]
 Project website http://www.2dchem.org
 Total cost 1˙831˙102 €
 EC max contribution 1˙831˙102 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2015-CoG
 Funding Scheme ERC-COG
 Starting year 2016
 Duration (year-month-day) from 2016-06-01   to  2021-05-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    UNIVERZITA PALACKEHO V OLOMOUCI CZ (OLOMOUC) coordinator 1˙831˙102.00

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 Project objective

The suite of graphene’s unique properties and applications can be enormously enhanced by its functionalization. As non-covalently functionalized graphenes do not target all graphene’s properties and may suffer from limited stability, covalent functionalization represents a promising way for controlling graphene’s properties. To date, only a few well-defined graphene derivatives have been introduced. Among them, fluorographene (FG) stands out as a prominent member because of its easy synthesis and high stability. Being a perfluorinated hydrocarbon, FG was believed to be as unreactive as the two-dimensional counterpart perfluoropolyethylene (Teflon®). However, our recent experiments showed that FG is not chemically inert and can be used as a viable precursor for synthesizing graphene derivatives. This surprising behavior indicates that common textbook grade knowledge cannot blindly be applied to the chemistry of 2D materials. Further, there might be specific rules behind the chemistry of 2D materials, forming a new chemical discipline we tentatively call 2D chemistry. The main aim of the project is to explore, identify and apply the rules of 2D chemistry starting from FG. Using the knowledge gained of 2D chemistry, we will attempt to control the chemistry of various 2D materials aimed at preparing stable graphene derivatives with designed properties, e.g., 1-3 eV band gap, fluorescent properties, sustainable magnetic ordering and dispersability in polar media. The new graphene derivatives will be applied in sensing, imaging, magnetic delivery and catalysis and new emerging applications arising from the synergistic phenomena are expected. We envisage that new applications will be opened up that benefit from the 2D scaffold and tailored properties of the synthesized derivatives. The derivatives will be used for the synthesis of 3D hybrid materials by covalent linking of the 2D sheets joined with other organic and inorganic molecules, nanomaterials or biomacromolecules.

 Publications

year authors and title journal last update
List of publications.
2019 Aristides Bakandritsos, Ravishankar G. Kadam, Pawan Kumar, Giorgio Zoppellaro, Miroslav Medved\', Jiří Tuček, Tiziano Montini, Ondřej Tomanec, Pavlína Andrýsková, Bohuslav Drahoš, Rajender S. Varma, Michal Otyepka, Manoj B. Gawande, Paolo Fornasiero, Radek Zbořil
Mixed‐Valence Single‐Atom Catalyst Derived from Functionalized Graphene
published pages: 1900323, ISSN: 0935-9648, DOI: 10.1002/adma.201900323
Advanced Materials 31/17 2019-08-29
2019 Aristides Bakandritsos, Petr Jakubec, Martin Pykal, Michal Otyepka
Covalently functionalized graphene as a supercapacitor electrode material
published pages: 25-33, ISSN: 2452-2627, DOI: 10.1016/j.flatc.2018.12.004
FlatChem 13 2019-08-29
2019 Hugo Barès, Aristides Bakandritsos, Miroslav Medveď, Juri Ugolotti, Petr Jakubec, Ondřej Tomanec, Sergii Kalytchuk, Radek Zbořil, Michal Otyepka
Bimodal role of fluorine atoms in fluorographene chemistry opens a simple way toward double functionalization of graphene
published pages: 251-258, ISSN: 0008-6223, DOI: 10.1016/j.carbon.2019.01.059
Carbon 145 2019-08-29
2019 Eleni C. Vermisoglou, Petr Jakubec, Aristides Bakandritsos, Martin Pykal, Smita Talande, Vojtěch Kupka, Radek Zbořil, Michal Otyepka
Chemical Tuning of Specific Capacitance in Functionalized Fluorographene
published pages: 4698-4709, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.9b00655
Chemistry of Materials 31/13 2019-08-29
2018 Bruno de la Torre, Martin Švec, Prokop Hapala, Jesus Redondo, Ondřej Krejčí, Rabindranath Lo, Debashree Manna, Amrit Sarmah, Dana Nachtigallová, Jiří Tuček, Piotr Błoński, Michal Otyepka, Radek Zbořil, Pavel Hobza, Pavel Jelínek
Non-covalent control of spin-state in metal-organic complex by positioning on N-doped graphene
published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-018-05163-y
Nature Communications 9/1 2019-02-28
2018 Petr Lazar, Eva Otyepková, Martin Pykal, Klára Čépe, Michal Otyepka
Role of the puckered anisotropic surface in the surface and adsorption properties of black phosphorus
published pages: 8979-8988, ISSN: 2040-3364, DOI: 10.1039/c8nr00329g
Nanoscale 10/19 2019-02-28
2018 Miroslav Medveď, Giorgio Zoppellaro, Juri Ugolotti, Dagmar Matochová, Petr Lazar, Tomáš Pospíšil, Aristides Bakandritsos, Jiří Tuček, Radek Zbořil, Michal Otyepka
Reactivity of fluorographene is triggered by point defects: beyond the perfect 2D world
published pages: 4696-4707, ISSN: 2040-3364, DOI: 10.1039/c7nr09426d
Nanoscale 10/10 2019-02-28
2018 Dagmar Matochová, Miroslav Medved’, Aristides Bakandritsos, Tomáš Steklý, Radek Zbořil, Michal Otyepka
2D Chemistry: Chemical Control of Graphene Derivatization
published pages: 3580-3585, ISSN: 1948-7185, DOI: 10.1021/acs.jpclett.8b01596
The Journal of Physical Chemistry Letters 9/13 2019-02-28
2018 Q Li, J P Froning, M Pykal, S Zhang, Z Wang, M Vondrák, P Banáš, K Čépe, P Jurečka, J Šponer, R Zbořil, M Dong, M Otyepka
RNA nanopatterning on graphene
published pages: 31006, ISSN: 2053-1583, DOI: 10.1088/2053-1583/aabdf7
2D Materials 5/3 2019-02-28
2018 Aristides Bakandritsos, Demetrios D. Chronopoulos, Petr Jakubec, Martin Pykal, Klára Čépe, Theodore Steriotis, Sergii Kalytchuk, Martin Petr, Radek Zbořil, Michal Otyepka
High-Performance Supercapacitors Based on a Zwitterionic Network of Covalently Functionalized Graphene with Iron Tetraaminophthalocyanine
published pages: 1801111, ISSN: 1616-301X, DOI: 10.1002/adfm.201801111
Advanced Functional Materials 28/29 2019-02-28
2018 Markéta Paloncýová, Michal Langer, Michal Otyepka
Structural Dynamics of Carbon Dots in Water and N , N -Dimethylformamide Probed by All-Atom Molecular Dynamics Simulations
published pages: 2076-2083, ISSN: 1549-9618, DOI: 10.1021/acs.jctc.7b01149
Journal of Chemical Theory and Computation 14/4 2019-02-28
2019 Dario Mosconi, Matías Blanco, Teresa Gatti, Laura Calvillo, Michal Otyepka, Aristides Bakandritsos, Enzo Menna, Stefano Agnoli, Gaetano Granozzi
Arene C H insertion catalyzed by ferrocene covalently heterogenized on graphene acid
published pages: 318-328, ISSN: 0008-6223, DOI: 10.1016/j.carbon.2018.11.010
Carbon 143 2019-02-28
2019 Demetrios D. Chronopoulos, Miroslav Medved’, Piotr Błoński, Zdeněk Nováček, Petr Jakubec, Ondřej Tomanec, Aristides Bakandritsos, Veronika Novotná, Radek Zbořil, Michal Otyepka
Alkynylation of graphene via the Sonogashira C–C cross-coupling reaction on fluorographene
published pages: 1088-1091, ISSN: 1359-7345, DOI: 10.1039/c8cc08492k
Chemical Communications 55/8 2019-02-28

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