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EnanSET SIGNED

Homogeneous and heterogeneous enantioselective Single Electron Transfer (SET) catalysis in cross-coupling reactions

Total Cost €

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EC-Contrib. €

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Partnership

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Project "EnanSET" data sheet

The following table provides information about the project.

Coordinator
UNIVERSIDAD DE GRANADA 

Organization address
address: CUESTA DEL HOSPICIO SN
city: GRANADA
postcode: 18071
website: www.ugr.es

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Spain [ES]
 Total cost 239˙191 €
 EC max contribution 239˙191 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2016
 Funding Scheme MSCA-IF-GF
 Starting year 2018
 Duration (year-month-day) from 2018-02-01   to  2021-05-01

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    UNIVERSIDAD DE GRANADA ES (GRANADA) coordinator 239˙191.00
2    THE SCRIPPS RESEARCH INSTITUTE US (LA JOLLA CA) partner 0.00

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 Project objective

Chirality of organic molecules plays a paramount role in our society as a consequence of the direct relation between the absolute molecular configuration and many properties and applications of molecular compounds and materials. The demand of enantiomerically pure compounds has increased considerably driven by the request of the pharmaceutical industry, as well as applications such as flavours, fragrances, and materials. In this context, the development of new methodologies to obtain enantiomerically pure compounds has become a challenge for the scientific community. This project entitled “Homogeneous and heterogeneous enantioselective Single Electron Transfer (SET) catalysis in cross-coupling reactions (EnanSET)” aims at developing novel enantioselective SET cross-coupling reactions of redox active esters (RAEs) by Ni-complex due to this kind of compounds do not need previous activation. Moreover, in order to develop more environmentally friendly processes, the methodology will be extended to non-toxic SET complex as titanium complexes, with the goal of developing the first Ti-catalysis of RAEs. Additionally, inspired by demand of the industrial processes, the need to develop clean and green chemical processes in order to avoid environmental concerns and the advantages that heterogeneous catalysis provides, we will develop the first SET heterogeneous catalysis with MOFs through the postsynthetic incorporation of chiral Ni or Ti-residues on the pore structure.

 Publications

year authors and title journal last update
List of publications.
2019 Javier Castells-Gil, Natalia M. Padial, Neyvis Almora-Barrios, Ivan da Silva, Diego Mateo, Josep Albero, Hermenegildo García, Carlos Martí-Gastaldo
De novo synthesis of mesoporous photoactive titanium( iv )–organic frameworks with MIL-100 topology
published pages: 4313-4321, ISSN: 2041-6520, DOI: 10.1039/c8sc05218b
Chemical Science 10/15 2020-04-03
2019 Natalia M. Padial, Javier Castells-Gil, Neyvis Almora-Barrios, María Romero-Angel, Iván da Silva, Mariam Barawi, Alba García-Sánchez, Víctor A. de la Peña O’Shea, Carlos Martí-Gastaldo
Hydroxamate Titanium–Organic Frameworks and the Effect of Siderophore-Type Linkers over Their Photocatalytic Activity
published pages: 13124-13133, ISSN: 0002-7863, DOI: 10.1021/jacs.9b04915
Journal of the American Chemical Society 141/33 2020-04-03
2019 Alejandro Nuñez‐Lopez, Marta Galbiati, Natalia M. Padial, Carolina R. Ganivet, Sergio Tatay, Emilio Pardo, Donatella Armentano, Carlos Martí‐Gastaldo
Direct Visualization of Pyrrole Reactivity upon Confinement within a Cyclodextrin Metal–Organic Framework
published pages: 9179-9183, ISSN: 1433-7851, DOI: 10.1002/anie.201904890
Angewandte Chemie International Edition 58/27 2020-04-03
2019 Shengyang Ni, Natalia M. Padial, Cian Kingston, Julien C. Vantourout, Daniel C. Schmitt, Jacob T. Edwards, Monika M. Kruszyk, Rohan R. Merchant, Pavel K. Mykhailiuk, Brittany B. Sanchez, Shouliang Yang, Matthew A. Perry, Gary M. Gallego, James J. Mousseau, Michael R. Collins, Robert J. Cherney, Pavlo S. Lebed, Jason S. Chen, Tian Qin, Phil S. Baran
A Radical Approach to Anionic Chemistry: Synthesis of Ketones, Alcohols, and Amines
published pages: 6726-6739, ISSN: 0002-7863, DOI: 10.1021/jacs.9b02238
Journal of the American Chemical Society 141/16 2020-04-03
2020 Dongmin Xu, Nazaret Rivas-Bascón, Natalia M. Padial, Kyle W. Knouse, Bin Zheng, Julien C. Vantourout, Michael A. Schmidt, Martin D. Eastgate, Phil S. Baran
Enantiodivergent Formation of C–P Bonds: Synthesis of P-Chiral Phosphines and Methylphosphonate Oligonucleotides
published pages: 5785-5792, ISSN: 0002-7863, DOI: 10.1021/jacs.9b13898
Journal of the American Chemical Society 142/12 2020-04-03

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