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ATTOLIQ SIGNED

Attosecond X-ray spectroscopy of liquids

Total Cost €

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EC-Contrib. €

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Partnership

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 ATTOLIQ project word cloud

Explore the words cloud of the ATTOLIQ project. It provides you a very rough idea of what is the project "ATTOLIQ" about.

tech    molecules    photovoltaic    source    liquid    flat    complexes    sensitivity    isolated    ultrathin    turn    dyne    applicable    transformations    outer    auger    achievements    resolution    underlying    innovative    dynamics    core    intermolecular    niques    first    scattering    285    transient    ray    coulombic    pho    inelastic    ev    sources    place    538    water    environments    transition    pulses    metal    reactions    hetero    raman    absorption    valence    complement    aqueous    species    calls    temporal    chemical    resonant    concentrate    decay    transfer    resolved    attosecond    purely    demonstrating    bandwidth    electron    liquids    femtosecond    scales    biological    complete    experimental    toelectron    time    realize    microjet    inner    goals    electronic    combine    emission    spectroscopy    relevance    measuring    toexcited    migration    detected    solvated    nanoparticles    variant    charge    microjets    ionization    naturally    window    energy   

Project "ATTOLIQ" data sheet

The following table provides information about the project.

Coordinator
EIDGENOESSISCHE TECHNISCHE HOCHSCHULE ZUERICH 

Organization address
address: Raemistrasse 101
city: ZUERICH
postcode: 8092
website: https://www.ethz.ch/de.html

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Switzerland [CH]
 Project website http://www.atto.ethz.ch
 Total cost 2˙750˙000 €
 EC max contribution 2˙750˙000 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2017-COG
 Funding Scheme ERC-COG
 Starting year 2018
 Duration (year-month-day) from 2018-04-01   to  2023-03-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    EIDGENOESSISCHE TECHNISCHE HOCHSCHULE ZUERICH CH (ZUERICH) coordinator 2˙750˙000.00

Map

 Project objective

Charge and energy transfer are the key steps underlying most chemical reactions and biological transformations. The purely electronic dynamics that control such processes take place on attosecond time scales. A complete understanding of these dynamics on the electronic level therefore calls for new experimental methods with attosecond resolution that are applicable to aqueous environments. We propose to combine the element sensitivity of X-ray spectroscopy with attosecond temporal resolution and ultrathin liquid microjets to study electronic dynamics of relevance to chemical, biological and photovoltaic processes. We will build on our recent achievements in demonstrating femtosecond time-resolved measurements in the water, attosecond pho-toelectron spectroscopy on a liquid microjet and measuring and controlling attosecond charge migration in isolated molecules. We will first concentrate on liquid water to study its electronic dynamics following outer-valence ionization, the formation pathway of the solvated electron and the time scales and intermolecular Coulombic decay following inner-valence or core-level ionization. Second, we will turn to solvated species and measure electronic dynamics and charge migration in solvated molecules, transition-metal complexes and pho-toexcited nanoparticles. These goals will be achieved by developing several innovative experimental tech-niques. We will develop a source of isolated attosecond pulses covering the water window (285-538 eV) and combine it with a flat liquid microjet to realize attosecond transient absorption in liquids. We will complement these measurements with attosecond X-ray emission spectroscopy, Auger spectroscopy and a novel hetero-dyne-detected variant of resonant inelastic Raman scattering, exploiting the large bandwidth that is naturally available from attosecond X-ray sources.

 Publications

year authors and title journal last update
List of publications.
2018 Tran Trung Luu, Zhong Yin, Arohi Jain, Thomas Gaumnitz, Yoann Pertot, Jun Ma, Hans Jakob Wörner
Extreme–ultraviolet high–harmonic generation in liquids
published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-018-06040-4
Nature Communications 9/1 2019-11-07

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