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DisorMetox SIGNED

Disorder and Order in the Conversion Mechanism of Metal Oxides in Lithium-ion Batteries

Total Cost €

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EC-Contrib. €

0

Partnership

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 DisorMetox project word cloud

Explore the words cloud of the DisorMetox project. It provides you a very rough idea of what is the project "DisorMetox" about.

drawn    reactions    li    rmc    prof    monte    identification    systematic    phases    view    electrode    ion    multiple    pulverisation    defected    heterogeneity    manganese    metal    model    nanoscopic    chemistry    crystallographic    stable    total    considerable    functional    nanostructuring    hindering    goodwin    libs    amorphous    fundamentals    reverse    formula    compounds    reaction    ray    conventional    commercial    anode    constituting    oxford    variations    undergo    found    efficiency    structures    library    characterization    obstacles    binary    expert    critical    andrew    good    investigation    oxides    hysteresis    emphasis    conversion    difficult    analytical    batteries    carlo    manifest    hosted    proven    data    mechanistic    mxoy    coexistence    desirable    thermodynamics    iron    coulombic    materials    structural    quantitative    compositional    transition    characterisation    series    neutron    disordered    material    overcome    chemical    electron    apparent    class    performance    last    earlier    devoted    unusual    efforts    disorder    hidden    accurate    capacities    scattering    decade   

Project "DisorMetox" data sheet

The following table provides information about the project.

Coordinator
THE CHANCELLOR, MASTERS AND SCHOLARS OF THE UNIVERSITY OF OXFORD 

Organization address
address: WELLINGTON SQUARE UNIVERSITY OFFICES
city: OXFORD
postcode: OX1 2JD
website: www.ox.ac.uk

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country United Kingdom [UK]
 Total cost 195˙454 €
 EC max contribution 195˙454 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2017
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2018
 Duration (year-month-day) from 2018-08-01   to  2020-07-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    THE CHANCELLOR, MASTERS AND SCHOLARS OF THE UNIVERSITY OF OXFORD UK (OXFORD) coordinator 195˙454.00

Map

 Project objective

Binary transition metal oxides (MxOy) have been studied as anode electrode materials for Li-ion batteries (LIBs) for many years. Defined as a class of conversion material, these MxOy undergo multi-electron reactions (per formula unit) leading to highly desirable capacities and have drawn considerable attention. Over the last decade, most of the earlier efforts were devoted to material nanostructuring, which has proven effective to enhance the overall material performance. However, critical issues such as the large hysteresis and low Coulombic efficiency remain key obstacles hindering the commercial application of MxOy. To overcome these obstacles requires a good understanding of the reaction fundamentals, which has yet been achieved due to the challenges involved in the characterisation of these MxOy. Previous mechanistic studies found that these MxOy undergo a chemical pulverisation leading to coexistence of multiple nanoscopic/defected or even amorphous/disordered phases. In view of these complex structural features and high heterogeneity of the system, it is difficult for a quantitative and accurate phase identification and structural characterization using conventional analytical approaches. This proposal will, therefore, develop a novel approach based on reverse Monte Carlo (RMC) method using the X-ray/neutron total scattering data, to study the reaction thermodynamics of these MxOy in the LIBs with emphasis on the investigation of the (apparent) structural disorder and (hidden) order present in the system. The proposed project will target a series of iron and manganese oxides as model compounds because they are the most studied conversion MxOy and their stable phases manifest considerable compositional/crystallographic variations constituting a large library of materials for a systematic study. The project will be hosted by Prof. Andrew Goodwin (Oxford Chemistry), an expert in studying complex structures of functional materials and their unusual properties.

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