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DisorMetox SIGNED

Disorder and Order in the Conversion Mechanism of Metal Oxides in Lithium-ion Batteries

Total Cost €

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EC-Contrib. €

0

Partnership

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 DisorMetox project word cloud

Explore the words cloud of the DisorMetox project. It provides you a very rough idea of what is the project "DisorMetox" about.

rmc    neutron    prof    chemical    capacities    electrode    drawn    nanoscopic    nanostructuring    crystallographic    monte    identification    conversion    disordered    compositional    reaction    decade    data    batteries    reverse    analytical    investigation    scattering    carlo    compounds    oxides    systematic    characterisation    model    amorphous    efforts    found    hindering    accurate    transition    thermodynamics    material    heterogeneity    iron    emphasis    proven    oxford    good    unusual    earlier    metal    variations    constituting    considerable    total    class    hosted    overcome    formula    coexistence    characterization    libs    li    chemistry    binary    series    phases    hysteresis    electron    critical    desirable    manganese    goodwin    structures    efficiency    obstacles    multiple    last    materials    devoted    anode    library    pulverisation    manifest    ion    defected    disorder    functional    mechanistic    coulombic    reactions    fundamentals    andrew    quantitative    structural    undergo    conventional    performance    difficult    hidden    apparent    stable    mxoy    expert    commercial    view    ray   

Project "DisorMetox" data sheet

The following table provides information about the project.

Coordinator
THE CHANCELLOR, MASTERS AND SCHOLARS OF THE UNIVERSITY OF OXFORD 

Organization address
address: WELLINGTON SQUARE UNIVERSITY OFFICES
city: OXFORD
postcode: OX1 2JD
website: www.ox.ac.uk

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country United Kingdom [UK]
 Total cost 195˙454 €
 EC max contribution 195˙454 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2017
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2018
 Duration (year-month-day) from 2018-08-01   to  2020-07-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    THE CHANCELLOR, MASTERS AND SCHOLARS OF THE UNIVERSITY OF OXFORD UK (OXFORD) coordinator 195˙454.00

Map

 Project objective

Binary transition metal oxides (MxOy) have been studied as anode electrode materials for Li-ion batteries (LIBs) for many years. Defined as a class of conversion material, these MxOy undergo multi-electron reactions (per formula unit) leading to highly desirable capacities and have drawn considerable attention. Over the last decade, most of the earlier efforts were devoted to material nanostructuring, which has proven effective to enhance the overall material performance. However, critical issues such as the large hysteresis and low Coulombic efficiency remain key obstacles hindering the commercial application of MxOy. To overcome these obstacles requires a good understanding of the reaction fundamentals, which has yet been achieved due to the challenges involved in the characterisation of these MxOy. Previous mechanistic studies found that these MxOy undergo a chemical pulverisation leading to coexistence of multiple nanoscopic/defected or even amorphous/disordered phases. In view of these complex structural features and high heterogeneity of the system, it is difficult for a quantitative and accurate phase identification and structural characterization using conventional analytical approaches. This proposal will, therefore, develop a novel approach based on reverse Monte Carlo (RMC) method using the X-ray/neutron total scattering data, to study the reaction thermodynamics of these MxOy in the LIBs with emphasis on the investigation of the (apparent) structural disorder and (hidden) order present in the system. The proposed project will target a series of iron and manganese oxides as model compounds because they are the most studied conversion MxOy and their stable phases manifest considerable compositional/crystallographic variations constituting a large library of materials for a systematic study. The project will be hosted by Prof. Andrew Goodwin (Oxford Chemistry), an expert in studying complex structures of functional materials and their unusual properties.

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