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NMR4CO2 SIGNED

Unveiling CO2 chemisorption mechanisms in solid adsorbents via surface-enhanced ex(in)-situ NMR

Total Cost €

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EC-Contrib. €

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Partnership

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 NMR4CO2 project word cloud

Explore the words cloud of the NMR4CO2 project. It provides you a very rough idea of what is the project "NMR4CO2" about.

simulated    adsorbed    cooperative    chemists    situ    elusive    deactivation    global    capacity    chemisorption    flow    carbon    nmr4co2    enhanced    reaching    dioxide    mainly    point    multiple    modification    desorption    tackle    chemisorb    determines    amine    co2    pressure    first    surface    time    regenerability    32    porous    sorbent    outcomes    speciation    gap    2017    emissions    tolerant    thermodynamically    species    effect    synthetic    inter    molecular    replacing    nuclear    polarization    historic    kinetics    encompasses    industrial    dynamic    removal    improvement    modified    combustion    amps    source    gases    environmental    adsorbents    monitoring    gigatonnes    gas    lower    stability    labeled    hindering    chemistry    competing    interfaces    emission    silicas    solid    nature    fossil    fuels    solution    surfaces    expertise    ssnmr    selectivity    spectroscopists    vi    acidic    3reaching    engaging    textural    isotopically    kinetically    technologies    liquid    moisture    cycles    identification    selectively    engineers    acid    fill    sorbents    mixtures    scrubbing    adsorption    decades    regeneration    spacing    combines    nmr    continue    ex    comprising    concentration    formed   

Project "NMR4CO2" data sheet

The following table provides information about the project.

Coordinator
UNIVERSIDADE DE AVEIRO 

Organization address
address: CAMPUS UNIVERSITÁRIO DE SANTIAGO
city: AVEIRO
postcode: 3810-193
website: www.ua.pt

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Portugal [PT]
 Total cost 1˙999˙793 €
 EC max contribution 1˙999˙793 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2019-COG
 Funding Scheme ERC-COG
 Starting year 2020
 Duration (year-month-day) from 2020-06-01   to  2025-05-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    UNIVERSIDADE DE AVEIRO PT (AVEIRO) coordinator 1˙999˙793.00

Map

 Project objective

Reaching a historic high of 3Reaching a historic high of 32.5 gigatonnes in 2017, global carbon dioxide emissions from fossil fuels combustion continue to increase. CO2 removal technologies are part of the solution to tackle this crucial environmental challenge. Because of their lower regeneration cost, amine-modified porous silicas (AMPS) are the most promising CO2-adsorbents for replacing the decades-old liquid amine scrubbing technology. AMPS are “moisture-tolerant” and selectively chemisorb CO2 from low-concentration mixtures, important features for operating under large-point CO2 emission source conditions. The nature of CO2 species formed on AMPS surfaces determines the gas adsorption capacity/kinetics, selectivity, stability, and regenerability. However, a molecular-scale understanding of the CO2-AMPS adsorption process remains elusive, hindering our ability to design improved sorbents. NMR4CO2 aims to fill in this gap, engaging for the first time state-of-the-art surface-enhanced ex- and in-situ solid-state NMR (SSNMR) to study the chemistry of acidic gases (mainly CO2) adsorbed on AMPS, and the gas-solid interfaces, using simulated industrial gas mixtures. The project combines the expertise of spectroscopists, chemists, and engineers to tackle these challenges. NMR4CO2 encompasses the design of novel SSNMR methods to study the kinetically- and thermodynamically-driven CO2-AMPS adsorption process, comprising in-situ flow NMR, dynamic nuclear polarization NMR, and isotopically-labeled gas mixtures. Important outcomes include: i) identification of competing CO2 chemisorption pathways; ii) effect on CO2 speciation of textural properties, amine type, inter-amine spacing, and amine-support cooperative effects; iii) real-time monitoring of acid gas speciation in multiple adsorption/desorption cycles; iv) identification of sorbent deactivation species; v) effect of pressure on CO2 speciation and vi) improvement of AMPS sorbent properties by synthetic modification.

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