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MesoSi-CO2 SIGNED

Design of low-cost and carbon-resistant Ni-based mesoporous silicas for chemical CO2 utilization through tri-reforming of methane

Total Cost €

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EC-Contrib. €

0

Partnership

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 MesoSi-CO2 project word cloud

Explore the words cloud of the MesoSi-CO2 project. It provides you a very rough idea of what is the project "MesoSi-CO2" about.

advantage    ratios    examine    assistance    xas    xrd    kinetic    reveal    conversion    flue    theory    technologies    solution    chemical    dsc    reforming    waste    operando    dft    led    nature    secondment    resistant    tga    xps    reactions    methane    co2    natural    sintering    functional    emissions    atmosphere    materials    deactivation    gas    converting    transient    renewable    bio    microwaves    lack    greenhouse    sorbonne    silica    gases    temperature    physico    reduce    selectivity    tpr    fired    trm    performed    zero    universit    dioxide    tri    sources    plant    mechanisms    carbon    stay    mesoporous    concentrations    ms    hinders    effect    increasing    eliminate    desired    tremendous    synthesis    ni    industrial    perform    superior    serious    france    sites    plants    catalysts    sorption    catalytic    active    global    density    eacute    ssitka    experiments    co    h2    steady    evident    isotopic    n2    composition    sufficient    optimal    stability    takes    operate    chemisorption    latter    power   

Project "MesoSi-CO2" data sheet

The following table provides information about the project.

Coordinator
NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU 

Organization address
address: HOGSKOLERINGEN 1
city: TRONDHEIM
postcode: 7491
website: www.ntnu.no

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Norway [NO]
 Total cost 202˙158 €
 EC max contribution 202˙158 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2019
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2020
 Duration (year-month-day) from 2020-10-01   to  2022-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU NO (TRONDHEIM) coordinator 202˙158.00

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 Project objective

Increasing carbon dioxide (CO2) concentrations in our atmosphere are becoming evident and are having a tremendous effect on the global temperature rise. Growing awareness of greenhouse gas emissions has led to the implementation of chemical CO2 utilization technologies. Tri-reforming of methane (TRM) can not only produce synthesis gas (CO H2) with desired H2/CO ratios (1.5–2.0) but can also eliminate carbon formation which is a serious problem in reforming of methane. Moreover, TRM allows converting CO2 directly from flue gases when applied in natural gas-fired power plants. However, a lack of catalysts able to operate efficiently with sufficient long-term stability hinders the development of the process. In this project, the proposed solution is to design a Ni-based mesoporous silica resistant to sintering and carbon formation and able to perform superior catalytic conversion of CO2. The synthesis of catalysts takes advantage of renewable bio-sources, zero-cost industrial waste and assistance of microwaves. The latter is applied to reduce power usage. The catalytic measurements will be performed with gas composition typical of flue gases from a natural-gas-fired power plant. The materials will be characterized by methods dedicated to examine physico-chemical features, such as XRD, N2 sorption, TPR, H2 chemisorption, TGA/DSC-MS, and XPS. The catalysts with optimal properties will be studied by steady-state isotopic transient kinetic analysis (SSITKA). Moreover, density functional theory (DFT) will be carried out to support the experiments. The understanding of possible deactivation mechanisms (carbon formation, sintering, selectivity towards side reactions) will be studied during the Secondment stay (Sorbonne Université, France). Operando XAS-XRD measurements will be performed to reveal the nature of active sites on the tri-reforming catalysts.

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