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MesoSi-CO2 SIGNED

Design of low-cost and carbon-resistant Ni-based mesoporous silicas for chemical CO2 utilization through tri-reforming of methane

Total Cost €

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EC-Contrib. €

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Partnership

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 MesoSi-CO2 project word cloud

Explore the words cloud of the MesoSi-CO2 project. It provides you a very rough idea of what is the project "MesoSi-CO2" about.

mechanisms    ratios    dsc    reforming    global    solution    tri    physico    operando    performed    density    chemisorption    gas    catalysts    stay    desired    effect    hinders    silica    sites    bio    superior    sources    temperature    technologies    methane    evident    carbon    reduce    kinetic    chemical    fired    reactions    universit    sorbonne    isotopic    tga    composition    examine    concentrations    takes    lack    trm    reveal    selectivity    eliminate    operate    waste    perform    secondment    plants    microwaves    dioxide    sorption    led    eacute    deactivation    steady    emissions    assistance    theory    catalytic    xas    xps    flue    nature    stability    tremendous    resistant    active    latter    n2    gases    dft    plant    experiments    conversion    sufficient    power    optimal    h2    converting    france    atmosphere    ni    advantage    ssitka    mesoporous    increasing    ms    tpr    functional    synthesis    xrd    serious    sintering    industrial    natural    materials    transient    zero    greenhouse    co2    renewable    co   

Project "MesoSi-CO2" data sheet

The following table provides information about the project.

Coordinator
NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU 

Organization address
address: HOGSKOLERINGEN 1
city: TRONDHEIM
postcode: 7491
website: www.ntnu.no

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Norway [NO]
 Total cost 202˙158 €
 EC max contribution 202˙158 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2019
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2020
 Duration (year-month-day) from 2020-10-01   to  2022-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU NO (TRONDHEIM) coordinator 202˙158.00

Map

 Project objective

Increasing carbon dioxide (CO2) concentrations in our atmosphere are becoming evident and are having a tremendous effect on the global temperature rise. Growing awareness of greenhouse gas emissions has led to the implementation of chemical CO2 utilization technologies. Tri-reforming of methane (TRM) can not only produce synthesis gas (CO H2) with desired H2/CO ratios (1.5–2.0) but can also eliminate carbon formation which is a serious problem in reforming of methane. Moreover, TRM allows converting CO2 directly from flue gases when applied in natural gas-fired power plants. However, a lack of catalysts able to operate efficiently with sufficient long-term stability hinders the development of the process. In this project, the proposed solution is to design a Ni-based mesoporous silica resistant to sintering and carbon formation and able to perform superior catalytic conversion of CO2. The synthesis of catalysts takes advantage of renewable bio-sources, zero-cost industrial waste and assistance of microwaves. The latter is applied to reduce power usage. The catalytic measurements will be performed with gas composition typical of flue gases from a natural-gas-fired power plant. The materials will be characterized by methods dedicated to examine physico-chemical features, such as XRD, N2 sorption, TPR, H2 chemisorption, TGA/DSC-MS, and XPS. The catalysts with optimal properties will be studied by steady-state isotopic transient kinetic analysis (SSITKA). Moreover, density functional theory (DFT) will be carried out to support the experiments. The understanding of possible deactivation mechanisms (carbon formation, sintering, selectivity towards side reactions) will be studied during the Secondment stay (Sorbonne Université, France). Operando XAS-XRD measurements will be performed to reveal the nature of active sites on the tri-reforming catalysts.

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