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MesoSi-CO2 SIGNED

Design of low-cost and carbon-resistant Ni-based mesoporous silicas for chemical CO2 utilization through tri-reforming of methane

Total Cost €

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EC-Contrib. €

0

Partnership

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 MesoSi-CO2 project word cloud

Explore the words cloud of the MesoSi-CO2 project. It provides you a very rough idea of what is the project "MesoSi-CO2" about.

density    greenhouse    synthesis    secondment    dft    takes    materials    gases    operando    bio    silica    global    zero    dioxide    composition    sorbonne    lack    superior    active    methane    tremendous    functional    reactions    serious    france    solution    technologies    operate    ni    experiments    reduce    tri    transient    increasing    theory    plant    sintering    catalytic    isotopic    universit    mesoporous    n2    physico    gas    xas    evident    natural    desired    assistance    co    h2    temperature    chemisorption    concentrations    selectivity    sources    xrd    perform    atmosphere    nature    latter    emissions    resistant    sorption    renewable    ratios    examine    sufficient    plants    trm    eliminate    carbon    performed    tga    stay    fired    sites    flue    industrial    co2    xps    effect    mechanisms    eacute    reforming    reveal    ssitka    power    chemical    kinetic    deactivation    led    ms    microwaves    dsc    stability    waste    converting    conversion    steady    hinders    optimal    tpr    advantage    catalysts   

Project "MesoSi-CO2" data sheet

The following table provides information about the project.

Coordinator
NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU 

Organization address
address: HOGSKOLERINGEN 1
city: TRONDHEIM
postcode: 7491
website: www.ntnu.no

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Norway [NO]
 Total cost 202˙158 €
 EC max contribution 202˙158 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2019
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2020
 Duration (year-month-day) from 2020-10-01   to  2022-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU NO (TRONDHEIM) coordinator 202˙158.00

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 Project objective

Increasing carbon dioxide (CO2) concentrations in our atmosphere are becoming evident and are having a tremendous effect on the global temperature rise. Growing awareness of greenhouse gas emissions has led to the implementation of chemical CO2 utilization technologies. Tri-reforming of methane (TRM) can not only produce synthesis gas (CO H2) with desired H2/CO ratios (1.5–2.0) but can also eliminate carbon formation which is a serious problem in reforming of methane. Moreover, TRM allows converting CO2 directly from flue gases when applied in natural gas-fired power plants. However, a lack of catalysts able to operate efficiently with sufficient long-term stability hinders the development of the process. In this project, the proposed solution is to design a Ni-based mesoporous silica resistant to sintering and carbon formation and able to perform superior catalytic conversion of CO2. The synthesis of catalysts takes advantage of renewable bio-sources, zero-cost industrial waste and assistance of microwaves. The latter is applied to reduce power usage. The catalytic measurements will be performed with gas composition typical of flue gases from a natural-gas-fired power plant. The materials will be characterized by methods dedicated to examine physico-chemical features, such as XRD, N2 sorption, TPR, H2 chemisorption, TGA/DSC-MS, and XPS. The catalysts with optimal properties will be studied by steady-state isotopic transient kinetic analysis (SSITKA). Moreover, density functional theory (DFT) will be carried out to support the experiments. The understanding of possible deactivation mechanisms (carbon formation, sintering, selectivity towards side reactions) will be studied during the Secondment stay (Sorbonne Université, France). Operando XAS-XRD measurements will be performed to reveal the nature of active sites on the tri-reforming catalysts.

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