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MesoSi-CO2 SIGNED

Design of low-cost and carbon-resistant Ni-based mesoporous silicas for chemical CO2 utilization through tri-reforming of methane

Total Cost €

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EC-Contrib. €

0

Partnership

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 MesoSi-CO2 project word cloud

Explore the words cloud of the MesoSi-CO2 project. It provides you a very rough idea of what is the project "MesoSi-CO2" about.

ni    deactivation    selectivity    transient    sorption    natural    temperature    methane    tpr    stay    plant    takes    performed    flue    kinetic    silica    theory    materials    optimal    assistance    hinders    physico    atmosphere    reveal    sources    solution    desired    h2    universit    evident    gas    sorbonne    trm    renewable    effect    mechanisms    isotopic    active    converting    steady    ms    plants    increasing    latter    gases    reactions    emissions    n2    ssitka    chemical    eliminate    waste    composition    technologies    global    stability    led    sufficient    dioxide    perform    eacute    co    functional    advantage    reduce    microwaves    experiments    ratios    greenhouse    mesoporous    sintering    industrial    superior    bio    co2    france    conversion    lack    dsc    sites    xrd    xps    catalysts    dft    operate    xas    nature    fired    operando    serious    secondment    tremendous    reforming    tri    synthesis    zero    examine    chemisorption    concentrations    power    resistant    tga    carbon    catalytic    density   

Project "MesoSi-CO2" data sheet

The following table provides information about the project.

Coordinator
NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU 

Organization address
address: HOGSKOLERINGEN 1
city: TRONDHEIM
postcode: 7491
website: www.ntnu.no

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Norway [NO]
 Total cost 202˙158 €
 EC max contribution 202˙158 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2019
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2020
 Duration (year-month-day) from 2020-10-01   to  2022-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    NORGES TEKNISK-NATURVITENSKAPELIGE UNIVERSITET NTNU NO (TRONDHEIM) coordinator 202˙158.00

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 Project objective

Increasing carbon dioxide (CO2) concentrations in our atmosphere are becoming evident and are having a tremendous effect on the global temperature rise. Growing awareness of greenhouse gas emissions has led to the implementation of chemical CO2 utilization technologies. Tri-reforming of methane (TRM) can not only produce synthesis gas (CO H2) with desired H2/CO ratios (1.5–2.0) but can also eliminate carbon formation which is a serious problem in reforming of methane. Moreover, TRM allows converting CO2 directly from flue gases when applied in natural gas-fired power plants. However, a lack of catalysts able to operate efficiently with sufficient long-term stability hinders the development of the process. In this project, the proposed solution is to design a Ni-based mesoporous silica resistant to sintering and carbon formation and able to perform superior catalytic conversion of CO2. The synthesis of catalysts takes advantage of renewable bio-sources, zero-cost industrial waste and assistance of microwaves. The latter is applied to reduce power usage. The catalytic measurements will be performed with gas composition typical of flue gases from a natural-gas-fired power plant. The materials will be characterized by methods dedicated to examine physico-chemical features, such as XRD, N2 sorption, TPR, H2 chemisorption, TGA/DSC-MS, and XPS. The catalysts with optimal properties will be studied by steady-state isotopic transient kinetic analysis (SSITKA). Moreover, density functional theory (DFT) will be carried out to support the experiments. The understanding of possible deactivation mechanisms (carbon formation, sintering, selectivity towards side reactions) will be studied during the Secondment stay (Sorbonne Université, France). Operando XAS-XRD measurements will be performed to reveal the nature of active sites on the tri-reforming catalysts.

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