ENREMOS

Enantioselective Reactions on Model Chirally Modified Surfaces

 Coordinatore MAX PLANCK GESELLSCHAFT ZUR FOERDERUNG DER WISSENSCHAFTEN E.V. 

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 Nazionalità Coordinatore Germany [DE]
 Totale costo 1˙589˙736 €
 EC contributo 1˙589˙736 €
 Programma FP7-IDEAS-ERC
Specific programme: "Ideas" implementing the Seventh Framework Programme of the European Community for research, technological development and demonstration activities (2007 to 2013)
 Code Call ERC-2013-StG
 Funding Scheme ERC-SG
 Anno di inizio 2014
 Periodo (anno-mese-giorno) 2014-01-01   -   2018-12-31

 Partecipanti

# participant  country  role  EC contrib. [€] 
1    MAX PLANCK GESELLSCHAFT ZUR FOERDERUNG DER WISSENSCHAFTEN E.V.

 Organization address address: Hofgartenstrasse 8
city: MUENCHEN
postcode: 80539

contact info
Titolo: Dr.
Nome: Swetlana
Cognome: Schauermann
Email: send email
Telefono: +49 30 84134142
Fax: +49 30 81434327

DE (MUENCHEN) hostInstitution 1˙589˙736.00
2    MAX PLANCK GESELLSCHAFT ZUR FOERDERUNG DER WISSENSCHAFTEN E.V.

 Organization address address: Hofgartenstrasse 8
city: MUENCHEN
postcode: 80539

contact info
Titolo: Prof.
Nome: Gert
Cognome: Von Helden
Email: send email
Telefono: 493084000000

DE (MUENCHEN) hostInstitution 1˙589˙736.00

Mappa


 Word cloud

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insights    chiral    enantioselective    catalytic    substrate    model    structure    molecular    dynamics    nanoparticles    modified    atomistic    metal    surfaces    enantiospecific    surface    reaction    kinetics    chirally    single   

 Obiettivo del progetto (Objective)

'Imparting chirality to non-chiral metal surfaces by adsorption of chiral modifiers is a highly promising route to create effective heterogeneously catalyzed processes for production of enantiopure pharmaceuticals. A molecular-level understanding of enantioselective processes on chiral surfaces is an importance prerequisite for the rational design of new enantiospecific catalysts. With the research outlined in this proposal we are aiming at a fundamental level understanding of the structure of chirally modified surfaces, the bonding of the prochiral substrate on the chiral media and the details of the kinetics and dynamics of enantioselective surface reactions. A full mechanistic picture can be obtained if these aspects will be understood both on the extended single crystal surfaces, mimicking a local interaction of the modifier-substrate complexes with a metal, as well as on the small chirally modified nanoparticles that more accurately resemble the structural properties and high catalytic activity of practically relevant powdered supported catalyst. To achieve these atomistic insights, we propose to apply a combination of ultrahigh vacuum (UHV) based methods for studying reaction kinetics and dynamics (multi-molecular beam techniques) and in-situ surface spectroscopic and microscopic tools on well-defined model surfaces consisting of metal nanoparticles supported on thin single crystalline oxide films. Complementary, the catalytic behaviour of these chirally modified model surfaces will be investigated under ambient pressure conditions with enantiospecific detection of the reaction products that will enable detailed atomistic insights into structure-reactivity relationships.'

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