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VIBCONTROL SIGNED

Vibronic control of organic electronic devices

Total Cost €

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EC-Contrib. €

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Partnership

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Project "VIBCONTROL" data sheet

The following table provides information about the project.

Coordinator
IMPERIAL COLLEGE OF SCIENCE TECHNOLOGY AND MEDICINE 

Organization address
address: SOUTH KENSINGTON CAMPUS EXHIBITION ROAD
city: LONDON
postcode: SW7 2AZ
website: http://www.imperial.ac.uk/

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country United Kingdom [UK]
 Total cost 1˙497˙257 €
 EC max contribution 1˙497˙257 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2014-STG
 Funding Scheme ERC-STG
 Starting year 2015
 Duration (year-month-day) from 2015-06-01   to  2021-05-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    IMPERIAL COLLEGE OF SCIENCE TECHNOLOGY AND MEDICINE UK (LONDON) coordinator 1˙490˙967.00
2    THE CHANCELLOR MASTERS AND SCHOLARSOF THE UNIVERSITY OF CAMBRIDGE UK (CAMBRIDGE) participant 6˙289.00

Map

 Project objective

Organic electronics (OE) is an expanding research field that exploits the electronic functionalities of organic molecules to make them robust and cost-efficient building blocks for future electronic devices. Due to the ‘soft’ character of organic materials, their electronic properties are defined by vibronic coupling (VC) phenomena which are a result of the interaction between electron and nuclear dynamics of the molecule. This research program aims to unlock a new direction of experimental studies investigating and exploiting VC in OE devices by using optical control of nuclear motion. The growing awareness that VC underlies diverse phenomena from physics to biology stimulates a broad interdisciplinary effort to address this issue. However, in the field of OE, the lack of synergy between device and optical studies holds the potential functionality offered by VC effects from being attained. In 2012, I proposed a direct route to control the performance of OE devices by optically switching the vibronic states of the molecules. Though this work came specifically in connection with organic photovoltaics, it provides the starting point for a more fundamental and broad reaching of VC phenomena. The proposed research program will use this opportunity. I will apply state-of-the-art developments in infrared light shaping to create a well-defined coherent superposition of molecular vibrational motions inside devices and study their influence on electron dynamics with device-specific spectroscopic techniques. This approach combines recent advances in ultrafast spectroscopy and OE to extend our fundamental understanding of molecular charge transport. Our methodology will become a tool for elucidating current pathways in organic nanodevices and offer access to non-equilibrium phenomena down to the level of molecular junctions. This research will lead to the development of new design rules for OE materials serving future advances in molecular electronics, computing and sensing.

 Publications

year authors and title journal last update
List of publications.
2018 Deping Qian, Zilong Zheng, Huifeng Yao, Wolfgang Tress, Thomas R. Hopper, Shula Chen, Sunsun Li, Jing Liu, Shangshang Chen, Jiangbin Zhang, Xiao-Ke Liu, Bowei Gao, Liangqi Ouyang, Yingzhi Jin, Galia Pozina, Irina A. Buyanova, Weimin M. Chen, Olle Inganäs, Veaceslav Coropceanu, Jean-Luc Bredas, He Yan, Jianhui Hou, Fengling Zhang, Artem A. Bakulin, Feng Gao
Design rules for minimizing voltage losses in high-efficiency organic solar cells
published pages: 703-709, ISSN: 1476-1122, DOI: 10.1038/s41563-018-0128-z
Nature Materials 17/8 2020-01-24
2016 Artem A. Bakulin, Carlos Silva, Eleonora Vella
Ultrafast Spectroscopy with Photocurrent Detection: Watching Excitonic Optoelectronic Systems at Work
published pages: 250-258, ISSN: 1948-7185, DOI: 10.1021/acs.jpclett.5b01955
The Journal of Physical Chemistry Letters 7/2 2020-01-24
2015 Artem A. Bakulin, Robert Lovrincic, Xi Yu, Oleg Selig, Huib J. Bakker, Yves L. A. Rezus, Pabitra K. Nayak, Alexandr Fonari, Veaceslav Coropceanu, Jean-Luc Brédas, David Cahen
Mode-selective vibrational modulation of charge transport in organic electronic devices
published pages: 7880, ISSN: 2041-1723, DOI: 10.1038/ncomms8880
Nature Communications 6 2020-01-24

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