Explore the words cloud of the MONACAT project. It provides you a very rough idea of what is the project "MONACAT" about.
The following table provides information about the project.
CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS
|Coordinator Country||France [FR]|
|Total cost||2˙472˙222 €|
|EC max contribution||2˙472˙222 € (100%)|
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
|Duration (year-month-day)||from 2016-06-01 to 2021-05-31|
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|1||CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS||FR (PARIS)||coordinator||2˙472˙222.00|
MONACAT proposes a novel approach to address the challenge of intermittent energy storage. Specifically, the purpose is to conceive and synthesize novel complex nano-objects displaying both physical and chemical properties that enable catalytic transformations with a fast and optimum energy conversion. It follows over 20 years of research on “organometallic nanoparticles”, an approach of nanoparticles (NPs) synthesis where the first goal is to control the surface of the particles as in molecular organometallic species. Two families of NPs will be studied: 1) magnetic NPs that can be heated by excitation with an alternating magnetic field and 2) plasmonic NPs that absorb visible light and transform it into heat. In all cases, deposition of additional materials as islands or thin layers will improve the NPs catalytic activity. Iron carbides NPs have recently been shown to heat efficiently upon magnetic excitation and to catalyse CO hydrogenation into hydrocarbons. In order to transform this observation into a viable process, MONACAT will address the following challenges: determination and control of surface temperature using fluorophores or quantum dots, optimization of heating capacity (size, anisotropy of the material, crystallinity, phases: FeCo, FeNi, chemical order), optimization of catalytic properties (islands vs core-shell structures; Ru, Ni for methane, Cu/Zn for methanol), stability and optimization of energy efficiency. A similar approach will be used for direct light conversion using as first proofs of concept Au or Ag NPs coated with Ru. Catalytic tests will be performed on two heterogeneous reactions after deposition of the NPs onto a support: CO2 hydrogenation into methane and methanol synthesis. In addition, the potential of catalysis making use of self-heated and magnetically recoverable NPs will be studied in solution (reduction of arenes or oxygenated functions, hydrogenation and hydrogenolysis of biomass platform molecules, Fischer-Tropsch).
|year||authors and title||journal||last update|
Julien Marbaix, Nicolas Mille, Lise-Marie Lacroix, Juan Manuel Asensio, Pier-Francesco Fazzini, Katerina Soulantica, Julian Carrey, Bruno Chaudret
Tuning the Composition of FeCo Nanoparticle Heating Agents for Magnetically Induced Catalysis
published pages: , ISSN: 2574-0970, DOI: 10.1021/acsanm.0c00444
|ACS Applied Nano Materials||2020-04-24|
Julien Marbaix, Pauline Kerroux, Ludovic Montastruc, Katerina Soulantica, Bruno Chaudret
CO2 methanation activated by magnetic heating: life cycle assessment and perspectives for successful renewable energy storage
published pages: , ISSN: 0948-3349, DOI: 10.1007/s11367-020-01734-8
|The International Journal of Life Cycle Assessment||2020-02-20|
Sumeet S. Kale, Juan M. Asensio, Marta Estrader, Mayke Werner, Alexis Bordet, Deliang Yi, Julien Marbaix, Pier-Francesco Fazzini, Katerina Soulantica, Bruno Chaudret
Iron carbide or iron carbide/cobalt nanoparticles for magnetically-induced CO 2 hydrogenation over Ni/SiRAlOx catalysts
published pages: 2601-2607, ISSN: 2044-4753, DOI: 10.1039/c9cy00437h
|Catalysis Science & Technology 9/10||2020-01-14|
Juan M. Asensio, Donia Bouzouita, Piet W. N. M. van Leeuwen, Bruno Chaudret
Ïƒ-Hâ€“H, Ïƒ-Câ€“H, and Ïƒ-Siâ€“H Bond Activation Catalyzed by Metal Nanoparticles
published pages: , ISSN: 0009-2665, DOI: 10.1021/acs.chemrev.9b00368
Edwin A. Baquero, HÃ©loÃ¯se Virieux, Robert A. Swain, AngÃ©lique Gillet, Arnaud Cros-Gagneux, Yannick Coppel, Bruno Chaudret, CÃ©line Nayral, Fabien Delpech
Synthesis of Oxide-Free InP Quantum Dots: Surface Control and H 2 -Assisted Growth
published pages: 9623-9627, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.7b04069
|Chemistry of Materials 29/22||2019-08-05|
Diego Mateo, Deborah Deâ€…Masi, Josep Albero, Liseâ€Marie Lacroix, Pierâ€Francesco Fazzini, Bruno Chaudret, Hermenegildo GarcÃa
Synergism of Au and Ru Nanoparticles in Lowâ€Temperature Photoassisted CO 2 Methanation
published pages: 18436-18443, ISSN: 0947-6539, DOI: 10.1002/chem.201803022
|Chemistry â€“ A European Journal 24/69||2019-04-18|
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