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MONACAT SIGNED

Magnetism and Optics for Nanoparticle Catalysis

Total Cost €

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EC-Contrib. €

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Partnership

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 MONACAT project word cloud

Explore the words cloud of the MONACAT project. It provides you a very rough idea of what is the project "MONACAT" about.

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Project "MONACAT" data sheet

The following table provides information about the project.

Coordinator
CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS 

Organization address
address: RUE MICHEL ANGE 3
city: PARIS
postcode: 75794
website: www.cnrs.fr

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country France [FR]
 Total cost 2˙472˙222 €
 EC max contribution 2˙472˙222 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2015-AdG
 Funding Scheme ERC-ADG
 Starting year 2016
 Duration (year-month-day) from 2016-06-01   to  2021-05-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS FR (PARIS) coordinator 2˙472˙222.00

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 Project objective

MONACAT proposes a novel approach to address the challenge of intermittent energy storage. Specifically, the purpose is to conceive and synthesize novel complex nano-objects displaying both physical and chemical properties that enable catalytic transformations with a fast and optimum energy conversion. It follows over 20 years of research on “organometallic nanoparticles”, an approach of nanoparticles (NPs) synthesis where the first goal is to control the surface of the particles as in molecular organometallic species. Two families of NPs will be studied: 1) magnetic NPs that can be heated by excitation with an alternating magnetic field and 2) plasmonic NPs that absorb visible light and transform it into heat. In all cases, deposition of additional materials as islands or thin layers will improve the NPs catalytic activity. Iron carbides NPs have recently been shown to heat efficiently upon magnetic excitation and to catalyse CO hydrogenation into hydrocarbons. In order to transform this observation into a viable process, MONACAT will address the following challenges: determination and control of surface temperature using fluorophores or quantum dots, optimization of heating capacity (size, anisotropy of the material, crystallinity, phases: FeCo, FeNi, chemical order), optimization of catalytic properties (islands vs core-shell structures; Ru, Ni for methane, Cu/Zn for methanol), stability and optimization of energy efficiency. A similar approach will be used for direct light conversion using as first proofs of concept Au or Ag NPs coated with Ru. Catalytic tests will be performed on two heterogeneous reactions after deposition of the NPs onto a support: CO2 hydrogenation into methane and methanol synthesis. In addition, the potential of catalysis making use of self-heated and magnetically recoverable NPs will be studied in solution (reduction of arenes or oxygenated functions, hydrogenation and hydrogenolysis of biomass platform molecules, Fischer-Tropsch).

 Publications

year authors and title journal last update
List of publications.
2020 Julien Marbaix, Nicolas Mille, Lise-Marie Lacroix, Juan Manuel Asensio, Pier-Francesco Fazzini, Katerina Soulantica, Julian Carrey, Bruno Chaudret
Tuning the Composition of FeCo Nanoparticle Heating Agents for Magnetically Induced Catalysis
published pages: , ISSN: 2574-0970, DOI: 10.1021/acsanm.0c00444
ACS Applied Nano Materials 2020-04-24
2020 Julien Marbaix, Pauline Kerroux, Ludovic Montastruc, Katerina Soulantica, Bruno Chaudret
CO2 methanation activated by magnetic heating: life cycle assessment and perspectives for successful renewable energy storage
published pages: , ISSN: 0948-3349, DOI: 10.1007/s11367-020-01734-8
The International Journal of Life Cycle Assessment 2020-02-20
2019 Sumeet S. Kale, Juan M. Asensio, Marta Estrader, Mayke Werner, Alexis Bordet, Deliang Yi, Julien Marbaix, Pier-Francesco Fazzini, Katerina Soulantica, Bruno Chaudret
Iron carbide or iron carbide/cobalt nanoparticles for magnetically-induced CO 2 hydrogenation over Ni/SiRAlOx catalysts
published pages: 2601-2607, ISSN: 2044-4753, DOI: 10.1039/c9cy00437h
Catalysis Science & Technology 9/10 2020-01-14
2019 Juan M. Asensio, Donia Bouzouita, Piet W. N. M. van Leeuwen, Bruno Chaudret
σ-H–H, σ-C–H, and σ-Si–H Bond Activation Catalyzed by Metal Nanoparticles
published pages: , ISSN: 0009-2665, DOI: 10.1021/acs.chemrev.9b00368
Chemical Reviews 2020-01-14
2017 Edwin A. Baquero, Héloïse Virieux, Robert A. Swain, Angélique Gillet, Arnaud Cros-Gagneux, Yannick Coppel, Bruno Chaudret, Céline Nayral, Fabien Delpech
Synthesis of Oxide-Free InP Quantum Dots: Surface Control and H 2 -Assisted Growth
published pages: 9623-9627, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.7b04069
Chemistry of Materials 29/22 2019-08-05
2018 Diego Mateo, Deborah De Masi, Josep Albero, Lise‐Marie Lacroix, Pier‐Francesco Fazzini, Bruno Chaudret, Hermenegildo García
Synergism of Au and Ru Nanoparticles in Low‐Temperature Photoassisted CO 2 Methanation
published pages: 18436-18443, ISSN: 0947-6539, DOI: 10.1002/chem.201803022
Chemistry – A European Journal 24/69 2019-04-18

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