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AMPLIPORE SIGNED

Understanding negative gas adsorption in highly porous networks for the design of pressure amplifying materials

Total Cost €

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EC-Contrib. €

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Partnership

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 AMPLIPORE project word cloud

Explore the words cloud of the AMPLIPORE project. It provides you a very rough idea of what is the project "AMPLIPORE" about.

transformation    amplipore    elaborate    materials    synthetic    elucidate    transportation    paradoxical    release    signatures    colossal    polymers    time    pressure    outer    macroscopic    micropumps    negative    mesopore    ranges    external    opposite    group    releasing    pneumatic    microfluidic    material    mesoscopic    force    always    instrumentation    insights    never    innovations    tailor    mechanisms    crystal    gas    nga    tailormade    2016    industrial    fundamental    normal    combining    react    temperature    direction    area    lungs    networks    transformations    solid    point    intrinsic    inner    micropore    artificial    dynamics    physical    amplifying    boundary    selfcompression    phenomena    reported    prerequisite    reservoir    structures    surface    adsorption    molecular    micropneumatic    solely    first    certain    investigations    counteracts    featuring    techniques    amplification    kinetic    counterintuitive    analytical    instead    thermodynamic    give    phenomenon    rescue    actuators    surrounding    explore    closed   

Project "AMPLIPORE" data sheet

The following table provides information about the project.

Coordinator
TECHNISCHE UNIVERSITAET DRESDEN 

Organization address
address: HELMHOLTZSTRASSE 10
city: DRESDEN
postcode: 1069
website: http://www.tu-dresden.de/

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Total cost 2˙363˙125 €
 EC max contribution 2˙363˙125 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2016-ADG
 Funding Scheme ERC-ADG
 Starting year 2017
 Duration (year-month-day) from 2017-09-01   to  2022-08-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    TECHNISCHE UNIVERSITAET DRESDEN DE (DRESDEN) coordinator 2˙363˙125.00

Map

 Project objective

Negative gas adsorption (NGA) is a new, counterintuitive and paradoxical phenomenon, for the first time reported by my group in 2016: Normal solid materials with significant outer or inner surface area always take up gas when the pressure in the surrounding reservoir is increased (adsorption). NGA networks instead react at a certain point in the opposite direction: They release gas upon external pressure increase, leading to an overall pressure amplification in a closed system. Comparable phenomena have never been reported before. What is so exciting about NGA? We have a unique material in hand, that counteracts to an external force by force amplification. So far NGA has solely been observed in one of our new coordination polymers, featuring a colossal selfcompression associated with a mesopore-to-micropore transformation. Gas pressure amplifying materials could lead to important innovations in gas releasing rescue systems, pneumatic control systems (production, transportation), micropumps, microfluidic devices, pneumatic actuators, and artificial lungs. A fundamental understanding of the physical mechanisms, structures, and thermodynamic boundary conditions is an essential prerequisite for any industrial application of this counterintuitive phenomenon. Combining strong synthetic methodologies with advanced analytical techniques, AMPLIPORE will elucidate the characteristic molecular and mesoscopic materials signatures as well as thermodynamic boundary conditions of NGA phenomena. We will elaborate a generic NGA-materials concept to tailor the pressure amplification and explore temperature and pressure ranges at which NGA can be applied. Developing tailormade instrumentation for kinetic investigations of NGA will give fundamental insights into the intrinsic and macroscopic dynamics of crystal-to-crystal transformations for applications in micropneumatic systems.

 Publications

year authors and title journal last update
List of publications.
2019 Simon Krause, Jack D. Evans, Volodymyr Bon, Irena Senkovska, Paul Iacomi, Felicitas Kolbe, Sebastian Ehrling, Erik Troschke, Jürgen Getzschmann, Daniel D. Többens, Alexandra Franz, Dirk Wallacher, Pascal G. Yot, Guillaume Maurin, Eike Brunner, Philip L. Llewellyn, François-Xavier Coudert, Stefan Kaskel
Towards General Network Architecture Design Criteria for Negative GasAdsorption Transitions in Ultraporous Frameworks
published pages: , ISSN: 2573-2293, DOI: 10.26434/chemrxiv.7796543.v1
ChemRxiv 2019-05-23
2018 Simon Krause, Volodymyr Bon, Irena Senkovska, Daniel M. Többens, Dirk Wallacher, Renjith S. Pillai, Guillaume Maurin, Stefan Kaskel
The effect of crystallite size on pressure amplification in switchable porous solids
published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-018-03979-2
Nature Communications 9/1 2019-05-23
2019 Jack D. Evans, Simon Krause, Stefan Kaskel, Martin B. Sweatman, Lev Sarkisov
Exploring the thermodynamic criteria for responsive adsorption processes
published pages: , ISSN: 2041-6520, DOI: 10.1039/c9sc01299k
Chemical Science 2019-05-23
2018 Simon Krause, Jack D. Evans, Volodymyr Bon, Irena Senkovska, Sebastian Ehrling, Ulrich Stoeck, Pascal Yot, Paul Iacomi, Philip Llewellyn, Guillaume Maurin, François-Xavier Coudert, Stefan Kaskel
Adsorption Contraction Mechanics: Understanding Breathing Energeticsin Isoreticular Metal-Organic Frameworks
published pages: , ISSN: 2573-2293, DOI: 10.26434/chemrxiv.5962240.v1
ChemRxiv 2019-05-27

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