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CASCAT SIGNED

Catalytic cascade reactions. From fundamentals of nanozymes to applications based on gas-diffusion electrodes

Total Cost €

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EC-Contrib. €

0

Partnership

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 CASCAT project word cloud

Explore the words cloud of the CASCAT project. It provides you a very rough idea of what is the project "CASCAT" about.

bimetallic    electrodes    particles    synergistically    co2    recycling    local    crossings    electrochemistry    perform    spectroscopy    channels    densities    reaction    electrolyte    h2    actualise    n2    channel    shell    nanoparticle    unprecedented    modulation    chemical    sites    additionally    hazardous    pollutants    substantial    reactions    extended    cycle    simplified    confined    anisotropic    electrolysers    catalysts    reactant    etched    converted    feasible    cascade    core    catalytically    selectivity    nh3    nanozymes    nano    decrease    electrocatalysis    layered    designed    tools    composition    hydrophobic    enzyme    nanoparticles    flow    diffusion    selectively    street    solution    boundary    substrate    locally    exemplified    gaseous    evaluation    carbon    economy    provision    catalytic    previously    emission    tree    rotating    alkaline    electrochemical    envisioning    contributions    generates    first    relative    gas    fundamental    density    catalysed    varying    mimic    operando    volumes    removal    cities    suppression    material    active    hydrocarbons    extensive    follow    catalyst    concave    competition    nox    structures    electrolyser    assemble    location    hydrophilic    entrance    surfaces    concerning    air    closed    endeavour   

Project "CASCAT" data sheet

The following table provides information about the project.

Coordinator
RUHR-UNIVERSITAET BOCHUM 

Organization address
address: UNIVERSITAETSSTRASSE 150
city: BOCHUM
postcode: 44801
website: www.rub.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Total cost 2˙499˙462 €
 EC max contribution 2˙499˙462 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2018-ADG
 Funding Scheme ERC-ADG
 Starting year 2019
 Duration (year-month-day) from 2019-09-01   to  2024-08-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    RUHR-UNIVERSITAET BOCHUM DE (BOCHUM) coordinator 2˙499˙462.00

Map

 Project objective

Nanoparticles with etched substrate channels are proposed as a simplified enzyme mimic, nanozymes, for electrocatalysis providing concave catalytically active sites together with the local modulation of electrolyte composition. This concept will be extended to bimetallic core-shell structures with etched channels to provide locally confined catalyst surfaces with varying selectivity. The first catalytic reaction at the channel entrance selectively generates a product, which is further converted in a follow-up reaction catalysed at the core material at the bottom of the channel. The endeavour to locally assemble catalysts with different properties in nano-confined reaction volumes to actualise cascade reaction pathways will be extended to layered nanoparticle structures. Together with an anisotropic provision of a gaseous reactant through a hydrophobic/hydrophilic phase boundary of specifically designed gas diffusion electrodes multi-step catalytic cascade reactions become feasible. The development and extensive evaluation of multi-catalyst gas-diffusion electrodes using operando electrochemistry/spectroscopy and nano-electrochemical tools as well as multi flow-through electrolysers will provide the fundamental knowledge concerning the relative location of different catalyst particles, which synergistically perform chemical cascade reaction with high selectivity and at high current densities. These gas-diffusion electrodes will be integrated in novel electrolyser concepts targeting CO2 recycling at high current density in alkaline solution under suppression of H2 competition with previously unprecedented selectivity for the formation of higher hydrocarbons envisioning contributions to a closed carbon cycle economy and a substantial decrease of CO2 emission. Additionally, a novel tree-type rotating electrolyser design is proposed for the removal of hazardous gaseous pollutants from air e.g. at street crossings in cities as exemplified by NOx reduction to N2 or NH3.

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The information about "CASCAT" are provided by the European Opendata Portal: CORDIS opendata.

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