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COUPC1 SIGNED

Coupling strategies for scavenging reactive C1 intermediates in hydrogen generation

Total Cost €

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EC-Contrib. €

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Partnership

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 COUPC1 project word cloud

Explore the words cloud of the COUPC1 project. It provides you a very rough idea of what is the project "COUPC1" about.

prof    reverse    country    pd    au    distances    close    requiring    water    promoted    co    microscopic    ceo2    dehydration    catalyze    gonz    shift    formic    de    hcooh    function    channelling    mixtures    gas    functions    iglesia    enrique    scavenging    feedstocks    positioning    group    detected    dehydrate    interfacial    carrier    hydrogenation    forms    notable    effect    aacute    intermediates    acid    basque    plausible    co2    cu    berkeley    reaction    recent    microreverse    summarizing    shuttle    gaseous    reactants    dehydrogenation    catalyst    situ    selective    unstable    selectively    return    pt    biogenic    university    completing    lez    intermediate    reactive    velasco    researcher    molecular    molecules    suggested    turnover    tio2    lsac    h2    mediated    promotional    oxides    diffusion    natural    formed    supervision    thermodynamically    involvement    bond    worldwide    h2o    precise    seconded    details    spain    permit    unveil    routes    methanol    mechanistic    usa    atomic    metals    contact    dehydrogenates    subsequent    c1    la    zno    uc    wgs    torre   

Project "COUPC1" data sheet

The following table provides information about the project.

Coordinator
UNIVERSIDAD DEL PAIS VASCO/ EUSKAL HERRIKO UNIBERTSITATEA 

Organization address
address: BARRIO SARRIENA S N
city: LEIOA
postcode: 48940
website: www.ehu.es

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Spain [ES]
 Total cost 204˙415 €
 EC max contribution 204˙415 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2019
 Funding Scheme MSCA-IF-GF
 Starting year 2020
 Duration (year-month-day) from 2020-04-01   to  2022-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    UNIVERSIDAD DEL PAIS VASCO/ EUSKAL HERRIKO UNIBERTSITATEA ES (LEIOA) coordinator 204˙415.00
2    THE REGENTS OF THE UNIVERSITY OF CALIFORNIA US (OAKLAND CA) partner 0.00

Map

 Project objective

Recent findings have suggested the plausible involvement of formic acid (HCOOH) as a gaseous molecular shuttle in WGS reaction , which is specifically promoted by oxides (ZnO, CeO2, TiO2) that are known to selectively dehydrate HCOOH (microreverse of HCOOH formation from CO and H2O) and metals (Cu, Pt, Pd, Au) that do dehydrogenation (to CO2 and H2 in WGS) and hydrogenation (to methanol). The intermediate of interest (HCOOH) is formed in situ from CO/H2O mixtures on metals and oxides that catalyze selective HCOOH dehydration, and thus its microscopic reverse. Subsequent HCOOH dehydrogenation would lead to the formation of H2 and CO2, completing a water-gas shift (WGS ) turnover without requiring interfacial contact among functions. A notable promotional effect has been recently detected in catalyst without requiring atomic contact, meaning that the two functions need to be “close” but not in atomic contact but involving a molecular carrier. The mechanistic details of such diffusion-mediated routes would unveil new opportunities for the specific channelling of such intermediates towards H2 and CO2, through precise positioning of a function that forms HCOOH from CO/H2O reactants and another function, present beyond atomic contact but within diffusion distances, that dehydrogenates gaseous HCOOH to H2 and CO2. Summarizing, this research would permit controlling the WGS process in order to increase H2 production worldwide. The proposed research will address the formation and scavenging of reactive and thermodynamically unstable intermediates without a C-C bond, which can be formed from C1 molecules (specifically natural gas or biogenic feedstocks), through the precise positioning for their formation and scavenging functions. The researcher U. De La Torre will be seconded to the LSAC group at UC Berkeley (USA) under the supervision of Prof. Enrique Iglesia, and will return to the University of the Basque Country (Spain) under the supervision of Prof. González-Velasco.

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