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FeREDCOUPLS SIGNED

FeREDCOUPLS - Reduced Iron Catalysts for Reduction and Coupling Reactions

Total Cost €

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EC-Contrib. €

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Partnership

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 FeREDCOUPLS project word cloud

Explore the words cloud of the FeREDCOUPLS project. It provides you a very rough idea of what is the project "FeREDCOUPLS" about.

efficient    metal    solvent    chemicals    demand    electron    vs    energy    economic    endeavour    complexes    technologies    synthesis    shortages    nanoparticles    coordinative    emphasis    preparations    arenes    active    liquids    reactions    species    manufacture    environmental    reducing    puzzle    accumulation    extends    societal    relevance    valuable    catalysts    ionic    centers    olefins    noble    ligands    transition    whereas    defunctionalization    centered    greener    transformations    hydrogenation    co    power    realm    reaction    substrates    capitalizes    coupling    greatest    sustainable    generation    planet    acids    oxidized    abundant    materials    carriers    activations    lewis    cross    catalytic    practical    toward    realization    catalysis    placed    operation    reductive    stabilized    accommodate    fe    direct    stabilization    bond    valent    piece    ligand    iron    cheap    mechanistic    spectroscopy    scientific    aerobic    sustainability    chemical    multidisciplinary    redox    exploits    metals    special   

Project "FeREDCOUPLS" data sheet

The following table provides information about the project.

Coordinator
UNIVERSITAET HAMBURG 

Organization address
address: MITTELWEG 177
city: HAMBURG
postcode: 20148
website: n.a.

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Total cost 1˙995˙400 €
 EC max contribution 1˙995˙400 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2015-CoG
 Funding Scheme ERC-COG
 Starting year 2016
 Duration (year-month-day) from 2016-10-01   to  2021-09-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    UNIVERSITAET HAMBURG DE (HAMBURG) coordinator 1˙645˙184.00
2    UNIVERSITAET REGENSBURG DE (REGENSBURG) participant 350˙215.00

Map

 Project objective

The aerobic conditions on our planet enable the accumulation of oxidized matter whereas reduced chemicals are the most valuable energy carriers. Future shortages of energy-rich resources make efficient reductive transformations one of the greatest scientific challenges. To address this societal, economic and environmental demand, we propose new approaches to the design and application of stabilized iron catalysts. Our endeavour exploits the higher reducing power of Fe (vs. noble metals) in challenging reductive transformations and capitalizes on the high sustainability of Fe catalysis over noble metal technologies. The use of low-valent Fe catalysts, the realization of new catalytic reactions and their mechanistic understanding will only be possible through the controlled generation and effective stabilization of reduced Fe species and active nanoparticles. Major emphasis will be placed on coordinative ligand/solvent systems which accommodate electron-rich Fe centers (olefins, arenes, Lewis acids, redox-ligands, ionic liquids). We address new approaches to the synthesis of low-valent Fe complexes and bottom-up/top-down preparations of Fe(0) nanoparticles. Catalytic reactions of high relevance to the manufacture of chemicals and materials will be studied (reduction, cross-coupling, hydrogenation, defunctionalization) with special emphasis on cheap abundant substrates. Mechanistic studies aim at understanding Fe-centered reductive bond activations and ligand co-operation. The proposed use of the most abundant transition metal for challenging reductive processes under practical conditions extends beyond the realm of synthesis, catalysis, and materials into spectroscopy, solvent technologies and reaction processing with direct relevance to sustainable chemicals and energy production. Our multidisciplinary program will provide new sets of active iron catalysts for reductive processes and is a major puzzle piece toward a greener chemical synthesis.

 Publications

year authors and title journal last update
List of publications.
2018 Guojiao Wu, Axel Jacobi von Wangelin
Stereoselective cobalt-catalyzed halofluoroalkylation of alkynes
published pages: 1795-1802, ISSN: 2041-6520, DOI: 10.1039/c7sc04916a
Chemical Science 9/7 2019-08-06
2017 Matteo Villa, Dominique Miesel, Alexander Hildebrandt, Fabio Ragaini, Dieter Schaarschmidt, Axel Jacobi von Wangelin
Synthesis and Catalysis of Redox-Active Bis(imino)acenaphthene (BIAN) Iron Complexes
published pages: 3203-3209, ISSN: 1867-3880, DOI: 10.1002/cctc.201700144
ChemCatChem 9/16 2019-07-02
2017 Tim N. Gieshoff, Uttam Chakraborty, Matteo Villa, Axel Jacobi von Wangelin
Alkene Hydrogenations by Soluble Iron Nanocluster Catalysts
published pages: 3585-3589, ISSN: 1433-7851, DOI: 10.1002/anie.201612548
Angewandte Chemie International Edition 56/13 2019-08-06
2017 Philipp Büschelberger, Dominik Gärtner, Efrain Reyes-Rodriguez, Friedrich Kreyenschmidt, Konrad Koszinowski, Axel Jacobi von Wangelin, Robert Wolf
Alkene Metalates as Hydrogenation Catalysts
published pages: 3139-3151, ISSN: 0947-6539, DOI: 10.1002/chem.201605222
Chemistry - A European Journal 23/13 2019-07-02
2018 Uttam Chakraborty, Efrain Reyes-Rodriguez, Serhiy Demeshko, Franc Meyer, Axel Jacobi von Wangelin
A Manganese Nanosheet: New Cluster Topology and Catalysis
published pages: 4970-4975, ISSN: 1433-7851, DOI: 10.1002/anie.201800079
Angewandte Chemie International Edition 57/18 2019-08-06
2018 Guojiao Wu, Uttam Chakraborty, Axel Jacobi von Wangelin
Regiocontrol in the cobalt-catalyzed hydrosilylation of alkynes
published pages: 12322-12325, ISSN: 1359-7345, DOI: 10.1039/c8cc07267a
Chemical Communications 54/87 2019-08-06

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