Explore the words cloud of the FeREDCOUPLS project. It provides you a very rough idea of what is the project "FeREDCOUPLS" about.
The following table provides information about the project.
|Coordinator Country||Germany [DE]|
|Total cost||1˙995˙400 €|
|EC max contribution||1˙995˙400 € (100%)|
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
|Duration (year-month-day)||from 2016-10-01 to 2021-09-30|
Take a look of project's partnership.
|1||UNIVERSITAET HAMBURG||DE (HAMBURG)||coordinator||1˙645˙184.00|
|2||UNIVERSITAET REGENSBURG||DE (REGENSBURG)||participant||350˙215.00|
The aerobic conditions on our planet enable the accumulation of oxidized matter whereas reduced chemicals are the most valuable energy carriers. Future shortages of energy-rich resources make efficient reductive transformations one of the greatest scientific challenges. To address this societal, economic and environmental demand, we propose new approaches to the design and application of stabilized iron catalysts. Our endeavour exploits the higher reducing power of Fe (vs. noble metals) in challenging reductive transformations and capitalizes on the high sustainability of Fe catalysis over noble metal technologies. The use of low-valent Fe catalysts, the realization of new catalytic reactions and their mechanistic understanding will only be possible through the controlled generation and effective stabilization of reduced Fe species and active nanoparticles. Major emphasis will be placed on coordinative ligand/solvent systems which accommodate electron-rich Fe centers (olefins, arenes, Lewis acids, redox-ligands, ionic liquids). We address new approaches to the synthesis of low-valent Fe complexes and bottom-up/top-down preparations of Fe(0) nanoparticles. Catalytic reactions of high relevance to the manufacture of chemicals and materials will be studied (reduction, cross-coupling, hydrogenation, defunctionalization) with special emphasis on cheap abundant substrates. Mechanistic studies aim at understanding Fe-centered reductive bond activations and ligand co-operation. The proposed use of the most abundant transition metal for challenging reductive processes under practical conditions extends beyond the realm of synthesis, catalysis, and materials into spectroscopy, solvent technologies and reaction processing with direct relevance to sustainable chemicals and energy production. Our multidisciplinary program will provide new sets of active iron catalysts for reductive processes and is a major puzzle piece toward a greener chemical synthesis.
|year||authors and title||journal||last update|
Guojiao Wu, Axel Jacobi von Wangelin
Stereoselective cobalt-catalyzed halofluoroalkylation of alkynes
published pages: 1795-1802, ISSN: 2041-6520, DOI: 10.1039/c7sc04916a
|Chemical Science 9/7||2019-08-06|
Matteo Villa, Dominique Miesel, Alexander Hildebrandt, Fabio Ragaini, Dieter Schaarschmidt, Axel Jacobiâ€…vonâ€…Wangelin
Synthesis and Catalysis of Redox-Active Bis(imino)acenaphthene (BIAN) Iron Complexes
published pages: 3203-3209, ISSN: 1867-3880, DOI: 10.1002/cctc.201700144
Tim N. Gieshoff, Uttam Chakraborty, Matteo Villa, Axel Jacobiâ€…vonâ€…Wangelin
Alkene Hydrogenations by Soluble Iron Nanocluster Catalysts
published pages: 3585-3589, ISSN: 1433-7851, DOI: 10.1002/anie.201612548
|Angewandte Chemie International Edition 56/13||2019-08-06|
Philipp BÃ¼schelberger, Dominik GÃ¤rtner, Efrain Reyes-Rodriguez, Friedrich Kreyenschmidt, Konrad Koszinowski, Axel Jacobiâ€…vonâ€…Wangelin, Robert Wolf
Alkene Metalates as Hydrogenation Catalysts
published pages: 3139-3151, ISSN: 0947-6539, DOI: 10.1002/chem.201605222
|Chemistry - A European Journal 23/13||2019-07-02|
Uttam Chakraborty, Efrain Reyes-Rodriguez, Serhiy Demeshko, Franc Meyer, Axel Jacobiâ€…vonâ€…Wangelin
A Manganese Nanosheet: New Cluster Topology and Catalysis
published pages: 4970-4975, ISSN: 1433-7851, DOI: 10.1002/anie.201800079
|Angewandte Chemie International Edition 57/18||2019-08-06|
Guojiao Wu, Uttam Chakraborty, Axel Jacobi von Wangelin
Regiocontrol in the cobalt-catalyzed hydrosilylation of alkynes
published pages: 12322-12325, ISSN: 1359-7345, DOI: 10.1039/c8cc07267a
|Chemical Communications 54/87||2019-08-06|
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