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NANOCHEM SIGNED

Nanopores for New Molecular Nitrogen Chemistry

Total Cost €

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EC-Contrib. €

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Partnership

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 NANOCHEM project word cloud

Explore the words cloud of the NANOCHEM project. It provides you a very rough idea of what is the project "NANOCHEM" about.

dynamic    n2h4    mof    assembly    construction    society    porous    stores    re    direct    capture    structural    pore    n2o4    decoration    containing    nox    stability    separation    no2    catalytic    gain    interactions    environmentally    host    impacts    catalysts    organic    adsorption    academia    chemistry    degradation    tests    molecules    improvement    functionalized    substrate    situ    confined    extensive    materials    efficient    hydrocarbons    relationships    clean    sustainable    function    doped    direction    denox    mild    portable    mofs    urea    capacity    transport    industry    functional    environment    pi    binding    molecular    synthesis    captured    metal    reactivity    loaded    scr    selective    characterisation    compounds    experiments    hybrid    medium    spectroscopic    nh3    nanopores    gas    computational    space    substrates    energy    energetic    nanoporous    relevance    n2o    fundamental    framework    mitigation    release    storage    emphasis    reactor    structure    static   

Project "NANOCHEM" data sheet

The following table provides information about the project.

Coordinator
THE UNIVERSITY OF MANCHESTER 

Organization address
address: OXFORD ROAD
city: MANCHESTER
postcode: M13 9PL
website: www.manchester.ac.uk

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country United Kingdom [UK]
 Total cost 2˙498˙645 €
 EC max contribution 2˙498˙645 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2016-ADG
 Funding Scheme ERC-ADG
 Starting year 2017
 Duration (year-month-day) from 2017-06-01   to  2022-05-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    THE UNIVERSITY OF MANCHESTER UK (MANCHESTER) coordinator 2˙498˙645.00

Map

 Project objective

We will study the adsorption, binding, transport and reactivity of N-containing substrates within the nanopores of functionalized and doped metal-organic framework (MOF) materials. A range of important target molecules (e.g., NH3, N2H4, N2O, NO, NO2 and N2O4) will be studied in this project, which aims to re-define the molecular chemistry for these energetic N-compounds in confined space, and to develop selective catalytic reduction (SCR) of NOx in the presence of NH3, urea and hydrocarbons. The PI has extensive experience in the field of coordination chemistry and hybrid materials, and seeks to change research direction to develop new gas phase catalysts and to gain fundamental understanding of molecular interactions, properties and function of specific energy, environmentally-related substrates within MOFs. Research objectives include the: • Design and synthesis of new porous MOFs with emphasis on the decoration of their pore environment and improvement of their structural stability and function; • Characterisation of host and substrate-loaded materials by state-of-the-art in situ structural, dynamic and spectroscopic methods for the construction of structure-function relationships, supported by computational analysis and modelling; • Adsorption, binding, release and separation of NH3, N2H4, N2O, NO, NO2 and N2O4 via both static and dynamic experiments; • Tests of degradation and selective catalytic reduction (SCR) of captured NOx molecules with NH3, urea and hydrocarbons under mild conditions using nanoporous MOFs as host catalysts; • Assembly of a MOF-based (i) catalytic deNOx reactor and (ii) NH3 storage system for potential portable applications. This project will deliver new functional materials as high capacity portable NH3 stores, efficient capture medium for NOx, and new catalysts for reduction and mitigation of NOx to deliver significant impacts to academia, industry and society of direct relevance to clean energy and sustainable environment.

 Publications

year authors and title journal last update
List of publications.
2019 Xinran Zhang, Ivan da Silva, Rodrigo Fazzi, Alena M. Sheveleva, Xue Han, Ben F. Spencer, Sergey A. Sapchenko, Floriana Tuna, Eric J. L. McInnes, Ming Li, Sihai Yang, Martin Schröder
Iodine Adsorption in a Redox-Active Metal–Organic Framework: Electrical Conductivity Induced by Host−Guest Charge-Transfer
published pages: 14145-14150, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.9b02176
Inorganic Chemistry 58/20 2020-01-29
2019 Jiangnan Li, Xue Han, Xinran Zhang, Alena M. Sheveleva, Yongqiang Cheng, Floriana Tuna, Eric J. L. McInnes, Laura J. McCormick McPherson, Simon J. Teat, Luke L. Daemen, Anibal J. Ramirez-Cuesta, Martin Schröder, Sihai Yang
Capture of nitrogen dioxide and conversion to nitric acid in a porous metal–organic framework
published pages: 1085-1090, ISSN: 1755-4330, DOI: 10.1038/s41557-019-0356-0
Nature Chemistry 11/12 2020-01-29
2019 Xinchen Kang, Kai Lyu, Lili Li, Jiangnan Li, Louis Kimberley, Bin Wang, Lifei Liu, Yongqiang Cheng, Mark D. Frogley, Svemir Rudić, Anibal J. Ramirez-Cuesta, Robert A. W. Dryfe, Buxing Han, Sihai Yang, Martin Schröder
Integration of mesopores and crystal defects in metal-organic frameworks via templated electrosynthesis
published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-019-12268-5
Nature Communications 10/1 2020-01-29
2019 Gemma L. Smith, Jennifer E. Eyley, Xue Han, Xinran Zhang, Jiangnan Li, Nicholas M. Jacques, Harry G. W. Godfrey, Stephen P. Argent, Laura J. McCormick McPherson, Simon J. Teat, Yongqiang Cheng, Mark D. Frogley, Gianfelice Cinque, Sarah J. Day, Chiu C. Tang, Timothy L. Easun, Svemir Rudić, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder
Reversible coordinative binding and separation of sulfur dioxide in a robust metal–organic framework with open copper sites
published pages: 1358-1365, ISSN: 1476-1122, DOI: 10.1038/s41563-019-0495-0
Nature Materials 18/12 2020-01-29
2019 Leo J. Small, Ryan C. Hill, James L. Krumhansl, Mara E. Schindelholz, Zhihengyu Chen, Karena W. Chapman, Xinran Zhang, Sihai Yang, Martin Schröder, Tina M. Nenoff
Reversible MOF-Based Sensors for the Electrical Detection of Iodine Gas
published pages: 27982-27988, ISSN: 1944-8244, DOI: 10.1021/acsami.9b09938
ACS Applied Materials & Interfaces 11/31 2020-01-29
2019 Harry G. W. Godfrey, Lydia Briggs, Xue Han, William J. F. Trenholme, Christopher G. Morris, Mathew Savage, Louis Kimberley, Oxana V. Magdysyuk, Michael Drakopoulos, Claire A. Murray, Chiu C. Tang, Mark D. Frogley, Gianfelice Cinque, Sihai Yang, Martin Schröder
Analysis by synchrotron X-ray scattering of the kinetics of formation of an Fe-based metal-organic framework with high CO 2 adsorption
published pages: 111104, ISSN: 2166-532X, DOI: 10.1063/1.5121644
APL Materials 7/11 2020-01-29
2019 Sergey A. Sapchenko, Marina O. Barsukova, Rodion V. Belosludov, Konstantin A. Kovalenko, Denis G. Samsonenko, Artem S. Poryvaev, Alena M. Sheveleva, Matvey V. Fedin, Artem S. Bogomyakov, Danil N. Dybtsev, Martin Schröder, Vladimir P. Fedin
Understanding Hysteresis in Carbon Dioxide Sorption in Porous Metal–Organic Frameworks
published pages: 6811-6820, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.9b00016
Inorganic Chemistry 58/10 2020-01-29
2019 Xue Han, Sihai Yang, Martin Schröder
Porous metal–organic frameworks as emerging sorbents for clean air
published pages: 108-118, ISSN: 2397-3358, DOI: 10.1038/s41570-019-0073-7
Nature Reviews Chemistry 3/2 2020-01-29
2018 Zhenzhong Lu, Harry G. W. Godfrey, Ivan da Silva, Yongqiang Cheng, Mathew Savage, Pascal Manuel, Svemir Rudić, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder
Direct observation of supramolecular binding of light hydrocarbons in vanadium( iii ) and ( iv ) metal–organic framework materials
published pages: 3401-3408, ISSN: 2041-6520, DOI: 10.1039/c8sc00330k
Chemical Science 9/13 2019-02-28
2017 Vladimir V. Korolkov, Ivan G. Timokhin, Rolf Haubrichs, Emily F. Smith, Lixu Yang, Sihai Yang, Neil R. Champness, Martin Schröder, Peter H. Beton
Supramolecular networks stabilise and functionalise black phosphorus
published pages: , ISSN: 2041-1723, DOI: 10.1038/s41467-017-01797-6
Nature Communications 8/1 2019-02-28
2018 Thien D. Duong, Sergey A. Sapchenko, Ivan da Silva, Harry G. W. Godfrey, Yongqiang Cheng, Luke L. Daemen, Pascal Manuel, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder
Optimal Binding of Acetylene to a Nitro-Decorated Metal–Organic Framework
published pages: 16006-16009, ISSN: 0002-7863, DOI: 10.1021/jacs.8b08504
Journal of the American Chemical Society 140/47 2019-02-28
2017 Adam D. Martin, Timothy L. Easun, Stephen P. Argent, William Lewis, Alexander J. Blake, Martin Schröder
The effect of carboxylate position on the structure of a metal organic framework derived from cyclotriveratrylene
published pages: 603-607, ISSN: 1466-8033, DOI: 10.1039/c6ce01965j
CrystEngComm 19/4 2019-02-28
2018 Nicholas M. Jacques, Peter R. E. Rought, Detlev Fritsch, Mathew Savage, Harry G. W. Godfrey, Lei Li, Tamoghna Mitra, Mark D. Frogley, Gianfelice Cinque, Sihai Yang, Martin Schröder
Locating the binding domains in a highly selective mixed matrix membrane via synchrotron IR microspectroscopy
published pages: 2866-2869, ISSN: 1359-7345, DOI: 10.1039/c7cc08932e
Chemical Communications 54/23 2019-02-28
2018 Tamoghna Mitra, Florian Moreau, Adam Nevin, Carlo U. Perotto, Alex Summerfield, E. Stephen Davies, Elizabeth A. Gibson, Timothy L. Easun, Martin Schröder
Characterisation of redox states of metal–organic frameworks by growth on modified thin-film electrodes
published pages: 6572-6579, ISSN: 2041-6520, DOI: 10.1039/c8sc00803e
Chemical Science 9/31 2019-02-28
2017 Marina S. Zavakhina, Irina V. Yushina, Denis G. Samsonenko, Danil N. Dybtsev, Vladimir P. Fedin, Stephen P. Argent, Alexander J. Blake, Martin Schröder
Halochromic coordination polymers based on a triarylmethane dye for reversible detection of acids
published pages: 465-470, ISSN: 1477-9226, DOI: 10.1039/c6dt03969c
Dalton Transactions 46/2 2019-02-20
2018 Yong Yan, Alice E. O’Connor, Gopikkaa Kanthasamy, George Atkinson, David R. Allan, Alexander J. Blake, Martin Schröder
Unusual and Tunable Negative Linear Compressibility in the Metal–Organic Framework MFM-133(M) (M = Zr, Hf)
published pages: 3952-3958, ISSN: 0002-7863, DOI: 10.1021/jacs.7b11747
Journal of the American Chemical Society 140/11 2019-02-28
2017 Yong Yan, Daniil I. Kolokolov, Ivan da Silva, Alexander G. Stepanov, Alexander J. Blake, Anne Dailly, Pascal Manuel, Chiu C. Tang, Sihai Yang, Martin Schröder
Porous Metal–Organic Polyhedral Frameworks with Optimal Molecular Dynamics and Pore Geometry for Methane Storage
published pages: 13349-13360, ISSN: 0002-7863, DOI: 10.1021/jacs.7b05453
Journal of the American Chemical Society 139/38 2019-02-28
2017 Aleksandr A. Sapianik, Ekaterina N. Zorina-Tikhonova, Mikhail A. Kiskin, Denis G. Samsonenko, Konstantin A. Kovalenko, Alexey A. Sidorov, Igor L. Eremenko, Danil N. Dybtsev, Alexander J. Blake, Stephen P. Argent, Martin Schröder, Vladimir P. Fedin
Rational Synthesis and Investigation of Porous Metal–Organic Framework Materials from a Preorganized Heterometallic Carboxylate Building Block
published pages: 1599-1608, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.6b02713
Inorganic Chemistry 56/3 2019-02-28
2019 Peter Rought, Christopher Marsh, Simona Pili, Ian P. Silverwood, Victoria García Sakai, Ming Li, Martyn S. Brown, Stephen P. Argent, Inigo Vitorica-Yrezabal, George Whitehead, Mark R. Warren, Sihai Yang, Martin Schröder
Modulating proton diffusion and conductivity in metal–organic frameworks by incorporation of accessible free carboxylic acid groups
published pages: , ISSN: 2041-6520, DOI: 10.1039/c8sc03022g
Chemical Science 2019-02-28
2018 Jian Lü, Cristina Perez-Krap, Fabien Trousselet, Yong Yan, Nada H. Alsmail, Bahar Karadeniz, Nicholas M. Jacques, William Lewis, Alexander J. Blake, François-Xavier Coudert, Rong Cao, Martin Schröder
Polycatenated 2D Hydrogen-Bonded Binary Supramolecular Organic Frameworks (SOFs) with Enhanced Gas Adsorption and Selectivity
published pages: 2555-2562, ISSN: 1528-7483, DOI: 10.1021/acs.cgd.8b00153
Crystal Growth & Design 18/4 2019-02-20
2017 Timothy L. Easun, Florian Moreau, Yong Yan, Sihai Yang, Martin Schröder
Structural and dynamic studies of substrate binding in porous metal–organic frameworks
published pages: 239-274, ISSN: 0306-0012, DOI: 10.1039/c6cs00603e
Chemical Society Reviews 46/1 2019-02-28
2018 Vsevolod A. Bolotov, Konstantin A. Kovalenko, Denis G. Samsonenko, Xue Han, Xinran Zhang, Gemma L. Smith, Laura J. MCormick, Simon J. Teat, Sihai Yang, Matthew J. Lennox, Alice Henley, Elena Besley, Vladimir P. Fedin, Danil N. Dybtsev, Martin Schröder
Enhancement of CO 2 Uptake and Selectivity in a Metal–Organic Framework by the Incorporation of Thiophene Functionality
published pages: 5074-5082, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.8b00138
Inorganic Chemistry 57/9 2019-02-28
2017 Andrea Laybourn, Juliano Katrib, Rebecca S. Ferrari-John, Christopher G. Morris, Sihai Yang, Ofonime Udoudo, Timothy L. Easun, Chris Dodds, Neil R. Champness, Samuel W. Kingman, Martin Schröder
Metal–organic frameworks in seconds via selective microwave heating
published pages: 7333-7338, ISSN: 2050-7488, DOI: 10.1039/c7ta01493g
Journal of Materials Chemistry A 5/16 2019-02-28
2018 Joseph H. Carter, Xue Han, Florian Y. Moreau, Ivan da Silva, Adam Nevin, Harry G. W. Godfrey, Chiu C. Tang, Sihai Yang, Martin Schröder
Exceptional Adsorption and Binding of Sulfur Dioxide in a Robust Zirconium-Based Metal–Organic Framework
published pages: 15564-15567, ISSN: 0002-7863, DOI: 10.1021/jacs.8b08433
Journal of the American Chemical Society 140/46 2019-02-28
2017 Sergey A. Sapchenko, Pavel A. Demakov, Denis G. Samsonenko, Danil N. Dybtsev, Martin Schröder, Vladimir P. Fedin
A Cryptand Metal-Organic Framework as a Platform for the Selective Uptake and Detection of Group I Metal Cations
published pages: 2286-2289, ISSN: 0947-6539, DOI: 10.1002/chem.201605895
Chemistry - A European Journal 23/10 2019-02-28
2017 Xinran Zhang, Ivan da Silva, Harry G. W. Godfrey, Samantha K. Callear, Sergey A. Sapchenko, Yongqiang Cheng, Inigo Vitórica-Yrezábal, Mark D. Frogley, Gianfelice Cinque, Chiu C. Tang, Carlotta Giacobbe, Catherine Dejoie, Svemir Rudić, Anibal J. Ramirez-Cuesta, Melissa A. Denecke, Sihai Yang, Martin Schröder
Confinement of Iodine Molecules into Triple-Helical Chains within Robust Metal–Organic Frameworks
published pages: 16289-16296, ISSN: 0002-7863, DOI: 10.1021/jacs.7b08748
Journal of the American Chemical Society 139/45 2019-02-28
2017 Iñigo J. Vitórica-Yrezábal, Daniel Florin Sava, Grigore A. Timco, Martyn S. Brown, Mathew Savage, Harry G. W. Godfrey, Florian Moreau, Martin Schröder, Flor Siperstein, Lee Brammer, Sihai Yang, Martin P. Attfield, Joseph J. W. McDouall, Richard E. P. Winpenny
Binding CO 2 by a Cr 8 Metallacrown
published pages: 5527-5530, ISSN: 1433-7851, DOI: 10.1002/anie.201701726
Angewandte Chemie International Edition 56/20 2019-02-28
2018 Harry G. W. Godfrey, Ivan da Silva, Lydia Briggs, Joseph H. Carter, Christopher G. Morris, Mathew Savage, Timothy L. Easun, Pascal Manuel, Claire A. Murray, Chiu C. Tang, Mark D. Frogley, Gianfelice Cinque, Sihai Yang, Martin Schröder
Ammonia Storage by Reversible Host-Guest Site Exchange in a Robust Metal-Organic Framework
published pages: 14778-14781, ISSN: 1433-7851, DOI: 10.1002/anie.201808316
Angewandte Chemie International Edition 57/45 2019-02-28
2019 Lei Li, Ivan da Silva, Daniil I. Kolokolov, Xue Han, Jiangnan Li, Gemma Smith, Yongqiang Cheng, Luke L. Daemen, Christopher G. Morris, Harry G. W. Godfrey, Nicholas M. Jacques, Xinran Zhang, Pascal Manuel, Mark D. Frogley, Claire A. Murray, Anibal J. Ramirez-Cuesta, Gianfelice Cinque, Chiu C. Tang, Alexander G. Stepanov, Sihai Yang, Martin Schroder
Post-synthetic modulation of the charge distribution in a metal–organic framework for optimal binding of carbon dioxide and sulfur dioxide
published pages: , ISSN: 2041-6520, DOI: 10.1039/c8sc01959b
Chemical Science 2019-02-28
2019 Jack D. Humby, Oguarabau Benson, Gemma L. Smith, Stephen P. Argent, Ivan da Silva, Yongqiang Cheng, Svemir Rudić, Pascal Manuel, Mark D. Frogley, Gianfelice Cinque, Lucy K. Saunders, Iñigo J. Vitórica-Yrezábal, George F. S. Whitehead, Timothy L. Easun, William Lewis, Alexander J. Blake, Anibal J. Ramirez-Cuesta, Sihai Yang, Martin Schröder
Host–guest selectivity in a series of isoreticular metal–organic frameworks: observation of acetylene-to-alkyne and carbon dioxide-to-amide interactions
published pages: 1098-1106, ISSN: 2041-6520, DOI: 10.1039/c8sc03622e
Chemical Science 10/4 2019-02-28
2016 Jamie A. Gould, Harprit Singh Athwal, Alexander J. Blake, William Lewis, Peter Hubberstey, Neil R. Champness, Martin Schröder
Gas adsorption and structural diversity in a family of Cu(II) pyridyl-isophthalate metal–organic framework materials
published pages: 20160334, ISSN: 1364-503X, DOI: 10.1098/rsta.2016.0334
Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences 375/2084 2019-02-28
2017 Christopher G. Morris, Nicholas M. Jacques, Harry G. W. Godfrey, Tamoghna Mitra, Detlev Fritsch, Zhenzhong Lu, Claire A. Murray, Jonathan Potter, Tom M. Cobb, Fajin Yuan, Chiu C. Tang, Sihai Yang, Martin Schröder
Stepwise observation and quantification and mixed matrix membrane separation of CO 2 within a hydroxy-decorated porous host
published pages: 3239-3248, ISSN: 2041-6520, DOI: 10.1039/c6sc04343g
Chemical Science 8/4 2019-02-20
2018 Xue Han, Harry G. W. Godfrey, Lydia Briggs, Andrew J. Davies, Yongqiang Cheng, Luke L. Daemen, Alena M. Sheveleva, Floriana Tuna, Eric J. L. McInnes, Junliang Sun, Christina Drathen, Michael W. George, Anibal J. Ramirez-Cuesta, K. Mark Thomas, Sihai Yang, Martin Schröder
Reversible adsorption of nitrogen dioxide within a robust porous metal–organic framework
published pages: 691-696, ISSN: 1476-1122, DOI: 10.1038/s41563-018-0104-7
Nature Materials 17/8 2019-02-20

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