Explore the words cloud of the SOLWET project. It provides you a very rough idea of what is the project "SOLWET" about.
The following table provides information about the project.
MAX-PLANCK-GESELLSCHAFT ZUR FORDERUNG DER WISSENSCHAFTEN EV
|Coordinator Country||Germany [DE]|
|Total cost||2˙250˙000 €|
|EC max contribution||2˙250˙000 € (100%)|
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
|Duration (year-month-day)||from 2018-08-01 to 2023-07-31|
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|1||MAX-PLANCK-GESELLSCHAFT ZUR FORDERUNG DER WISSENSCHAFTEN EV||DE (MUENCHEN)||coordinator||2˙250˙000.00|
Building fuel cells, electrolyzers or photoelectrochemical cells based on water (photo)electrolysis is extremely challenging. One origin of this challenge is the complexity of the underlying physical chemistry. Most such devices require transfer of electrons between solid(s) and water and thus building the best possible devices requires understanding the link between transient changes in bulk solid electronic structure, interfacial electronic structure and interfacial chemistry. Essentially all existing approaches address only part of this picture: e.g. they only probe electronic structure (optical absorption), or extracted current or provide elemental insight but are insensitive to the presence of hydrogen (x-ray absorption).
In SOLWET, I will address this gap using interface-specific optical spectroscopies, in the visible and infrared, to probe interfacial electronic and vibrational transitions and their coupling. By combining these probes with an additional intense laser pulse I will watch (photo)electrolysis of water in real time as it happens. In particular, I will directly probe the coupling of transiently perturbed solid electronic structure to interfacial electronic structure and watch how this perturbation drives water’s oxidation, for a hematite photoanode, or reduction, for a Pt cathode, through the interfacial vibrational response. By describing how these couplings change with solid modification (e.g. an alumina overlayer on hematite) or changes in aqueous solution composition (e.g. changing the pH in contact with Pt) the results of SOLWET will offer the physical insights necessary to build the best possible hematite and Pt containing photoelectrochemical devices. Moreover, because the novel all-optical tools developed in SOLWET are not system-specific, the approach demonstrated in this work will be widely applicable.
|year||authors and title||journal||last update|
Igor Ying Zhang, Gregor Zwaschka, Zhenhua Wang, Martin Wolf, R. Kramer Campen, Yujin Tong
Resolving the chemical identity of H 2 SO 4 derived anions on Pt(111) electrodes: they\'re sulfate
published pages: 19147-19152, ISSN: 1463-9076, DOI: 10.1039/c9cp03397a
|Physical Chemistry Chemical Physics 21/35||2020-04-03|
Tobias Garling, R. Kramer Campen, Martin Wolf, Martin ThÃ¤mer
A General Approach To Combine the Advantages of Collinear and Noncollinear Spectrometer Designs in Phase-Resolved Second-Order Nonlinear Spectroscopy
published pages: 11022-11030, ISSN: 1089-5639, DOI: 10.1021/acs.jpca.9b09927
|The Journal of Physical Chemistry A 123/51||2020-04-03|
G. Zwaschka, Y. Tong, M. Wolf, R. Kramerâ€…Campen
Probing the Hydrogen Evolution Reaction and Charge Transfer on Platinum Electrodes on Femtosecond Timescales
published pages: 2675-2682, ISSN: 2196-0216, DOI: 10.1002/celc.201900336
Riko Kiessling, Yujin Tong, Alexander J. Giles, Sandy Gewinner, Wieland SchÃ¶llkopf, Joshua D. Caldwell, Martin Wolf, Alexander Paarmann
Surface Phonon Polariton Resonance Imaging Using Long-Wave Infrared-Visible Sum-Frequency Generation Microscopy
published pages: 3017-3023, ISSN: 2330-4022, DOI: 10.1021/acsphotonics.9b01335
|ACS Photonics 6/11||2020-04-03|
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The information about "SOLWET" are provided by the European Opendata Portal: CORDIS opendata.
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