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DEFNET SIGNED

DEFect NETwork materials science and engineering

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EC-Contrib. €

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Project "DEFNET" data sheet

The following table provides information about the project.

Coordinator
RUHR-UNIVERSITAET BOCHUM 

Organization address
address: UNIVERSITAETSSTRASSE 150
city: BOCHUM
postcode: 44801
website: www.rub.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Project website http://www.defnet-etn.eu
 Total cost 3˙804˙639 €
 EC max contribution 3˙804˙639 € (100%)
 Programme 1. H2020-EU.1.3.1. (Fostering new skills by means of excellent initial training of researchers)
 Code Call H2020-MSCA-ITN-2014
 Funding Scheme MSCA-ITN-ETN
 Starting year 2015
 Duration (year-month-day) from 2015-01-01   to  2018-12-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    RUHR-UNIVERSITAET BOCHUM DE (BOCHUM) coordinator 498˙432.00
2    KATHOLIEKE UNIVERSITEIT LEUVEN BE (LEUVEN) participant 751˙680.00
3    CENTRE NATIONAL DE LA RECHERCHE SCIENTIFIQUE CNRS FR (PARIS) participant 525˙751.00
4    AGENCIA ESTATAL CONSEJO SUPERIOR DEINVESTIGACIONES CIENTIFICAS ES (MADRID) participant 495˙745.00
5    THE CHANCELLOR, MASTERS AND SCHOLARS OF THE UNIVERSITY OF OXFORD UK (OXFORD) participant 273˙287.00
6    SOFTWARE FOR CHEMISTRY & MATERIALS BV NL (AMSTERDAM) participant 255˙374.00
7    UNIVERSITEIT UTRECHT NL (UTRECHT) participant 255˙374.00
8    UNIVERSITEIT GENT BE (GENT) participant 250˙560.00
9    TECHNISCHE UNIVERSITAET BERGAKADEMIE FREIBERG DE (FREIBERG) participant 249˙216.00
10    TECHNISCHE UNIVERSITAET MUENCHEN DE (MUENCHEN) participant 249˙216.00
11    RUBOTHERM GMBH DE (BOCHUM) participant 0.00
12    British American Tobacco UK (London) partner 0.00
13    CLARIANT PRODUKTE (DEUTSCHLAND) GMBH DE (FRANKFURT AM MAIN) partner 0.00
14    COMPANIA ESPANOLA DE PETROLEOS SA ES (MADRID) partner 0.00
15    DIAMOND LIGHT SOURCE LIMITED UK (DIDCOT) partner 0.00
16    Evonik Industries AG DE (ESSEN) partner 0.00
17    LINDE AG DE (MUNCHEN) partner 0.00
18    SOLVAY SA BE (BRUXELLES) partner 0.00

Map

 Project objective

Porous coordination network materials, also known as Metal-organic Frameworks (MOFs), are at the cutting edge of molecular materials science. DEFNET, “DEFect NETwork materials science and engineering”, is the first European Training Network (ETN) at the intersection of chemistry, physics and engineering aimed at structural and functional complexity of MOFs. It provides a unique interdisciplinary training platform for early stage researchers and combines the expertise of the academic and the non-academic sector for fundamental development and industrial application and technology transfer aspects. The research and the training program in materials synthesis, characterization, computational modelling and application is accomplished in a coordinated effort involving 8 academic and 8 industrial partners from 6 European countries. DEFNET will particularly investigate defects, disorder and correlated phenomena in MOFs and related materials. The understanding and the intentional modification of defect structures of porous coordination networks is essential for advanced controlling their properties in catalysis, gas capture and separation beyond existing materials limitations. Benchmarking will be done against selected zeolite materials, which are very well established for large scale industrial applications. It is anticipated that superior functionalities of defect engineered MOFs will be identified which cannot be achieved by employing other porous materials.

 Deliverables

List of deliverables.
Scientific Publications in Peer reviewed journals Websites, patent fillings, videos etc. 2019-07-22 08:26:49
Scientific Presentations at Int. conferences (oral + poster) Websites, patent fillings, videos etc. 2019-07-22 08:26:54
ESR led activities: Networking and Doctoral Symposium Documents, reports 2019-07-22 08:26:49
DEFNET Kick-off and web page launching activities Documents, reports 2019-07-10 14:57:36
Supervisory Board of the network Other 2019-07-10 14:57:36

Take a look to the deliverables list in detail:  detailed list of DEFNET deliverables.

 Publications

year authors and title journal last update
List of publications.
2018 Chiara Caratelli, Julianna Hajek, Sven M. J. Rogge, Steven Vandenbrande, Evert Jan Meijer, Michel Waroquier, Veronique Van Speybroeck
Influence of a Confined Methanol Solvent on the Reactivity of Active Sites in UiO-66
published pages: 420-429, ISSN: 1439-4235, DOI: 10.1002/cphc.201701109
ChemPhysChem 19/4 2019-07-10
2018 Stefano Dissegna, Pia Vervoorts, Claire L. Hobday, Tina Düren, Dominik Daisenberger, Andrew J. Smith, Roland A. Fischer, Gregor Kieslich
Tuning the Mechanical Response of Metal–Organic Frameworks by Defect Engineering
published pages: 11581-11584, ISSN: 0002-7863, DOI: 10.1021/jacs.8b07098
Journal of the American Chemical Society 140/37 2019-07-10
2018 Haowei Huang, Haifeng Yuan, Kris P. F. Janssen, Guillermo Solís-Fernández, Ying Wang, Collin Y. X. Tan, Dries Jonckheere, Elke Debroye, Jinlin Long, Jelle Hendrix, Johan Hofkens, Julian A. Steele, Maarten B. J. Roeffaers
Efficient and Selective Photocatalytic Oxidation of Benzylic Alcohols with Hybrid Organic–Inorganic Perovskite Materials
published pages: 755-759, ISSN: 2380-8195, DOI: 10.1021/acsenergylett.8b00131
ACS Energy Letters 3/4 2019-07-10
2018 Carlos Marquez, Francisco G. Cirujano, Cédric Van Goethem, Ivo Vankelecom, Dirk De Vos, Trees De Baerdemaeker
Tunable Prussian blue analogues for the selective synthesis of propargylamines through A 3 coupling
published pages: 2061-2065, ISSN: 2044-4753, DOI: 10.1039/c8cy00073e
Catalysis Science & Technology 8/8 2019-07-10
2018 Penghu Guo, Christian Froese, Qi Fu, Yen-Ting Chen, Baoxiang Peng, Wolfgang Kleist, Roland A. Fischer, Martin Muhler, Yuemin Wang
CuPd Mixed-Metal HKUST-1 as a Catalyst for Aerobic Alcohol Oxidation
published pages: 21433-21440, ISSN: 1932-7447, DOI: 10.1021/acs.jpcc.8b05882
The Journal of Physical Chemistry C 122/37 2019-07-10
2017 Bart Bueken, Niels Van Velthoven, Andraž Krajnc, Simon Smolders, Francis Taulelle, Caroline Mellot-Draznieks, Gregor Mali, Thomas D. Bennett, Dirk De Vos
Tackling the Defect Conundrum in UiO-66: A Mixed-Linker Approach to Engineering Missing Linker Defects
published pages: 10478-10486, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.7b04128
Chemistry of Materials 29/24 2019-07-10
2019 Paul Iacomi, U-Hwang Lee, Anil H. Valekar, Jong-San Chang, Philip L. Llewellyn
Investigating the effect of alumina shaping on the sorption properties of promising metal–organic frameworks
published pages: 7128-7135, ISSN: 2046-2069, DOI: 10.1039/c9ra00534j
RSC Advances 9/13 2019-07-10
2018 H.-H. Mautschke, F. Drache, I. Senkovska, S. Kaskel, F. X. Llabrés i Xamena
Catalytic properties of pristine and defect-engineered Zr-MOF-808 metal organic frameworks
published pages: 3610-3616, ISSN: 2044-4753, DOI: 10.1039/c8cy00742j
Catalysis Science & Technology 8/14 2019-07-10
2016 Wenhua Zhang, Zhihao Chen, Majd Al-Naji, Penghu Guo, Stefan Cwik, Olesia Halbherr, Yuemin Wang, Martin Muhler, Nicole Wilde, Roger Gläser, Roland A. Fischer
Simultaneous introduction of various palladium active sites into MOF via one-pot synthesis: Pd@[Cu 3−x Pd x (BTC) 2 ] n
published pages: 14883-14887, ISSN: 1477-9226, DOI: 10.1039/c6dt02893d
Dalton Transactions 45/38 2019-07-10
2018 Chen-Xia Liu, Wen-Hua Zhang, Nan Wang, Penghu Guo, Martin Muhler, Yuemin Wang, Shiru Lin, Zhongfang Chen, Guang Yang
Highly Efficient Photocatalytic Degradation of Dyes by a Copper-Triazolate Metal-Organic Framework
published pages: 16804-16813, ISSN: 0947-6539, DOI: 10.1002/chem.201803306
Chemistry - A European Journal 24/63 2019-07-10
2018 Adam F. Sapnik, Harry S. Geddes, Emily M. Reynolds, Hamish H.-M. Yeung, Andrew L. Goodwin
Compositional inhomogeneity and tuneable thermal expansion in mixed-metal ZIF-8 analogues
published pages: 9651-9654, ISSN: 1359-7345, DOI: 10.1039/c8cc04172e
Chemical Communications 54/69 2019-07-10
2018 Miguel Rivera‐Torrente, Matthias Filez, Rifan Hardian, Emily Reynolds, Beatriz Seoane, Marie‐Vanessa Coulet, Freddy E. Oropeza Palacio, Jan P. Hofmann, Roland A. Fischer, Andrew L. Goodwin, Philip L. Llewellyn, Bert M. Weckhuysen
Metal‐Organic Frameworks as Catalyst Supports: Influence of Lattice Disorder on Metal Nanoparticle Formation
published pages: 7498-7506, ISSN: 0947-6539, DOI: 10.1002/chem.201800694
Chemistry – A European Journal 24/29 2019-07-10
2019 Miguel Rivera-Torrente, Paul D. Pletcher, Maarten K. Jongkind, Nikolaos Nikolopoulos, Bert M. Weckhuysen
Ethylene Polymerization over Metal–Organic Framework Crystallites and the Influence of Linkers on Their Fracturing Process
published pages: 3059-3069, ISSN: 2155-5435, DOI: 10.1021/acscatal.9b00150
ACS Catalysis 9/4 2019-07-10
2018 Simon Krause, Jack D. Evans, Volodymyr Bon, Irena Senkovska, Sebastian Ehrling, Ulrich Stoeck, Pascal G. Yot, Paul Iacomi, Philip Llewellyn, Guillaume Maurin, François-Xavier Coudert, Stefan Kaskel
Adsorption Contraction Mechanics: Understanding Breathing Energetics in Isoreticular Metal–Organic Frameworks
published pages: 19171-19179, ISSN: 1932-7447, DOI: 10.1021/acs.jpcc.8b04549
The Journal of Physical Chemistry C 122/33 2019-07-10
2018 Franziska Drache, Francisco G. Cirujano, Khoa D. Nguyen, Volodymyr Bon, Irena Senkovska, Francesc X. Llabrés i Xamena, Stefan Kaskel
Anion Exchange and Catalytic Functionalization of the Zirconium-Based Metal–Organic Framework DUT-67
published pages: 5492-5500, ISSN: 1528-7483, DOI: 10.1021/acs.cgd.8b00832
Crystal Growth & Design 18/9 2019-07-10
2015 Ignacio Luz, Christoph Rösler, Konstantin Epp, Francesc X. Llabrés i Xamena, Roland A. Fischer
Pd@UiO-66-Type MOFs Prepared by Chemical Vapor Infiltration as Shape-Selective Hydrogenation Catalysts
published pages: 3904-3912, ISSN: 1434-1948, DOI: 10.1002/ejic.201500299
European Journal of Inorganic Chemistry 2015/23 2019-07-10
2018 Chiara Caratelli, Julianna Hajek, Sven M. J. Rogge, Steven Vandenbrande, Evert Jan Meijer, Michel Waroquier, Veronique Van Speybroeck
Influence of a Confined Methanol Solvent on the Reactivity of Active Sites in UiO-66
published pages: 420-429, ISSN: 1439-4235, DOI: 10.1002/cphc.201701109
ChemPhysChem 19/4 2019-07-10
2019 Joao Marreiros, Chiara Caratelli, Julianna Hajek, Andraž Krajnc, Guillaume Fleury, Bart Bueken, Dirk E. De Vos, Gregor Mali, Maarten B. J. Roeffaers, Veronique Van Speybroeck, Rob Ameloot
Active Role of Methanol in Post-Synthetic Linker Exchange in the Metal–Organic Framework UiO-66
published pages: 1359-1369, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.8b04734
Chemistry of Materials 31/4 2019-07-10
2018 A.F. Sapnik, X. Liu, H.L.B. Boström, C.S. Coates, A.R. Overy, E.M. Reynolds, A. Tkatchenko, A.L. Goodwin
Uniaxial negative thermal expansion and metallophilicity in Cu3[Co(CN)6]
published pages: 298-306, ISSN: 0022-4596, DOI: 10.1016/j.jssc.2017.10.009
Journal of Solid State Chemistry 258 2019-07-10
2016 Sven M. J. Rogge, Jelle Wieme, Louis Vanduyfhuys, Steven Vandenbrande, Guillaume Maurin, Toon Verstraelen, Michel Waroquier, Veronique Van Speybroeck
Thermodynamic Insight in the High-Pressure Behavior of UiO-66: Effect of Linker Defects and Linker Expansion
published pages: 5721-5732, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.6b01956
Chemistry of Materials 28/16 2019-07-10
2016 Eva Plessers, Guangxia Fu, Collin Tan, Dirk De Vos, Maarten Roeffaers
Zr-Based MOF-808 as Meerwein–Ponndorf–Verley Reduction Catalyst for Challenging Carbonyl Compounds
published pages: 104, ISSN: 2073-4344, DOI: 10.3390/catal6070104
Catalysts 6/7 2019-07-10
2016 Víctor L. Rechac, Francisco G. Cirujano, Avelino Corma, Francesc X. Llabrés i Xamena
Diastereoselective Synthesis of Pyranoquinolines on Zirconium-Containing UiO-66 Metal-Organic Frameworks
published pages: 4512-4516, ISSN: 1434-1948, DOI: 10.1002/ejic.201600372
European Journal of Inorganic Chemistry 2016/27 2019-07-10
2016 Sarah A. Hodgson, Sarah J. Hunt, Thomas Just Sørensen, Amber L. Thompson, Emily M. Reynolds, Stephen Faulkner, Andrew L. Goodwin
Anomalous Thermal Expansion and Luminescence Thermochromism in Silver(I) Dicyanamide
published pages: 4378-4381, ISSN: 1434-1948, DOI: 10.1002/ejic.201600246
European Journal of Inorganic Chemistry 2016/27 2019-07-10
2016 Alistair R. Overy, Andrew B. Cairns, Matthew J. Cliffe, Arkadiy Simonov, Matthew G. Tucker, Andrew L. Goodwin
Design of crystal-like aperiodic solids with selective disorder–phonon coupling
published pages: 10445, ISSN: 2041-1723, DOI: 10.1038/ncomms10445
Nature Communications 7 2019-07-10
2016 Nicole L. Evans, Peter M. M. Thygesen, Hanna L. B. Boström, Emily M. Reynolds, Ines E. Collings, Anthony E. Phillips, Andrew L. Goodwin
Control of Multipolar and Orbital Order in Perovskite-like [C(NH 2 ) 3 ]Cu x Cd 1– x (HCOO) 3 Metal–Organic Frameworks
published pages: 9393-9396, ISSN: 0002-7863, DOI: 10.1021/jacs.6b05208
Journal of the American Chemical Society 138/30 2019-07-10
2017 Arthur De Vos, Kevin Hendrickx, Pascal Van Der Voort, Veronique Van Speybroeck, Kurt Lejaeghere
Missing Linkers: An Alternative Pathway to UiO-66 Electronic Structure Engineering
published pages: 3006-3019, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.6b05444
Chemistry of Materials 29/7 2019-07-10
2017 Chiara Caratelli, Julianna Hajek, Francisco G. Cirujano, Michel Waroquier, Francesc X. Llabrés i Xamena, Veronique Van Speybroeck
Nature of active sites on UiO-66 and beneficial influence of water in the catalysis of Fischer esterification
published pages: 401-414, ISSN: 0021-9517, DOI: 10.1016/j.jcat.2017.06.014
Journal of Catalysis 352 2019-07-10
2017 Julianna Hajek, Bart Bueken, Michel Waroquier, Dirk De Vos, Veronique Van Speybroeck
The Remarkable Amphoteric Nature of Defective UiO-66 in Catalytic Reactions
published pages: 2203-2210, ISSN: 1867-3880, DOI: 10.1002/cctc.201601689
ChemCatChem 9/12 2019-07-10
2016 Wenhua Zhang, Max Kauer, Olesia Halbherr, Konstantin Epp, Penghu Guo, Miguel I. Gonzalez, Dianne J. Xiao, Christian Wiktor, Francesc X. LIabrés i Xamena, Christof Wöll, Yuemin Wang, Martin Muhler, Roland A. Fischer
Ruthenium Metal-Organic Frameworks with Different Defect Types: Influence on Porosity, Sorption, and Catalytic Properties
published pages: 14297-14307, ISSN: 0947-6539, DOI: 10.1002/chem.201602641
Chemistry - A European Journal 22/40 2019-07-10
2018 Stefano Dissegna, Konstantin Epp, Werner R. Heinz, Gregor Kieslich, Roland A. Fischer
Defective Metal-Organic Frameworks
published pages: 1704501, ISSN: 0935-9648, DOI: 10.1002/adma.201704501
Advanced Materials 2019-07-10
2017 S. M. J. Rogge, A. Bavykina, J. Hajek, H. Garcia, A. I. Olivos-Suarez, A. Sepúlveda-Escribano, A. Vimont, G. Clet, P. Bazin, F. Kapteijn, M. Daturi, E. V. Ramos-Fernandez, F. X. Llabrés i Xamena, V. Van Speybroeck, J. Gascon
Metal–organic and covalent organic frameworks as single-site catalysts
published pages: 3134-3184, ISSN: 0306-0012, DOI: 10.1039/C7CS00033B
Chemical Society Reviews 46/11 2019-07-10
2017 Stefano Dissegna, Rifan Hardian, Konstantin Epp, Gregor Kieslich, Marie-Vanessa Coulet, Philip Llewellyn, Roland A. Fischer
Using water adsorption measurements to access the chemistry of defects in the metal–organic framework UiO-66
published pages: 4137-4141, ISSN: 1466-8033, DOI: 10.1039/c7ce00224f
CrystEngComm 19/29 2019-07-10
2017 Christoph Rösler, Stefano Dissegna, Victor L. Rechac, Max Kauer, Penghu Guo, Stuart Turner, Kevin Ollegott, Hirokazu Kobayashi, Tomokazu Yamamoto, Daniel Peeters, Yuemin Wang, Syo Matsumura, Gustaaf Van Tendeloo, Hiroshi Kitagawa, Martin Muhler, Francesc X. Llabrés i Xamena, Roland A. Fischer
Encapsulation of Bimetallic Metal Nanoparticles into Robust Zirconium-Based Metal-Organic Frameworks: Evaluation of the Catalytic Potential for Size-Selective Hydrogenation
published pages: 3583-3594, ISSN: 0947-6539, DOI: 10.1002/chem.201603984
Chemistry - A European Journal 23/15 2019-07-10
2017 A. V. Bavykina, H.-H. Mautscke, M. Makkee, F. Kapteijn, J. Gascon, F. X. Llabrés i Xamena
Base free transfer hydrogenation using a covalent triazine framework based catalyst
published pages: 4166-4170, ISSN: 1466-8033, DOI: 10.1039/c7ce00561j
CrystEngComm 19/29 2019-07-10
2018 Julianna Hajek, Chiara Caratelli, Ruben Demuynck, Kristof De Wispelaere, Louis Vanduyfhuys, Michel Waroquier, Veronique Van Speybroeck
On the intrinsic dynamic nature of the rigid UiO-66 metal–organic framework
published pages: 2723-2732, ISSN: 2041-6520, DOI: 10.1039/c7sc04947a
Chemical Science 9/10 2019-07-10

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