Opendata, web and dolomites

TRANSFORMERS

Creating transformation-stable microstructures through shared crystallographic motifs

Total Cost €

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EC-Contrib. €

0

Partnership

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 TRANSFORMERS project word cloud

Explore the words cloud of the TRANSFORMERS project. It provides you a very rough idea of what is the project "TRANSFORMERS" about.

alternative    decays    looping    fuel    immediately    microstructure    renewable    3d    power    removed    sequestration    prone    material    solid    regenerate    cheap    supports    microstructures    conductors    oldest    caco3    absorption    metal    structures    purpose    prepare    abundant    mechanically    capacity    scientific    later    chemical    techniques    stability    ion    release    cells    flue    undesirable    materials    reacts    stage    tomography    phases    atomic    transition    limestone    transformations    co2    retain    starting    bonding    sorption    micro    suffer    crystal    emissions    battery    solution    capture    time    fossil    similarities    gas    plants    degradation    ray    electrodes    chemically    catalyst    cycling    porosity    oxide    sources    ternary    repeated    pure    place    situ    industrial    designed    evolution    decrease    stable    spectroscopic    performance    ceramics    mechanical    continue    networks    visualization    space    while    thermal   

Project "TRANSFORMERS" data sheet

The following table provides information about the project.

Coordinator
THE CHANCELLOR MASTERS AND SCHOLARSOF THE UNIVERSITY OF CAMBRIDGE 

Organization address
address: TRINITY LANE THE OLD SCHOOLS
city: CAMBRIDGE
postcode: CB2 1TN
website: www.cam.ac.uk

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country United Kingdom [UK]
 Project website http://www.michaelgaultois.com/co2_looping.html
 Total cost 183˙454 €
 EC max contribution 183˙454 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2014
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2015
 Duration (year-month-day) from 2015-05-01   to  2017-04-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    THE CHANCELLOR MASTERS AND SCHOLARSOF THE UNIVERSITY OF CAMBRIDGE UK (CAMBRIDGE) coordinator 183˙454.00

Map

 Project objective

While we continue to develop alternative and renewable power sources, the capture and sequestration of CO2 from flue gas in fossil fuel power plants and other industrial processes is one viable solution to decrease our CO2 emissions. CO2 can be removed from flue gas by chemical looping, where a material chemically reacts with CO2 and is treated at a later stage to release pure CO2 and regenerate the starting material. Limestone, CaCO3, is the oldest material to be used for this purpose. However, although limestone is abundant and cheap, the CO2 absorption capacity rapidly decays with use because of undesirable changes to the microstructure. The proposed work will prepare and investigate novel ternary metal oxide ceramics designed to be mechanically stable after repeated thermal and CO2 cycling. In particular, the proposed work will determine whether similarities in the crystal structures of materials (the atomic scale) before and after a transition will lead to robust microstructures (the micro scale) that will retain functionality – in this case, high porosity and CO2 sorption capacity. The complex crystal structures, rich phase space, and strong bonding networks available in ternary phases to be studied will lead to materials that are less prone to degradation. This evolution will be studied at the atomic level using in situ spectroscopic techniques, and the microstructure evolution will be studied using novel in situ X-ray tomography methods, which allow the 3D visualization of the microstructure in real time as the chemical transformations take place. These new approaches to material design will be immediately relevant to many other scientific fields where chemical transformations and mechanical stability are important, such as battery electrodes, solid oxide fuel cells, solid ion conductors, and catalyst supports, all of which suffer from performance loss over time due to microstructure changes.

 Publications

year authors and title journal last update
List of publications.
2016 Anton O. Oliynyk, Erin Antono, Taylor D. Sparks, Leila Ghadbeigi, Michael W. Gaultois, Bryce Meredig, Arthur Mar
High-Throughput Machine-Learning-Driven Synthesis of Full-Heusler Compounds
published pages: 7324-7331, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.6b02724
Chemistry of Materials 28/20 2019-07-24
2016 Anton O. Oliynyk, Taylor D. Sparks, Michael W. Gaultois, Leila Ghadbeigi, Arthur Mar
Gd 12 Co 5.3 Bi and Gd 12 Co 5 Bi, Crystalline Doppelgänger with Low Thermal Conductivities
published pages: 6625-6633, ISSN: 0020-1669, DOI: 10.1021/acs.inorgchem.6b00826
Inorganic Chemistry 55/13 2019-07-24
2016 Matthew T. Dunstan, Serena A. Maugeri, Wen Liu, Matthew G. Tucker, Oluwadamilola O. Taiwo, Belen Gonzalez, Phoebe K. Allan, Michael W. Gaultois, Paul R. Shearing, David A. Keen, Anthony E. Phillips, Martin T. Dove, Stuart A. Scott, John S. Dennis, Clare P. Grey
In situ studies of materials for high temperature CO 2 capture and storage
published pages: 217-240, ISSN: 1359-6640, DOI: 10.1039/C6FD00047A
Faraday Discuss. 192 2019-07-24
2016 Michael W. Gaultois, Anton O. Oliynyk, Arthur Mar, Taylor D. Sparks, Gregory J. Mulholland, Bryce Meredig
Perspective: Web-based machine learning models for real-time screening of thermoelectric materials properties
published pages: 53213, ISSN: 2166-532X, DOI: 10.1063/1.4952607
APL Materials 4/5 2019-07-24
2017 Matthew J. Cliffe, Elizabeth Castillo-Martínez, Yue Wu, Jeongjae Lee, Alexander C. Forse, Francesca C. N. Firth, Peyman Z. Moghadam, David Fairen-Jimenez, Michael W. Gaultois, Joshua A. Hill, Oxana V. Magdysyuk, Ben Slater, Andrew L. Goodwin, Clare P. Grey
Metal–Organic Nanosheets Formed via Defect-Mediated Transformation of a Hafnium Metal–Organic Framework
published pages: 5397-5404, ISSN: 0002-7863, DOI: 10.1021/jacs.7b00106
Journal of the American Chemical Society 139/15 2019-07-24
2017 Wei Meng, Roberta Pigliapochi, Paul M. Bayley, Oliver Pecher, Michael W. Gaultois, Ieuan D. Seymour, Han-Pu Liang, Wenqian Xu, Kamila M. Wiaderek, Karena W. Chapman, Clare P. Grey
Unraveling the Complex Delithiation and Lithiation Mechanisms of the High Capacity Cathode Material V 6 O 13
published pages: 5513-5524, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.7b00428
Chemistry of Materials 29/13 2019-07-24

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