PICOPROP SIGNED
Photo Induced Collective Properties of Hybrid Halide Perovskites
Total Cost €
0EC-Contrib. €
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Project "PICOPROP" data sheet
The following table provides information about the project.
| Coordinator |
ECOLE POLYTECHNIQUE FEDERALE DE LAUSANNE
Organization address contact info |
| Coordinator Country | Switzerland [CH] |
| Total cost | 2˙495˙712 € |
| EC max contribution | 2˙495˙712 € (100%) |
| Programme |
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC)) |
| Code Call | ERC-2014-ADG |
| Funding Scheme | ERC-ADG |
| Starting year | 2015 |
| Duration (year-month-day) | from 2015-09-01 to 2020-08-31 |
Partnership
Take a look of project's partnership.
| # | ||||
|---|---|---|---|---|
| 1 | ECOLE POLYTECHNIQUE FEDERALE DE LAUSANNE | CH (LAUSANNE) | coordinator | 2˙495˙712.00 |
Map
Project objective
The recent discovery of the organo-inorganic perovskite CH3NH3PbI3 as very efficient material in photoelectric conversion is multifaceted: it turns out that this compound is promising not only in photovoltaics, but it is lasing, it gives bright light emitting diodes, promising in water splitting and we are persuaded that it can play an important role in basic sciences, as well. We have recently realized that under white light illumination the photoelectrons, due to their very long recombination time, stay in the conduction band and the resistivity of a single crystal shows a metallic behavior. If the lifetime is sufficiently long and the density of these excited carrier is high enough they could condense into a Fermi sea. The project’s goal is to realize this highly unusual state and to document its properties by magneto-transport and spectroscopic techniques. We will check in our model compound the long-sought superconductivity of photo-excited carriers, extensively searched for in cuprates, if we could stabilize it by fine tuning the interactions by hydrostatic pressure under constant illumination. The availability of high quality samples is primordial for this program. It turns out that CH3NH3PbI3 is ideal compound, it seems to be almost free of charged defects (its room temperature resistance is 5 orders of magnitude higher than that of Phosphorus doped Silicon at 1013 cm-3 doping concentration) and we can grow excellent single crystals of it. Furthermore, it has a flexibility in material design: one can vary all the constituents, and even the dimensionality by making layered materials with the main chemical motifs. A special effort will be devoted to tune the spin-orbit coupling by different elements, since this could be at the origin of the long recombination time of the photo-electrons. We suspect that the highly tunable, clean and disorder-free doping obtained by shining light on these ionic crystals opens a new era in material discovery.
Publications
| year | authors and title | journal | last update |
|---|---|---|---|
| 2016 |
Alla Arakcheeva, Dmitry Chernyshov, Massimo Spina, László Forró, Endre Horváth CH 3 NH 3 PbI 3 : precise structural consequences of water absorption at ambient conditions published pages: 716-722, ISSN: 2052-5206, DOI: 10.1107/S2052520616010428 |
Acta Crystallographica Section B Structural Science, Crystal Engineering and Materials 72/5 | 2019-04-18 |
| 2018 |
Anastasiia Glushkova, Alla Arakcheeva, Philip Pattison, Márton Kollár, Pavao AndriÄević, Bálint Náfrádi, László Forró, Endre Horváth Influence of the organic cation disorder on photoconductivity in ethylenediammonium lead iodide, NH 3 CH 2 CH 2 NH 3 PbI 4 published pages: 3543-3549, ISSN: 1466-8033, DOI: 10.1039/C8CE00259B |
CrystEngComm 20/25 | 2019-04-18 |
| 2017 |
Márton Kollár, Luka Ćirić, J. Hugo Dil, Andrew Weber, Stefan Muff, Henrik M. Ronnow, Bálint Náfrádi, Benjamin Pierre Monnier, Jeremy Scott Luterbacher, László Forró, Endre Horváth Clean, cleaved surfaces of the photovoltaic perovskite published pages: , ISSN: 2045-2322, DOI: 10.1038/s41598-017-00799-0 |
Scientific Reports 7/1 | 2019-04-18 |
| 2016 |
Iness R. Benmessaoud, Anne-Laure Mahul-Mellier, Endre Horváth, Bohumil Maco, Massimo Spina, Hilal A. Lashuel, Là szló Forró Health hazards of methylammonium lead iodide based perovskites: cytotoxicity studies published pages: 407-419, ISSN: 2045-452X, DOI: 10.1039/C5TX00303B |
Toxicology Research 5/2 | 2019-04-18 |
| 2016 |
Massimo Spina, Claudio Grimaldi, Bálint Náfrádi, László Forró, Endre Horváth Rapid thickness reading of CH 3 NH 3 PbI 3 nanowire thin films from color maps published pages: 2017-2023, ISSN: 1862-6300, DOI: 10.1002/pssa.201533067 |
physica status solidi (a) 213/8 | 2019-04-18 |
| 2018 |
L. Ćirić, K. Ashby, T. Abadie, M. Spina, M. Duchamp, B. Náfrádi, M. Kollár, L. Forró, E. Horváth Mechanical response of CH 3 NH 3 PbI 3 nanowires published pages: 111901, ISSN: 0003-6951, DOI: 10.1063/1.5023115 |
Applied Physics Letters 112/11 | 2019-04-18 |
| 2017 |
Massimo Spina, Ayat Karimi, Wanda Andreoni, Carlo A. Pignedoli, Bálint Náfrádi, László Forró, Endre Horváth Mechanical signatures of degradation of the photovoltaic perovskite CH 3 NH 3 PbI 3 upon water vapor exposure published pages: 121903, ISSN: 0003-6951, DOI: 10.1063/1.4978687 |
Applied Physics Letters 110/12 | 2019-04-18 |
| 2018 |
Konstantins Mantulnikovs, Anastasiia Glushkova, Péter Matus, Luka Ćirić, Márton Kollár, László Forró, Endre Horváth, Andrzej Sienkiewicz Morphology and Photoluminescence of CH 3 NH 3 PbI 3 Deposits on Nonplanar, Strongly Curved Substrates published pages: 1476-1485, ISSN: 2330-4022, DOI: 10.1021/acsphotonics.7b01496 |
ACS Photonics 5/4 | 2019-04-18 |
| 2016 |
Alla Arakcheeva, Dmitry Chernyshov, Massimo Spina, László Forró, Endre Horváth Organic-inorganic hybrid perovskite CH 3 NH 3 PbI 3 : structural consequences of water absorption published pages: s294-s295, ISSN: 2053-2733, DOI: 10.1107/S2053273316095577 |
Acta Crystallographica Section A Foundations and Advances 72/a1 | 2019-04-18 |
| 2017 |
Pavao AndriÄević, Márton Kollár, Xavier Mettan, Bálint Náfrádi, Andrzej Sienkiewicz, Dóra Fejes, Klára Hernádi, László Forró, Endre Horváth Three-Dimensionally Enlarged Photoelectrodes by a Protogenetic Inclusion of Vertically Aligned Carbon Nanotubes into CH 3 NH 3 PbBr 3 Single Crystals published pages: 13549-13556, ISSN: 1932-7447, DOI: 10.1021/acs.jpcc.7b03421 |
The Journal of Physical Chemistry C 121/25 | 2019-04-18 |
| 2017 |
Massimo Spina, László Mihály, Károly Holczer, Bálint Náfrádi, Andrea Pisoni, László Forró, Endre Horváth Photodiode Response in a CH 3 NH 3 PbI 3 /CH 3 NH 3 SnI 3 Heterojunction published pages: 10198-10202, ISSN: 1944-8244, DOI: 10.1021/acsami.6b12392 |
ACS Applied Materials & Interfaces 9/11 | 2019-04-18 |
| 2017 |
Alla Arakcheeva, Volodymyr Svitlyk, Márton Kollár, Bálint Náfrádi, László Forró, Endre Horváth High-pressure transformation of MAPbI 3 : role of the noble-gas medium published pages: C1416-C1416, ISSN: 2053-2733, DOI: 10.1107/S2053273317081608 |
Acta Crystallographica Section A Foundations and Advances 73/a2 | 2019-04-18 |
| 2017 |
Hajnalka M. Tóháti, Ãron Pekker, Pavao AndriÄević, László Forró, Bálint Náfrádi, Márton Kollár, Endre Horváth, Katalin Kamarás Optical detection of charge dynamics in CH 3 NH 3 PbI 3 /carbon nanotube composites published pages: 17781-17787, ISSN: 2040-3364, DOI: 10.1039/C7NR06136F |
Nanoscale 9/45 | 2019-04-18 |
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