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Opendata, web and dolomites

NanoSiAl

Silica and alumina nanophases – the building blocks for the ground under our feet.

Total Cost €

EC-Contrib. €

Partnership

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Outcomes and
results

NanoSiAl project word cloud

Explore the words cloud of the NanoSiAl project. It provides you a very rough idea of what is the project "NanoSiAl" about.

lt climate varying complemented direct methodology solution mechanistic resolution combination electron life hard aluminosilicates earth utilising microscopy specifying habitable types occurrence characterisation synchrotron global usual blocks nanosial building regard silica aqueous scattering liquid interface colloid form quantitative points dissolved nano play complete techniques insights nucleate reactions destruction solid near interactions weathering situ condensation assembly colloidal rock atomic water cell nanophases artefacts underlying picture containing si sized validate tem time nm hydrolysis grow nanoparticles unprecedented indication al lacking alumina kinetic phases original species transmission molecular undergo geological length structural controls insufficient objects vacuum

Project "NanoSiAl" data sheet

The following table provides information about the project.

Coordinator	HELMHOLTZ ZENTRUM POTSDAM DEUTSCHESGEOFORSCHUNGSZENTRUM GFZ Organization address address: TELEGRAFENBERG 17 city: POTSDAM postcode: 14473 website: www.gfz-potsdam.de contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.
Coordinator Country	Germany [DE]
Project website	https://github.com/tomaszstawski/SilicaLysozymeSAXS
Total cost	171˙460 €
EC max contribution	171˙460 € (100%)
Programme	1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
Code Call	H2020-MSCA-IF-2015
Funding Scheme	MSCA-IF-EF-ST
Starting year	2017
Duration (year-month-day)	from 2017-05-01 to 2019-10-30

Partnership

Take a look of project's partnership.

#	participants	country	role	EC contrib. [€]
1	HELMHOLTZ ZENTRUM POTSDAM DEUTSCHESGEOFORSCHUNGSZENTRUM GFZ HELMHOLTZ ZENTRUM POTSDAM DEUTSCHESGEOFORSCHUNGSZENTRUM GFZ Organization address address: TELEGRAFENBERG 17 city: POTSDAM postcode: 14473 website: www.gfz-potsdam.de contact info title: n.a. name: n.a. surname: n.a. function: n.a. email: n.a. telephone: n.a. fax: n.a.	DE (POTSDAM)	coordinator	171˙460.00

Map

Project objective

Alumina and silica nanophases play a crucial role in rock weathering and their formation and destruction controls Earth’s response to global climate change. The presence of various products of aqueous weathering of aluminosilicates points to a complex activity of water, and is considered as the geological indication for the occurrence of life-habitable conditions. In this regard, a more complete picture of the water-alumina-silica interactions would allow for better specifying the molecular-level conditions for early life. Upon weathering the original Al- and Si-containing phases are dissolved at the solid-water interface, undergo hydrolysis and condensation reactions and form new colloidal nanoparticles. However, quantitative and mechanistic understanding of the underlying processes that lead to the formation and types of Al and Si phases is still lacking, due to the insufficient in situ methodology providing structural information about the colloidal species in solution.

Therefore, the main objective of the NanoSiAl project is to develop, test and validate the methods for the direct in situ and real-time structural and kinetic characterisation of the alumina and silica colloid formation pathways at the length-scale of < 100 nm. I will achieve this by utilising state-of-the-art in situ liquid-cell transmission electron microscopy (L-C TEM) complemented with synchrotron-based scattering methods. This way I will be able to fully avoid the usual artefacts of sample varying and hard-vacuum conditions, because the L-C TEM and scattering methods allow for direct in situ characterisation of nano-sized objects in solution with a near-atomic-resolution. This combination of novel techniques will provide unprecedented insights on properties of the molecular building blocks for alumina and silica as they nucleate, grow and assembly with each other.

Publications

List of publications.
year	authors and title	journal	last update
2019	Tomasz M. Stawski, Helen M. Freeman, Alexander E. S. Van Driessche, JÃ¶rn HÃ¶velmann, Rogier Besselink, Richard Wirth, Liane G. Benning Particle-Mediated Nucleation Pathways Are Imprinted in the Internal Structure of Calcium Sulfate Single Crystals published pages: 3714-3721, ISSN: 1528-7483, DOI: 10.1021/acs.cgd.9b00066	Crystal Growth & Design 19/7	2020-03-20
2017	Mercedes Ossorio, Tomasz Stawski, Juan RodrÃguez-Blanco, Mike Sleutel, Juan GarcÃa-Ruiz, Liane Benning, Alexander Van Driessche Physicochemical and Additive Controls on the Multistep Precipitation Pathway of Gypsum published pages: 140, ISSN: 2075-163X, DOI: 10.3390/min7080140	Minerals 7/8	2020-03-20
2019	JÃ¶rn HÃ¶velmann, Tomasz M. Stawski, Rogier Besselink, Helen M. Freeman, Karen M. Dietmann, Sathish Mayanna, Brian R. Pauw, Liane G. Benning A template-free and low temperature method for the synthesis of mesoporous magnesium phosphate with uniform pore structure and high surface area published pages: 6939-6951, ISSN: 2040-3364, DOI: 10.1039/c8nr09205b	Nanoscale 11/14	2020-03-20
2018	Adriana Matamoros-Veloza, Tomasz M. Stawski, Liane G. Benning Nanoparticle Assembly Leads to Mackinawite Formation published pages: 6757-6764, ISSN: 1528-7483, DOI: 10.1021/acs.cgd.8b01025	Crystal Growth & Design 18/11	2020-03-20
2018	Daniela B. van den Heuvel, Tomasz M. Stawski, Dominique J. Tobler, Richard Wirth, Caroline L. Peacock, Liane G. Benning Formation of Silica-Lysozyme Composites Through Co-Precipitation and Adsorption published pages: , ISSN: 2296-8016, DOI: 10.3389/fmats.2018.00019	Frontiers in Materials 5	2020-03-20
2017	R. Besselink, J. D. Rodriguez-Blanco, T. M. Stawski, L. G. Benning, D. J. Tobler How Short-Lived Ikaite Affects Calcite Crystallization published pages: 6224-6230, ISSN: 1528-7483, DOI: 10.1021/acs.cgd.7b00743	Crystal Growth & Design 17/12	2020-03-20
2019	Tomasz M. Stawski, Alexander E. S. Van Driessche, Rogier Besselink, Emily H. Byrne, Paolo Raiteri, Julian D. Gale, Liane G. Benning The Structure of CaSO 4 Nanorods: The Precursor of Gypsum published pages: 23151-23158, ISSN: 1932-7447, DOI: 10.1021/acs.jpcc.9b04268	The Journal of Physical Chemistry C 123/37	2020-03-20
2019	A.E.S. Van Driessche, T.M. Stawski, M. Kellermeier Calcium sulfate precipitation pathways in natural and engineering environments published pages: 119274, ISSN: 0009-2541, DOI: 10.1016/j.chemgeo.2019.119274	Chemical Geology	2020-03-20
2019	JÃ¶rn HÃ¶velmann, Tomasz M. Stawski, Helen M. Freeman, Rogier Besselink, Sathish Mayanna, Jeffrey Paulo H. Perez, Nicole S. Hondow, Liane G. Benning Struvite Crystallisation and the Effect of Co2+ Ions published pages: 503, ISSN: 2075-163X, DOI: 10.3390/min9090503	Minerals 9/9	2020-03-20
2019	Tomasz M Stawski, Daniela B van den Heuvel, Rogier Besselink, Dominique J Tobler, Liane G Benning Mechanism of silicaâ€“lysozyme composite formation unravelled by in situ fast SAXS published pages: 182-197, ISSN: 2190-4286, DOI: 10.3762/bjnano.10.17	Beilstein Journal of Nanotechnology 10	2020-03-20
2018	Daniela B. van den Heuvel, Einar Gunnlaugsson, Ingvi Gunnarsson, Tomasz M. Stawski, Caroline L. Peacock, Liane G. Benning Understanding amorphous silica scaling under well-constrained conditions inside geothermal pipelines published pages: 231-241, ISSN: 0375-6505, DOI: 10.1016/j.geothermics.2018.07.006	Geothermics 76	2020-03-20
2018	Tomasz M. Stawski, Teresa Roncal-Herrero, Alejandro Fernandez-Martinez, Adriana Matamoros-Veloza, Roland KrÃ¶ger, Liane G. Benning â€œOn demandâ€ triggered crystallization of CaCO 3 from solute precursor species stabilized by the water-in-oil microemulsion published pages: 13825-13835, ISSN: 1463-9076, DOI: 10.1039/C8CP00540K	Physical Chemistry Chemical Physics 20/20	2020-03-20

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