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TUCAS SIGNED

Tuneable Catalyst Surfaces for Heterogeneous Catalysis – Electrochemical Switching of Selectivity and Activity

Total Cost €

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EC-Contrib. €

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Partnership

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 TUCAS project word cloud

Explore the words cloud of the TUCAS project. It provides you a very rough idea of what is the project "TUCAS" about.

dopants    oxide    offers    stimulation    emerge    polarisation    catalysis    nanoparticle    reversibly    structure    incorporate    group    renewable    ground    uniformly    time    tried    possibilities    ageing    leads    modify    21st    conversion    reaction    catalytic    signal    combination    co2    exsolution    tackle    active    excellent    dopant    selectivity    solutions    tuneable    versatility    opportunity    coking    external    tackling    dispersed    sintering    nanoparticles    improvement    guest    materials    modification    realistic    voltage    chemistry    fundamental    continuous    lattice    electrochemistry    environment    heterogeneous    catalysts    fuel    form    tune    opens    situ    selectively    efficient    unprecedented    breaking    deactivation    requirement    surfaces    adjust    perovskite    possibility    performance    electrochemical    catalytically    surface    decorated    correlation    science    consequence    mechanistic    direct    century    multidisciplinary    clusters    particles    utilisation    enhancement    catalyst    preparation   

Project "TUCAS" data sheet

The following table provides information about the project.

Coordinator
TECHNISCHE UNIVERSITAET WIEN 

Organization address
address: KARLSPLATZ 13
city: WIEN
postcode: 1040
website: www.tuwien.ac.at

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Austria [AT]
 Total cost 1˙997˙202 €
 EC max contribution 1˙997˙202 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2017-STG
 Funding Scheme ERC-STG
 Starting year 2018
 Duration (year-month-day) from 2018-01-01   to  2022-12-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    TECHNISCHE UNIVERSITAET WIEN AT (WIEN) coordinator 1˙997˙202.00

Map

 Project objective

In heterogeneous catalysis surfaces decorated with uniformly dispersed, catalytically highly active particles are a key requirement for excellent performance. One of the main tasks in catalysis research is the continuous improvement or development of catalytically active materials.

An emerging concept in catalyst design, and the aim of this project, is to selectively and reversibly tune and modify the surface chemistry by electrochemical polarisation. Perovskite-type catalysts raise the opportunity to incorporate guest elements as dopants. Upon electrochemical polarisation these dopants emerge from the oxide lattice to form catalytically active clusters or nanoparticles on the surface (by exsolution). In consequence this leads to a strong modification or enhancement of catalytic selectivity and activity. Electrochemical polarisation offers the possibility to adjust the surface chemistry in response to an external signal (here the applied voltage).

Studies in a realistic catalytic reaction environment (in-situ) will enable a direct correlation of surface structure with catalytic activity, selectivity and the electrochemical stimulation. The unique combination of surface science, heterogeneous catalysis and electrochemistry will take this research to a new ground-breaking level. No research group has yet tried to tackle this topic on a fundamental mechanistic level by this multidisciplinary approach.

The proposed project opens unprecedented possibilities for catalyst design and in-situ control due to the versatility of perovskite-type catalyst materials and dopant elements. Nanoparticle exsolution is a highly time- and cost-efficient way of catalyst preparation and it will offer solutions to major problems in heterogeneous catalysis, such as ageing (sintering) or catalyst deactivation (coking). Tuneable catalyst surfaces will facilitate tackling a major concern of the 21st century, the utilisation of CO2 and its conversion to renewable fuel.

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The information about "TUCAS" are provided by the European Opendata Portal: CORDIS opendata.

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