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IL-E-CAT SIGNED

Enhancing electrocatalysis in low temperature fuel cells by ionic liquid modification

Total Cost €

0

EC-Contrib. €

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Partnership

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 IL-E-CAT project word cloud

Explore the words cloud of the IL-E-CAT project. It provides you a very rough idea of what is the project "IL-E-CAT" about.

remarkable    tuning    exploration    leaching    suitable    site    intense    stabilization    strategy    scientific    modification    engineering    herein    structure    preliminary    catalysts    durability    fundamental    efforts    particle    situ    structures    ils    synthesis    active    electrocatalytic    time    excellent    immobilized    stop    carbon    applicability    demonstrated    cell    ionic    fixed    electrochemical    surrounding    demanding    ligand    manner    interplay    sites    materials    performance    electrostatic    solutions    sieving    solvent    pore    temperature    core    layer    stability    liquid    co2    il    infrastructure    enhanced    local    interaction    pt    ions    principals    devoted    longstanding    sound    fuel    activation    assisted    cells    synthesized    apparently    model    influences    innovative    molecular    microenvironment    mesoporous    restricted    cathode    optimization    rational    versatility    shell    deduced    structural    tackle    issue    commercialization    steric    dramatically    employed    full    realization    orr    catalyst    catalytic   

Project "IL-E-CAT" data sheet

The following table provides information about the project.

Coordinator
TECHNISCHE UNIVERSITAT DARMSTADT 

Organization address
address: KAROLINENPLATZ 5
city: DARMSTADT
postcode: 64289
website: www.tu-darmstadt.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Total cost 1˙999˙465 €
 EC max contribution 1˙999˙465 € (100%)
 Programme 1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC))
 Code Call ERC-2015-CoG
 Funding Scheme ERC-COG
 Starting year 2016
 Duration (year-month-day) from 2016-05-01   to  2021-04-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    TECHNISCHE UNIVERSITAT DARMSTADT DE (DARMSTADT) coordinator 1˙999˙465.00

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 Project objective

The commercialization of low temperature fuel cells is restricted by the high cost and low durability of cathode catalysts. Intense efforts have been devoted to tackle this issue by engineering the structure of Pt-based catalysts. Herein, a novel concept towards enhancing the performance of low temperature fuel cell catalysts is proposed, namely by tuning the local active site microenvironment with an immobilized ionic liquid (IL) phase. As demonstrated by the applicant in preliminary work, a suitable IL layer strongly influences the active catalytic site in a very promising manner, apparently via a highly complex interplay of solvent-, ligand- and electrostatic-stabilization effects. As the structural versatility of ILs allows for rational engineering of this modification at molecular level, the proposed project aims for a full scientific exploration of the remarkable activation and stabilization effects in ORR, to enable the realization of an innovative fuel cell cathode with dramatically enhanced performance. To achieve this ambitious goal, a sound fundamental understanding of the interaction of ILs with electrocatalytic sites will be derived by making use of the excellent research infrastructure and longstanding experience in ionic liquid design and catalytic materials at our institute. To demonstrate the general applicability, the deduced principals will also be applied to CO2 electrochemical reduction. The approach will not stop at the design of novel catalyst systems, but will address solutions to ensure long-term stability of the IL modification. To avoid IL leaching from the catalyst over time, the recent success of the applicant in the synthesis of novel core/shell carbon materials will be employed. The IL will be synthesized in situ within a mesoporous core and the steric demanding ions fixed through a molecular sieving shell surrounding each catalyst particle. A model-assisted strategy will be applied for optimization of the core/shell pore structures.

 Publications

year authors and title journal last update
List of publications.
2016 Zhang, Gui-Rong; Munoz, Macarena; Etzold, Bastian JM
Engineering Ionic Liquid Modification for Pt/C Oxygen Reduction Catalysts
published pages: , ISSN: , DOI: 10.5281/zenodo.1065388
2019-06-18
2016 Zhang, Gui-Rong; Munoz, Macarena; Etzold, Bastian JM
Accelerating Oxygen Reduction Catalysts through Preventing Poisoning with Non-Reactive Species by Using Hydrophobic Ionic Liquids
published pages: , ISSN: , DOI: 10.5281/zenodo.1065378
2019-06-18
2017 Wolker, Thomas; Zhang, Gui-Rong; Etzold, Bastian JM
Improving performance of electrocatalysts by ionic liquid modifications
published pages: , ISSN: , DOI: 10.5281/zenodo.1065392
\"1st German-Chinese-Symposium \"\"Development and Technology of Carbon Materials\"\"\" 2019-06-18
2016 Zhang, Gui-Rong; Munoz, Macarena; Etzold, Bastian JM
Boosting Performance of Carbon Supported Pt Catalysts for Fuel Cell Catalysis through Ionic Liquid Modifications
published pages: , ISSN: , DOI: 10.5281/zenodo.1065398
2019-06-18
2017 Gui-Rong Zhang; Munoz, Macarena; Etzold, Bastian JM
Accelerating Oxygen Reduction Catalysts through Preventing Poisoning with Non-Reactive Species by Using Hydrophobic Ionic Liquids
published pages: , ISSN: , DOI: 10.5281/zenodo.1065440
Green Solvent Conference 2017 2019-06-18
2017 Liu-Liu Shen, Gui-Rong Zhang, Wei Li, Markus Biesalski, Bastian J. M. Etzold
Modifier-Free Microfluidic Electrochemical Sensor for Heavy-Metal Detection
published pages: 4593-4603, ISSN: 2470-1343, DOI: 10.1021/acsomega.7b00611
ACS Omega 2/8 2019-06-18
2017 Ariyanto, Teguh; Zeiger, Marco; Zhang, Gui-Rong; Presser, Volker; Etzold, Bastian JM
Core-shell carbide-derived carbons as platform for high-performance electrochemical energy storage and electrocatalysis
published pages: , ISSN: , DOI: 10.5281/zenodo.1065417
2019-06-18
2017 Wolker, Thomas; Zhang, Gui-Rong; Erini, Nina; Kramm, Ulrike I; Etzold, Bastian JM
Improving Electrocatalytic Performance of Noble-Metal-Free Catalysts by Ionic Liquid Modification T. Wolker, G.-R. Zhang, N. Erini, U. Kramm, B.J.M. Etzold*
published pages: , ISSN: , DOI: 10.5281/zenodo.1065442
2019-06-18
2017 Zhang, Gui-Rong; Munoz, Macarena; Jeschonek, Katharina; Etzold, Bastian JM
Boosting Oxygen Reduction Catalysts through Preventing Active Sites Poisoning by Using Hydrophobic Ionic Liquids
published pages: , ISSN: , DOI: 10.5281/zenodo.1065407
2019-06-18
2017 Shen, Liu-Liu; Zhang, Gui-Rong; Etzold, Bastian JM
Modifier-Free Microfluidic Electrochemical Sensor for Heavy Metal Detection
published pages: , ISSN: , DOI: 10.5281/zenodo.1065433
2019-06-18
2016 Etzold, Bastian JM
Carbon Based Catalysts
published pages: , ISSN: , DOI: 10.5281/zenodo.1116315
Novel Aspects in Petrochemistry and Refining 1 2019-06-18
2017 Zhang, Gui-Rong; Kramm, Ulrike I; Etzold, Bastian JM
Improving ORR Catalysts by Ionic Liquid Modifications
published pages: , ISSN: , DOI: 10.5281/zenodo.1065429
\"1st German-Chinese-Symposium \"\"Development and Technology of Carbon Materials\"\"\" 2019-06-18
2017 George, Michael; Zhang, Gui-Rong; Munoz, Macarena; Etzold, Bastian JM
Accelerating Oxygen Reduction Catalysts through Preventing Poisoning with Non-Reactive Species by Using Hydrophobic Ionic Liquids
published pages: , ISSN: , DOI: 10.5281/zenodo.1065415
2019-06-18
2016 Zhang, Gui-Rong; Munoz, Macarena; Etzold, Bastian JM
Accelerating Oxygen Reduction Catalysts for Fuel Cell Applications through Ionic Liquid Modification
published pages: , ISSN: , DOI: 10.5281/zenodo.1065386
2019-06-18
2019 Liu-Liu Shen, Gui-Rong Zhang, Tizian Venter, Markus Biesalski, Bastian J.M. Etzold
Towards best practices for improving paper-based microfluidic fuel cells
published pages: 389-399, ISSN: 0013-4686, DOI: 10.1016/j.electacta.2018.12.077
Electrochimica Acta 298 2019-06-07
2018 Zhang, Gui-Rong; Wolker, Thomas; Sandbeck, Daniel; Munoz, Macarena; Mayrhofer, Karl; Etzold, Bastian JM
Tuning performance of Pt/C catalysts toward ORR by ionic liquid modifications
published pages: , ISSN: , DOI: 10.5281/zenodo.1478742
2019-05-27
2018 George, Michael; Reif, Phillip; Zhang, Gui-Rong; Etzold, Bastian JM
Boosting the ORR Performance of PtNi/C Catalysts with Ionic Liquids: The influence of Carbon Support
published pages: , ISSN: , DOI: 10.5281/zenodo.1478778
2019-05-27
2018 Zhang, Gui-Rong; Wolker, Thomas; Sandbeck, Daniel; Munoz, Macarena; Mayrhofer, Karl; Etzold, Bastian JM
Tuning the Electrocatalytic Performance of Ionic Liquid Modified Pt Catalysts for Oxygen Reduction Reaction by Cationic Chain Engineering
published pages: , ISSN: , DOI: 10.5281/zenodo.1478762
2019-05-13
2018 Zhang, Gui-Rong; Wolker, Thomas; Sandbeck, Daniel; Munoz, Macarena; Mayrhofer, Karl; Cherevko, Serhiy; Etzold, Bastian JM
Tuning the Electrocatalytic Performance of Ionic Liquid Modified Pt Catalysts for Oxygen Reduction Reaction via Cationic Chain Engineering
published pages: , ISSN: , DOI: 10.5281/zenodo.1480670
2019-05-13
2018 Ariyanto, Teguh; Zeiger, Marco; Zhang, Gui-Rong; Presser, Volker; Etzold, Bastian JM
Core-shell carbide-derived carbons as platform for high-performance electrochemical energy storage and electrocatalysis
published pages: , ISSN: , DOI: 10.5281/zenodo.1478698
2019-05-03
2018 Straub, Sascha-Dominic; Zhang, Gui-Rong; Etzold, Bastian JM
Influence of IL-modification on Cu based catalysts for the electrochemical reduction of CO2
published pages: , ISSN: , DOI: 10.5281/zenodo.1479013
2019-05-03
2018 Ioanna Martinaiou, Thomas Wolker, Ali Shahraei, Gui-Rong Zhang, Arne Janßen, Stephan Wagner, Natascha Weidler, Robert W. Stark, Bastian J.M. Etzold, Ulrike I. Kramm
Improved electrochemical performance of Fe-N-C catalysts through ionic liquid modification in alkaline media
published pages: 222-232, ISSN: 0378-7753, DOI: 10.1016/j.jpowsour.2017.07.028
Journal of Power Sources 375 2019-05-03
2018 Wolker, Thomas; Martinaiou, Ioanna; Shahraei, Ali; Zhang, Gui-Rong; Janßen, A.; Wagner, Stephan; Weidler, Natascha; Stark, Robert W; Etzold, Bastian JM; Kramm, Ulrike I
Improved electrochemical performance of Fe-N-C catalysts through ionic liquid modification in alkaline media
published pages: , ISSN: , DOI: 10.5281/zenodo.1478774
2019-05-03
2018 Gui-Rong Zhang, Thomas Wolker, Daniel J. S. Sandbeck, Macarena Munoz, Karl J. J. Mayrhofer, Serhiy Cherevko, Bastian J. M. Etzold
Tuning the Electrocatalytic Performance of Ionic Liquid Modified Pt Catalysts for the Oxygen Reduction Reaction via Cationic Chain Engineering
published pages: 8244-8254, ISSN: 2155-5435, DOI: 10.1021/acscatal.8b02018
ACS Catalysis 8/9 2019-05-03
2018 Shen, Liu-Liu; Zhang, Gui-Rong; Venter, Tizian; Biesalski, Markus; Etzold, Bastian JM
Towards Best Practices for Improving Paper-Based Microfluidic Fuel Cells
published pages: , ISSN: , DOI: 10.5281/zenodo.1478757
2019-05-03
2018 Wolker, Thomas; Martinaiou, Ioanna; Shahraei, Ali; Zhang, Gui-Rong; Janßen, A.; Wagner, Stephan; Weidler, Natascha; Stark, Robert W; Etzold, Bastian JM; Kramm, Ulrike I
Improved electrochemical performance of Fe-N-C catalysts through ionic liquid modification
published pages: , ISSN: , DOI: 10.5281/zenodo.1478750
2019-05-03
2018 Wöllner, Sebastian; Zhang, Gui-Rong; Rockstroh, Nils; Brückner, Angelika; Etzold, Bastian JM
Electrooxidation of water and 5-Hydroxymethylfurfural (HMF) on non-noble multi metal catalysts
published pages: , ISSN: , DOI: 10.5281/zenodo.1479111
2019-05-03
2018 Steldinger, Hendryk; Gläsel, Jan; Etzold, Bastian JM
High Surface Area Activated Carbon Monolith from 3D Printed
published pages: , ISSN: , DOI: 10.5281/zenodo.1478767
2019-05-03

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