CSI.interface SIGNED
A molecular interface science approach: Decoding single molecular reactions and interactions at dynamic solid/liquid interfaces
Total Cost €
0EC-Contrib. €
0Partnership
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Project "CSI.interface" data sheet
The following table provides information about the project.
| Coordinator |
TECHNISCHE UNIVERSITAET WIEN
Organization address contact info |
| Coordinator Country | Austria [AT] |
| Project website | http://www.iap.tuwien.ac.at/www/interface/index |
| Total cost | 1˙499˙750 € |
| EC max contribution | 1˙499˙750 € (100%) |
| Programme |
1. H2020-EU.1.1. (EXCELLENT SCIENCE - European Research Council (ERC)) |
| Code Call | ERC-2015-STG |
| Funding Scheme | ERC-STG |
| Starting year | 2016 |
| Duration (year-month-day) | from 2016-07-01 to 2021-06-30 |
Partnership
Take a look of project's partnership.
| # | ||||
|---|---|---|---|---|
| 1 | TECHNISCHE UNIVERSITAET WIEN | AT (WIEN) | coordinator | 1˙146˙875.00 |
| 2 | TECHNISCHE UNIVERSITAET BERGAKADEMIE FREIBERG | DE (FREIBERG) | participant | 352˙875.00 |
Map
Project objective
After decades of truly transformative advancements in single molecule (bio)physics and surface science, it is still no more than a vision to predict and control macroscopic phenomena such as adhesion or electrochemical reaction rates at solid/liquid interfaces based on well-characterized single molecular interactions. How exactly do inherently dynamic and simultaneous interactions of a countless number of interacting “crowded” molecules lead to a concerted outcome/property on a macroscopic scale? Here, I propose a unique approach that will allow us to unravel the scaling of single molecule interactions towards macroscopic properties at adhesive and redox-active solid/liquid interfaces. Combining Atomic Force Microscopy (AFM) based single molecule force spectroscopy and macroscopic Surface Forces Apparatus (SFA) experiments CSI.interface will (1) derive rules for describing nonlinearities observed in complex, crowded (water and ions) and chemically diverse adhesive solid/liquid interfaces; (2) uniquely characterize all relevant kinetic parameters (interaction free energy and transition states) of electrochemical and adhesive reactions/interactions of single molecules at chemically defined surfaces as well as electrified single crystal facets and step edges. Complementary, (3) my team and I will build a novel molecular force apparatus in order to measure single-molecule steady-state dynamics of both redox cycles as well as binding unbinding cycles of specific interactions, and how these react to environmental triggers. CSI.interface goes well beyond present applications of AFM and SFA and has the long-term potential to revolutionize our understanding of interfacial interaction under steady state, responsive and dynamic conditions. This work will pave the road for knowledge based designing of next-generation technologies in gluing, coating, bio-adhesion, materials design and much beyond.
Publications
| year | authors and title | journal | last update |
|---|---|---|---|
| 2017 |
Philipp Stock, Jacob I. Monroe, Thomas Utzig, David J. Smith, M. Scott Shell, Markus Valtiner Unraveling Hydrophobic Interactions at the Molecular Scale Using Force Spectroscopy and Molecular Dynamics Simulations published pages: 2586-2597, ISSN: 1936-0851, DOI: 10.1021/acsnano.6b06360 |
ACS Nano 11/3 | 2019-06-19 |
| 2017 |
Qingyun Hu, Christian Weber, Hsiu-Wei Cheng, Frank Uwe Renner, Markus Valtiner Anion Layering and Steric Hydration Repulsion on Positively Charged Surfaces in Aqueous Electrolytes published pages: 3056-3065, ISSN: 1439-4235, DOI: 10.1002/cphc.201700865 |
ChemPhysChem 18/21 | 2019-06-19 |
| 2019 |
Claudia Merola, Hsiuâ€Wei Cheng, Dominik Dworschak, Chingâ€Shun Ku, Chingâ€Yu Chiang, Frank Uwe Renner, Markus Valtiner Nanometer Resolved Real Time Visualization of Acidification and Material Breakdown in Confinement published pages: 1802069, ISSN: 2196-7350, DOI: 10.1002/admi.201802069 |
Advanced Materials Interfaces | 2019-05-27 |
| 2019 |
Kai A. Schwenzfeier, Andreas Erbe, Pierluigi Bilotto, Maximilian Lengauer, Claudia Merola, Hsiu-Wei Cheng, Laura L. E. Mears, Markus Valtiner Optimizing multiple beam interferometry in the surface forces apparatus: Novel optics, reflection mode modeling, metal layer thicknesses, birefringence, and rotation of anisotropic layers published pages: 43908, ISSN: 0034-6748, DOI: 10.1063/1.5085210 |
Review of Scientific Instruments 90/4 | 2019-05-27 |
| 2017 |
Laila Moreno Ostertag, Thomas Utzig, Christine Klinger, Markus Valtiner Tether-Length Dependence of Bias in Equilibrium Free-Energy Estimates for Surface-to-Molecule Unbinding Experiments published pages: 766-772, ISSN: 0743-7463, DOI: 10.1021/acs.langmuir.7b02844 |
Langmuir 34/3 | 2019-03-12 |
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