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SEARCh SIGNED

SurfacE structure-Activity-Relationship in atomically-defined, ultrathin film perovskite Catalysts

Total Cost €

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EC-Contrib. €

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Partnership

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 SEARCh project word cloud

Explore the words cloud of the SEARCh project. It provides you a very rough idea of what is the project "SEARCh" about.

structures    electrocatalyst    neutral    mechanisms    deduce    ni    influence    film    world    epitaxial    due    communicate    techniques    crystallographic    amorphous    perovskite    oxy    relationships    receive    hydr    transition    composition    scattering    lengths    spectroscopy    commercial    carbon    underlying    electrolysers    orientation    electronic    record    cutting    goals    transferable    characterization    technologies    deployment    structure    edge    training    rules    renewable    stable    oxides    probe    performance    attractive    penetration    electrocatalysts    hindered    multidisciplinary    energy    climate    skills    hydrogen    line    materials    fe    revalidate    strategic    surface    electricity    scanning    sustainable    bond    atomically    absence    benefitting    atomistic    tools    attain    operando    atomic    candidate    unattainable    market    reaction    fuel    chemical    catalysts    synchrotron    disseminating    abundant    conversion    catalysis    found    earth    thin    degradation    catalytic    substantial    researcher    catalyst    inexpensive    innovative    intermittency    plan    polycrystalline    search    electrolysis    undefined    bulk    termination    international    communities    derive   

Project "SEARCh" data sheet

The following table provides information about the project.

Coordinator
RHEINISCH-WESTFAELISCHE TECHNISCHE HOCHSCHULE AACHEN 

Organization address
address: TEMPLERGRABEN 55
city: AACHEN
postcode: 52062
website: www.rwth-aachen.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Project website http://www.epicatalysts.rwth-aachen.de
 Total cost 214˙828 €
 EC max contribution 214˙828 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2017
 Funding Scheme MSCA-IF-GF
 Starting year 2018
 Duration (year-month-day) from 2018-06-01   to  2020-11-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    RHEINISCH-WESTFAELISCHE TECHNISCHE HOCHSCHULE AACHEN DE (AACHEN) coordinator 214˙828.00
2    BOARD OF TRUSTEES OF THE LELAND STANFORD JUNIOR UNIVERSITY US (STANFORD) partner 0.00

Map

 Project objective

Due to the intermittency of renewable electricity, conversion to chemical fuel is a necessity for the success of the transition to sustainable energy. A simple and attractive candidate for climate-neutral fuel is hydrogen, which can be produced directly through electrolysis. But substantial market penetration by commercial electrolysers has been hindered by the absence of high-activity, stable, inexpensive, and earth-abundant, catalytic materials. To develop and exploit these materials, a detailed understanding of the underlying relationships between catalytic activity and atomic-level surface structure is required, which has so far been unattainable due to often-case undefined surface areas and structures, as is the case for today’s record-performance electrocatalysts, i.e. Ni-Fe (oxy)(hydr)oxides. Therefore, epitaxial, atomically defined Ni-Fe-based perovskite thin film catalysts will be investigated with advanced operando characterization tools (including synchrotron-based scattering and spectroscopy, and scanning probe approaches) to achieve the following objectives:

- Revalidate activity trends found for polycrystalline and amorphous structures, disseminating the influence from the bulk electronic structure (composition), bond lengths, crystallographic orientation and surface termination

- Derive an atomistic understanding of the catalysis reaction and degradation mechanisms

- Deduce design rules for beyond-state-of-the-art electrocatalyst materials and communicate them to the catalyst research and production communities for exploitation in “real-world” catalyst materials

The results of SEARCh will thus contribute to the goals of development and deployment of low-carbon technologies in line with the EU’s Strategic Energy Technology Plan and the experienced researcher will receive training in innovative, cutting-edge techniques and attain transferable skills, benefitting from a multidisciplinary, international collaboration.

 Publications

year authors and title journal last update
List of publications.
2020 Felix V. E. Hensling, Christoph Baeumer, Marc-André Rose, Felix Gunkel, Regina Dittmann
SrTiO 3 termination control: a method to tailor the oxygen exchange kinetics
published pages: 31-40, ISSN: 2166-3831, DOI: 10.1080/21663831.2019.1682705
Materials Research Letters 8/1 2020-01-30
2019 Venkata R. Nallagatla, Thomas Heisig, Christoph Baeumer, Vitaliy Feyer, Matteo Jugovac, Giovanni Zamborlini, Claus M. Schneider, Rainer Waser, Miyoung Kim, Chang Uk Jung, Regina Dittmann
Topotactic Phase Transition Driving Memristive Behavior
published pages: 1903391, ISSN: 0935-9648, DOI: 10.1002/adma.201903391
Advanced Materials 31/40 2019-10-29
2019 Moritz L. Weber, Christoph Baeumer, David N. Mueller, Lei Jin, Chun-Lin Jia, Daniel S. Bick, Rainer Waser, Regina Dittmann, Ilia Valov, Felix Gunkel
Electrolysis of Water at Atomically Tailored Epitaxial Cobaltite Surfaces
published pages: 2337-2346, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.8b04577
Chemistry of Materials 31/7 2019-10-10

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