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SEARCh SIGNED

SurfacE structure-Activity-Relationship in atomically-defined, ultrathin film perovskite Catalysts

Total Cost €

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EC-Contrib. €

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Partnership

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 SEARCh project word cloud

Explore the words cloud of the SEARCh project. It provides you a very rough idea of what is the project "SEARCh" about.

electrocatalysts    search    oxy    innovative    market    attractive    training    goals    abundant    mechanisms    carbon    undefined    world    synchrotron    catalysis    scattering    deployment    crystallographic    researcher    attain    bond    international    operando    characterization    line    found    electricity    communicate    relationships    materials    atomically    rules    stable    amorphous    commercial    catalytic    perovskite    sustainable    energy    technologies    electronic    multidisciplinary    due    candidate    unattainable    spectroscopy    orientation    revalidate    thin    reaction    catalyst    inexpensive    derive    disseminating    electrolysis    degradation    penetration    receive    cutting    composition    chemical    ni    structure    surface    performance    scanning    record    termination    absence    transferable    epitaxial    underlying    renewable    atomic    intermittency    benefitting    film    tools    strategic    probe    bulk    climate    communities    atomistic    hindered    transition    fe    conversion    neutral    earth    deduce    edge    influence    oxides    lengths    substantial    hydrogen    catalysts    electrocatalyst    structures    hydr    techniques    polycrystalline    electrolysers    skills    fuel    plan   

Project "SEARCh" data sheet

The following table provides information about the project.

Coordinator
RHEINISCH-WESTFAELISCHE TECHNISCHE HOCHSCHULE AACHEN 

Organization address
address: TEMPLERGRABEN 55
city: AACHEN
postcode: 52062
website: www.rwth-aachen.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Project website http://www.epicatalysts.rwth-aachen.de
 Total cost 214˙828 €
 EC max contribution 214˙828 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2017
 Funding Scheme MSCA-IF-GF
 Starting year 2018
 Duration (year-month-day) from 2018-06-01   to  2020-11-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    RHEINISCH-WESTFAELISCHE TECHNISCHE HOCHSCHULE AACHEN DE (AACHEN) coordinator 214˙828.00
2    BOARD OF TRUSTEES OF THE LELAND STANFORD JUNIOR UNIVERSITY US (STANFORD) partner 0.00

Map

 Project objective

Due to the intermittency of renewable electricity, conversion to chemical fuel is a necessity for the success of the transition to sustainable energy. A simple and attractive candidate for climate-neutral fuel is hydrogen, which can be produced directly through electrolysis. But substantial market penetration by commercial electrolysers has been hindered by the absence of high-activity, stable, inexpensive, and earth-abundant, catalytic materials. To develop and exploit these materials, a detailed understanding of the underlying relationships between catalytic activity and atomic-level surface structure is required, which has so far been unattainable due to often-case undefined surface areas and structures, as is the case for today’s record-performance electrocatalysts, i.e. Ni-Fe (oxy)(hydr)oxides. Therefore, epitaxial, atomically defined Ni-Fe-based perovskite thin film catalysts will be investigated with advanced operando characterization tools (including synchrotron-based scattering and spectroscopy, and scanning probe approaches) to achieve the following objectives:

- Revalidate activity trends found for polycrystalline and amorphous structures, disseminating the influence from the bulk electronic structure (composition), bond lengths, crystallographic orientation and surface termination

- Derive an atomistic understanding of the catalysis reaction and degradation mechanisms

- Deduce design rules for beyond-state-of-the-art electrocatalyst materials and communicate them to the catalyst research and production communities for exploitation in “real-world” catalyst materials

The results of SEARCh will thus contribute to the goals of development and deployment of low-carbon technologies in line with the EU’s Strategic Energy Technology Plan and the experienced researcher will receive training in innovative, cutting-edge techniques and attain transferable skills, benefitting from a multidisciplinary, international collaboration.

 Publications

year authors and title journal last update
List of publications.
2020 Felix V. E. Hensling, Christoph Baeumer, Marc-André Rose, Felix Gunkel, Regina Dittmann
SrTiO 3 termination control: a method to tailor the oxygen exchange kinetics
published pages: 31-40, ISSN: 2166-3831, DOI: 10.1080/21663831.2019.1682705
Materials Research Letters 8/1 2020-01-30
2019 Venkata R. Nallagatla, Thomas Heisig, Christoph Baeumer, Vitaliy Feyer, Matteo Jugovac, Giovanni Zamborlini, Claus M. Schneider, Rainer Waser, Miyoung Kim, Chang Uk Jung, Regina Dittmann
Topotactic Phase Transition Driving Memristive Behavior
published pages: 1903391, ISSN: 0935-9648, DOI: 10.1002/adma.201903391
Advanced Materials 31/40 2019-10-29
2019 Moritz L. Weber, Christoph Baeumer, David N. Mueller, Lei Jin, Chun-Lin Jia, Daniel S. Bick, Rainer Waser, Regina Dittmann, Ilia Valov, Felix Gunkel
Electrolysis of Water at Atomically Tailored Epitaxial Cobaltite Surfaces
published pages: 2337-2346, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.8b04577
Chemistry of Materials 31/7 2019-10-10

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