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SEARCh SIGNED

SurfacE structure-Activity-Relationship in atomically-defined, ultrathin film perovskite Catalysts

Total Cost €

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EC-Contrib. €

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Partnership

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 SEARCh project word cloud

Explore the words cloud of the SEARCh project. It provides you a very rough idea of what is the project "SEARCh" about.

atomistic    commercial    intermittency    unattainable    operando    electrocatalysts    absence    revalidate    deployment    communicate    chemical    structures    synchrotron    sustainable    carbon    penetration    tools    lengths    electronic    abundant    fe    record    atomically    atomic    scattering    market    catalytic    search    disseminating    found    amorphous    electrolysers    catalysis    skills    structure    climate    catalysts    deduce    influence    world    materials    thin    researcher    hydr    rules    training    international    attain    mechanisms    conversion    electrocatalyst    composition    communities    cutting    line    orientation    oxides    transition    renewable    bond    edge    undefined    receive    techniques    inexpensive    due    derive    multidisciplinary    underlying    stable    degradation    substantial    surface    probe    perovskite    plan    electricity    crystallographic    hydrogen    reaction    transferable    performance    strategic    energy    ni    neutral    scanning    termination    benefitting    relationships    epitaxial    fuel    film    electrolysis    earth    hindered    candidate    polycrystalline    innovative    goals    characterization    catalyst    attractive    technologies    oxy    spectroscopy    bulk   

Project "SEARCh" data sheet

The following table provides information about the project.

Coordinator
RHEINISCH-WESTFAELISCHE TECHNISCHE HOCHSCHULE AACHEN 

Organization address
address: TEMPLERGRABEN 55
city: AACHEN
postcode: 52062
website: www.rwth-aachen.de

contact info
title: n.a.
name: n.a.
surname: n.a.
function: n.a.
email: n.a.
telephone: n.a.
fax: n.a.

 Coordinator Country Germany [DE]
 Project website http://www.epicatalysts.rwth-aachen.de
 Total cost 214˙828 €
 EC max contribution 214˙828 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2017
 Funding Scheme MSCA-IF-GF
 Starting year 2018
 Duration (year-month-day) from 2018-06-01   to  2020-11-30

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    RHEINISCH-WESTFAELISCHE TECHNISCHE HOCHSCHULE AACHEN DE (AACHEN) coordinator 214˙828.00
2    BOARD OF TRUSTEES OF THE LELAND STANFORD JUNIOR UNIVERSITY US (STANFORD) partner 0.00

Map

 Project objective

Due to the intermittency of renewable electricity, conversion to chemical fuel is a necessity for the success of the transition to sustainable energy. A simple and attractive candidate for climate-neutral fuel is hydrogen, which can be produced directly through electrolysis. But substantial market penetration by commercial electrolysers has been hindered by the absence of high-activity, stable, inexpensive, and earth-abundant, catalytic materials. To develop and exploit these materials, a detailed understanding of the underlying relationships between catalytic activity and atomic-level surface structure is required, which has so far been unattainable due to often-case undefined surface areas and structures, as is the case for today’s record-performance electrocatalysts, i.e. Ni-Fe (oxy)(hydr)oxides. Therefore, epitaxial, atomically defined Ni-Fe-based perovskite thin film catalysts will be investigated with advanced operando characterization tools (including synchrotron-based scattering and spectroscopy, and scanning probe approaches) to achieve the following objectives:

- Revalidate activity trends found for polycrystalline and amorphous structures, disseminating the influence from the bulk electronic structure (composition), bond lengths, crystallographic orientation and surface termination

- Derive an atomistic understanding of the catalysis reaction and degradation mechanisms

- Deduce design rules for beyond-state-of-the-art electrocatalyst materials and communicate them to the catalyst research and production communities for exploitation in “real-world” catalyst materials

The results of SEARCh will thus contribute to the goals of development and deployment of low-carbon technologies in line with the EU’s Strategic Energy Technology Plan and the experienced researcher will receive training in innovative, cutting-edge techniques and attain transferable skills, benefitting from a multidisciplinary, international collaboration.

 Publications

year authors and title journal last update
List of publications.
2020 Felix V. E. Hensling, Christoph Baeumer, Marc-André Rose, Felix Gunkel, Regina Dittmann
SrTiO 3 termination control: a method to tailor the oxygen exchange kinetics
published pages: 31-40, ISSN: 2166-3831, DOI: 10.1080/21663831.2019.1682705
Materials Research Letters 8/1 2020-01-30
2019 Venkata R. Nallagatla, Thomas Heisig, Christoph Baeumer, Vitaliy Feyer, Matteo Jugovac, Giovanni Zamborlini, Claus M. Schneider, Rainer Waser, Miyoung Kim, Chang Uk Jung, Regina Dittmann
Topotactic Phase Transition Driving Memristive Behavior
published pages: 1903391, ISSN: 0935-9648, DOI: 10.1002/adma.201903391
Advanced Materials 31/40 2019-10-29
2019 Moritz L. Weber, Christoph Baeumer, David N. Mueller, Lei Jin, Chun-Lin Jia, Daniel S. Bick, Rainer Waser, Regina Dittmann, Ilia Valov, Felix Gunkel
Electrolysis of Water at Atomically Tailored Epitaxial Cobaltite Surfaces
published pages: 2337-2346, ISSN: 0897-4756, DOI: 10.1021/acs.chemmater.8b04577
Chemistry of Materials 31/7 2019-10-10

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