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ORRmetIR SIGNED

Development and in situ Infrared study of Novel Strained Core-shell Electrocatalysts: Towards an Understanding of the Oxygen Reduction Mechanism

Total Cost €

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EC-Contrib. €

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Partnership

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 Outcomes and results

 ORRmetIR project word cloud

Explore the words cloud of the ORRmetIR project. It provides you a very rough idea of what is the project "ORRmetIR" about.

hindered    fuels    interpretation    team    nanomaterial    combines    culture    catalysts    host    university    collaborations    time    horizon    inexpensive    property    barrier    critical    broad    featuring    spectroscopy    academic    generation    kinetics    electrocatalysts    synthesising    strained    efficient    infrared    electrocatalysis    expertise    transfer    vincent    synthesis    cells    group    training    infrastructure    impacts    structure    receive    oxygen    sluggish    ranging    sectors    metals    catalytic    pt    hosted    skills    ni    electrochemistry    fellow    renewable    turnover    combining    goals    hydrogen    cu    benefit    aiding    intermediates    characterisation    fc    commercialisation    strain    materials    interdisciplinary    competitiveness    industrial    nanoparticles    core    first    oxford    electricity    suited    spectral    metal    supporting    2020    implementing    fuel    surface    orr    energy    spectroscopic    co    modifying    catalysis    situ    operando    reaction    intellectual    gained    corrosion    vibrational    alcohols    mechanism    understand    security    poor    techniques    uniquely    shell    ir    realistic    batteries   

Project "ORRmetIR" data sheet

The following table provides information about the project.

Coordinator		 THE CHANCELLOR, MASTERS AND SCHOLARS OF THE UNIVERSITY OF OXFORD 

Organization address
address: WELLINGTON SQUARE UNIVERSITY OFFICES
city: OXFORD
postcode: OX1 2JD
website: www.ox.ac.uk

contact info
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email: n.a.
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 Coordinator Country United Kingdom [UK]
 Project website http://vincent.chem.ox.ac.uk/
 Total cost 195˙454 €
 EC max contribution 195˙454 € (100%)
 Programme 1. H2020-EU.1.3.2. (Nurturing excellence by means of cross-border and cross-sector mobility)
 Code Call H2020-MSCA-IF-2014
 Funding Scheme MSCA-IF-EF-ST
 Starting year 2015
 Duration (year-month-day) from 2015-04-01   to  2017-03-31

 Partnership

Take a look of project's partnership.

# participants  country  role  EC contrib. [€] 
1    THE CHANCELLOR, MASTERS AND SCHOLARS OF THE UNIVERSITY OF OXFORD UK (OXFORD) coordinator 195˙454.00

Map

 Project objective

The oxygen reduction reaction (ORR) is critical in fuel cells (FC), batteries and corrosion. Sluggish kinetics of the ORR remains a key barrier to efficient electricity generation in FC operating on renewable fuels such as hydrogen or alcohols. Poor understanding of the ORR mechanism has hindered development of cost-effective and improved FC catalysts. This project aims to bring about a step change in development and understanding of ORR catalysts by (i) synthesising metal nanoparticles with a strained surface structure, and (ii) developing and implementing new in situ and operando infrared (IR) spectroscopic techniques to understand how strain impacts the ORR mechanism. Novel strained core-shell Pt-based catalysts will be developed, featuring a core of inexpensive metals including Ni, Co or Cu. For the first time, insight into the ORR mechanism for supported electrocatalysts under realistic catalytic turnover will be gained by modifying an approach to combining IR spectroscopy and electrochemistry developed in the Vincent group. The University of Oxford is uniquely suited for this ambitious project: the applicant will be hosted in a strong research culture in catalysis, have access to state-of-the-art research infrastructure and technical expertise in spectroscopy and materials characterisation and industrial collaborations. The fellow will receive broad-ranging training in the synthesis of catalysts and surface characterisation. The host team will benefit from her skills in in situ vibrational spectroscopy, especially spectral interpretation of ORR intermediates. This highly interdisciplinary project combines nanomaterial synthesis, spectroscopy and electrocatalysis, and has strong potential for generation of intellectual property and commercialisation of new catalysts for FC, aiding knowledge transfer between academic and industrial sectors. This will increase Europe’s competitiveness in FC and electrocatalysis, supporting Horizon 2020’s Energy Security goals.

 Publications

year authors and title journal last update
List of publications.
2016 Pabitra K. Nayak, David T. Moore, Bernard Wenger, Simantini Nayak, Amir A. Haghighirad, Adam Fineberg, Nakita K. Noel, Obadiah G. Reid, Garry Rumbles, Philipp Kukura, Kylie A. Vincent, Henry J. Snaith
Mechanism for rapid growth of organic–inorganic halide perovskite crystals
published pages: 13303, ISSN: 2041-1723, DOI: 10.1038/ncomms13303 		Nature Communications 7 2019-06-17
2017 Nobuya Sakai, Amir Abbas Haghighirad, Marina R. Filip, Pabitra K. Nayak, Simantini Nayak, Alexandra Ramadan, Zhiping Wang, Feliciano Giustino, Henry J. Snaith
Solution-Processed Cesium Hexabromopalladate(IV), Cs 2 PdBr 6 , for Optoelectronic Applications
published pages: 6030-6033, ISSN: 0002-7863, DOI: 10.1021/jacs.6b13258 		Journal of the American Chemical Society 139/17 2019-06-17
2016 Sha Li, Shanshan Wang, Matteo M. Salamone, Alex W. Robertson, Simantini Nayak, Heeyeon Kim, S. C. Edman Tsang, Mauro Pasta, Jamie H. Warner
Edge-Enriched 2D MoS 2 Thin Films Grown by Chemical Vapor Deposition for Enhanced Catalytic Performance
published pages: 877-886, ISSN: 2155-5435, DOI: 10.1021/acscatal.6b02663 		ACS Catalysis 7/1 2019-06-17
2016 Philip A. Ash, Holly A. Reeve, Jonathan Quinson, Ricardo Hidalgo, Tianze Zhu, Ian J. McPherson, Min-Wen Chung, Adam J. Healy, Simantini Nayak, Thomas H. Lonsdale, Katia Wehbe, Chris S. Kelley, Mark D. Frogley, Gianfelice Cinque, Kylie A. Vincent
Synchrotron-Based Infrared Microanalysis of Biological Redox Processes under Electrochemical Control
published pages: 6666-6671, ISSN: 0003-2700, DOI: 10.1021/acs.analchem.6b00898 		Analytical Chemistry 88/13 2019-06-17

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